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An Insight in Electrocoagulation Process through Current Density Distribution (CDD)

DOI: 10.4236/oalib.1106142, PP. 1-12

Subject Areas: Environmental Sciences

Keywords: Electrocoagulation, Computational Fluid Dynamic (CFD), Current Density Distribution (CDD), Natural Organic Matter (NOM), Fluoride, Arsenic

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Abstract

Electrocoagulation (EC) is a flourishing technique in the field of water treatment implementations. Numerous investigations have been performed to assess the performance of EC to eliminate different pollutants; however, the more basic electrochemical features of the technique are usually ignored. Scientists such as McBeath et al. [1] provided an understanding of the essential link of water flow, electrochemical metal dissolution, and current density distribution (CDD) via computational fluid dynamic (CFD) models, mathematical models, and in situ CDD determination tests. They established, in theory, that current distributed over the electrode was inversely proportional to the water flow rate. By means of the CFD models and current distribution determining technique, they noted that current density was distributed unequally and pursued the tendency anticipated via theory. Eliminating natural organic matter was decreased as much as 79% when the inter-electrode distance was diminished from 10 to 1 mm. As a perspective, more efforts are required to better understand the CDD at the anodes surface and electric charges transfer from electrodes to the bulk of the solution. Mechanisms related to interactions of anodic metallic cations and various pollutants should be more investigated.

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Ghernaout, D. and Elboughdiri, N. (2020). An Insight in Electrocoagulation Process through Current Density Distribution (CDD). Open Access Library Journal, 7, e6142. doi: http://dx.doi.org/10.4236/oalib.1106142.

