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An Effective Method for Adsorption of Pb2 , Cd2 , and Cu2 from Wastewater by Using NaXZeolite-Derived from Coal Gangue

DOI: 10.4236/oalib.1109102, PP. 1-12

Subject Areas: Environmental Sciences, Hydrology

Keywords: Coal Gangue, Adsorption of Pb2 , Cu2 and Cd2 , NaXzeolite, Langmuir, Freundlich and Temkin Isotherms

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Abstract

A study was conducted to investigate the behavior and mechanics of NaXzeolite on the adsorption of (Pb2 , Cd2 , and Cu2 ) from simulated wastewater. NaXzeolite was synthesized from coal gangue by an Alkali-based hydrothermal process. A number of techniques have been employed to analyze the production of adsorbents, including X-ray diffraction (XRD), scanning electron microscopy with X-ray energy analysis (SEM-EDX), Fourier transform infrared (FT-IR), X-ray fluorescent (XRF), and Brunauer-Emmett-Teller (BET). The effects of adsorbent dosage, pH, time, temperature, and initial concentration of NaXzeolite on the adsorption of Pb2 , Cd2 , and Cu2 were investigated. To investigate the mechanisms and capacities of experimental adsorption, Langmuir, Freundlich, and Temkin isotherms were employed. In certain conditions, the Langmuir isotherm showed that the adsorbent layer had an adsorption capacity of 88.3, 87.9 and 88.5 mg/g of Pb2 , Cu2 and Cd2 , with linear regression coefficients (R2 > 0.979) for all three metals. Bioavailability, Optimal doses of 0.5 g/L NaXzeolite at pH of 5 & 6 in condition 25°C in 90 minutes removed >99% for all three metals.

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Ahmadi, H. , Duan, Y. , Hussain, S. , Hafiz, S. S. , Sharifi, H. and Habibi, S. S. (2022). An Effective Method for Adsorption of Pb2 , Cd2 , and Cu2 from Wastewater by Using NaXZeolite-Derived from Coal Gangue. Open Access Library Journal, 9, e9102. doi: http://dx.doi.org/10.4236/oalib.1109102.

References

[1]  Jung, K., Choi, B., Jeong, T. and Ahn, K. (2016) Facile Synthesis of Magnetic bio-Char/Fe3O4 Nanocomposites Using Electro-Magnetization Technique and Its Application on the Removal of Acid Orange 7 from Aqueous Media. Bioresource Technology, 220, 672-676. https://doi.org/10.1016/j.biortech.2016.09.035
[2]  Jin, H., Capareda, S., Chang, Z., Gao, J., Xu, Y. and Zhang, J. (2014) Biochar Pyrolytically Produced from Municipal Solid Wastes for Aqueous As (V) Removal: Adsorption Property and Its Improvement with KOH Activation. Bioresource technology, 169, 622-629. https://doi.org/10.1016/j.biortech.2014.06.103
[3]  Ding, Z., Hu, X., Wan, Y., Wang, S. and Gao, B. (2016). Removal of Lead, Copper, Cadmium, Zinc, and Nickel from Aqueous Solutions by Alkali-Modified Biochar: Batch and Column Tests. Journal of Industrial and Engineering Chemistry, 33, 239-245. https://doi.org/10.1016/j.jiec.2015.10.007
[4]  Yang, G.X. and Jiang, H. (2014) Amino Modification of Biochar for Enhanced Adsorption of Copper Ions from Synthetic Wastewater. Water Research, 48, 396-405. https://doi.org/10.1016/j.watres.2013.09.050
[5]  Zhu, X., Liu, Y., Qian, F., Zhou, C., Zhang, S. and Chen, J. (2014) Preparation of Magnetic Porous Carbon from Waste Hydrochar by Simultaneous Activation and Magnetization for Tetracycline Removal. Bioresource Technology, 154, 209-214. https://doi.org/10.1016/j.biortech.2013.12.019
[6]  Zhou, N., Chen, H., Feng, Q., Yao, D., Chen, H.,Wang, H. and Lu, X. (2017a) Effect of Phosphoric Acid on the Surface Properties and Pb(II) Adsorption Mechanisms of Hydrochars Prepared from Fresh Banana Peels. Journal of Cleaner Production, 165, 221-230. https://doi.org/10.1016/j.jclepro.2017.07.111
[7]  Peligro, F., Pavlovic, L., Rojas, R. and Barriga, C. (2016) Removal of Heavy Metals from Simulated Wastewater by in Situ Formation of Layered Double Hydroxides. Chemical Engineering Journal, 306, 1035-1040. https://doi.org/10.1016/j.cej.2016.08.054
[8]  Fu, F. and Wang, Q. (2011) Removal of Heavy Metal Ions from Wastewaters: A Review. Journal of Environmental Management, 92, 407-418. https://doi.org/10.1016/j.jenvman.2010.11.011
[9]  Huang, Z., Lu, L., Cai, Z. and Ren, Z. (2016) Individual and Competitive Removal of Heavy Metals Using Capacitive Deionization. Journal of Hazardous Materials, 302, 323-331. https://doi.org/10.1016/j.jhazmat.2015.09.064
[10]  Shen, Y., Zhao, P., Shao, Q., Ma, D., Takahashi, F. and Yoshikawa, K. (2014) In-situ Catalytic Conversion of Tar Using Rice Husk Char-Supported Nickel-Iron Catalysts for Biomass Pyrolysis/ Gasification. Applied Catalysis B: Environmental, 152-153, 140-151. https://doi.org/10.1016/j.apcatb.2014.01.032
[11]  Vukovic, G.D., Marinkovic, A.D., Colic, M., Ristic, M.D., Aleksic, R., Peric-Grujic, A.A. and Uskokovic, P.S. (2010) Removal of Cadmium from Aqueous Solutions by Oxidized and Ethylenediamine-Functionalized Multi-Walled Carbon Nano-tubes. Chemical Engineering Journal, 157, 238-248. https://doi.org/10.1016/j.cej.2009.11.026
[12]  Poonam, B.S.K. and Kumar, N. (2018) Kinetic Study of Lead (Pb2 ) Removal from Battery Manufacturing Wastewater Using Bagasse Biochar as Biosorbent. Applied Water Science, 8, Article No. 119. https://doi.org/10.1007/s13201-018-0765-z
[13]  Qin, L. and Gao, X. (2019) Properties of Coal Gangue-Portland Cement Mixture with Carbonation. Fuel, 245, 1-12. https://doi.org/10.1016/j.fuel.2019.02.067

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