References

[1]  McBeath, S.T., Nouri-Khorasani, A., Mohseni, M. and Wilkinson, D.P. (2020) In-Situ Determination of Current Density Distribution and Fluid Modeling of an Electrocoagulation Process and Its Effects on Naturalorganic Matter Removal for Drinking Water Treatment. Water Research, 171, Article ID: 115404.
https://doi.org/10.1016/j.watres.2019.115404
[2]  Radjenovic, J. and Sedlak, D.L. (2015) Challenges and Opportunities for Electrochemical Processes as Next-Generation Technologies for the Treatment of Contaminated Water. Environmental Science & Technology, 49, 11292-11302.
https://doi.org/10.1021/acs.est.5b02414
[3]  Ghernaout, D., Ghernaout, B. and Naceur, M.W. (2011) Embodying the Chemical Water Treatment in the Green Chemistry: A Review. Desalination, 271, 1-10.
https://doi.org/10.1016/j.desal.2011.01.032
[4]  Ghernaout, D. (2017) Environmental Principles in the Holy Koran and the Sayings of the Prophet Muhammad. American Journal of Environmental Protection, 6, 75-79. https://doi.org/10.11648/j.ajep.20170603.13
[5]  Ghernaout, D., Elboughdiri, N. and Ghareba, S. (2020) Fenton Technology for Wastewater Treatment: Dares and Trends. Open Access Library Journal, 7, e6045.
https://doi.org/10.4236/oalib.1106045
[6]  Ghernaout, D., Naceur, M.W. and Ghernaout, B. (2011) A Review of Electrocoagulation as a Promising Coagulation Process for Improved Organic and Inorganic Matters Removal by Electrophoresis and Electroflotation. Desalination and Water Treatment, 28, 287-320. https://doi.org/10.5004/dwt.2011.1493
[7]  Ghernaout, D. (2018) Electrocoagulation Process: Achievements and Green Perspectives. Colloid and Surface Science, 3, 1-5.
https://doi.org/10.11648/j.css.20180301.11
[8]  Ghernaout, D. and Elboughdiri, N. (2020) Electrochemical Technology for Wastewater Treatment: Dares and Trends. Open Access Library Journal, 7, e6020.
https://doi.org/10.4236/oalib.1106020
[9]  Ghernaout, B., Ghernaout, D. and Saiba, A. (2010) Algae and Cyanotoxins Removal by Coagulation/Flocculation: A Review. Desalination and Water Treatment, 20, 133-143. https://doi.org/10.5004/dwt.2010.1202
[10]  Ghernaout, D. and Ghernaout, B. (2012) Sweep Flocculation as a Second Form of Charge Neutralization: A Review. Desalination and Water Treatment, 44, 15-28.
https://doi.org/10.1080/19443994.2012.691699
[11]  Ghernaout, D. and Ghernaout, B. (2012) On the Concept of the Future Drinking Water Treatment Plant: Algae Harvesting from the Algal Biomass for Biodiesel Production: A Review. Desalination and Water Treatment, 49, 1-18.
https://doi.org/10.1080/19443994.2012.708191
[12]  Ghernaout, D. (2014) The Hydrophilic/Hydrophobic Ratio vs. Dissolved Organics Removal by Coagulation: A Review. Journal of King Saud University-Science, 26, 169-180. https://doi.org/10.1016/j.jksus.2013.09.005
[13]  Ghernaout, D., Al-Ghonamy, A.I., Naceur, M.W., Ait Messaoudene, N. and Aichouni, M. (2014) Influence of Operating Parameters on Electrocoagulation of C.I. Disperse Yellow 3. Journal of Electrochemical Science and Engineering, 4, 271-283. https://doi.org/10.5599/jese.2014.0065
[14]  Ghernaout, D., Al-Ghonamy, A.I., Irki, S.,?Grini, A., Naceur, M.W., Ait Messaoudene, N. and Aichouni, M. (2014) Decolourization of Bromophenol Blue by Electrocoagulation Process. Trends in Chemical Engineering, 15, 29-39.
[15]  Ghernaout, D., Benblidia, C. and Khemici, F. (2015) Microalgae Removal from Ghrib Dam (Ain Defla, Algeria) Water by Electroflotation Using Stainless Steel Electrodes. Desalination and Water Treatment, 54, 3328-3337.
https://doi.org/10.1080/19443994.2014.907749
[16]  Ghernaout, D., Al-Ghonamy, A.I., Ait Messaoudene, N., Aichouni, M., Naceur, M.W., Benchelighem, F.Z. and Boucherit, A. (2015) Electrocoagulation of Direct Brown 2 (DB) and BF Cibacete Blue (CB) Using Aluminum Electrodes. Separation Science and Technology, 50, 1413-1420.
https://doi.org/10.1080/01496395.2014.982763
[17]  Ghernaout, D. (2017) Microorganisms’ Electrochemical Disinfection Phenomena. EC Microbiology, 9, 160-169.
[18]  Ghernaout, D., Aichouni, M. and Touahmia, M. (2019) Mechanistic Insight into Disinfection by Electrocoagulation: A Review. Desalination and Water Treatment, 141, 68-81. https://doi.org/10.5004/dwt.2019.23457
[19]  Ghernaout, D., Alghamdi, A. and Ghernaout, B. (2019) Microorganisms’ Killing: Chemical Disinfection vs. Electrodisinfection. Applied Engineering, 3, 13-19.
[20]  Ghernaout, D. (2019) Greening Electrocoagulation Process for Disinfecting Water. Applied Engineering, 3, 27-31.
[21]  Ghernaout, D. (2019) Electrocoagulation Process for Microalgal Biotechnology: A Review. Applied Engineering, 3, 85-94.
[22]  Ghernaout, D. (2019) Virus Removal by Electrocoagulation and Electrooxidation: New Findings and Future Trends. Journal of Environmental Science?and?Allied Research, 2019, 85-90. https://doi.org/10.29199/2637-7063/ESAR-202024
[23]  Ghernaout, D. (2019) Electrocoagulation and Electrooxidation for Disinfecting Water: New Breakthroughs and Implied Mechanisms. Applied Engineering, 3, 125-133.
[24]  Ghernaout, D., Badis, A., Ghernaout, B. and Kellil, A. (2008) Application of Electrocoagulation in Escherichia coli Culture and Two Surface Waters. Desalination, 219, 118-125. https://doi.org/10.1016/j.desal.2007.05.010
[25]  Ghernaout, D., Ghernaout, B. and Kellil, A. (2009) Natural Organic Matter Removal and Enhanced Coagulation as a Link between Coagulation and Electrocoagulation. Desalination and Water Treatment, 2, 203-222.
https://doi.org/10.5004/dwt.2009.116
[26]  Ghernaout, D., Ghernaout, B., Boucherit, A., Naceur, M.W., Khelifa, A. and Kellil, A. (2009) Study on Mechanism of Electrocoagulation with Iron Electrodes in Idealised Conditions and Electrocoagulation of Humic Acids Solution in Batch Using Aluminium Electrodes. Desalination and Water Treatment, 8, 91-99.
https://doi.org/10.5004/dwt.2009.668
[27]  Ghernaout, D., Ghernaout, B. and Boucherit, A. (2008) Effect of pH on Electrocoagulation of Bentonite Suspensions in Batch Using Iron Electrodes. Journal of Dispersion Science and Technology, 29, 1272-1275.
https://doi.org/10.1080/01932690701857483
[28]  Ghernaout, D., Ghernaout, B., Saiba, A., Boucherit, A. and Kellil, A. (2009) Removal of Humic Acids by Continuous Electromagnetic Treatment Followed by Electrocoagulation in Batch Using Aluminium Electrodes. Desalination, 239, 295-308.
https://doi.org/10.1016/j.desal.2008.04.001
[29]  Saiba, A., Kourdali, S., Ghernaout, B. and Ghernaout, D. (2010) In Desalination, from 1987 to 2009, the Birth of a New Seawater Pretreatment Process: Electrocoagulation: An Overview. Desalination and Water Treatment, 16, 201-217.
https://doi.org/10.5004/dwt.2010.1094
[30]  Ghernaout, D. (2013) Advanced Oxidation Phenomena in Electrocoagulation Process: A Myth or a Reality? Desalination and Water Treatment, 51, 7536-7554.
https://doi.org/10.1080/19443994.2013.792520
[31]  Belhout, D., Ghernaout, D., Djezzar-Douakh, S. and Kellil, A. (2010) Electrocoagulation of a Raw Water of Ghrib Dam (Algeria) in Batch Using Iron Electrodes. Desalination and Water Treatment, 16, 1-9. https://doi.org/10.5004/dwt.2010.1081
[32]  Ghernaout, D., Mariche, A., Ghernaout, B. and Kellil, A. (2010) Electromagnetic Treatment-Bi-Electrocoagulation of Humic Acid in Continuous Mode Using Response Surface Method for Its Optimization and Application on Two Surface Waters. Desalination and Water Treatment, 22, 311-329.
https://doi.org/10.5004/dwt.2010.1120
[33]  Ghernaout, D. and Naceur, M.W. (2011) Ferrate(VI): In Situ Generation and Water Treatment: A Review. Desalination and Water Treatment, 30, 319-332.
https://doi.org/10.5004/dwt.2011.2217
[34]  Ghernaout, D., Irki, S. and Boucherit, A. (2014) Removal of Cu2 and Cd2 , and Humic Acid and Phenol by Electrocoagulation Using Iron Electrodes. Desalination and Water Treatment, 52, 3256-3270.
https://doi.org/10.1080/19443994.2013.852484
[35]  Irki, S., Ghernaout, D. and Naceur, M.W. (2017) Decolourization of Methyl Orange (MO) by Electrocoagulation (EC) Using Iron Electrodes under a Magnetic Field (MF). Desalination and Water Treatment, 79, 368-377.
https://doi.org/10.5004/dwt.2017.20797
[36]  Irki, S., Ghernaout, D., Naceur, M.W., Alghamdi, A. and Aichouni, M. (2018) Decolorization of Methyl Orange (MO) by Electrocoagulation (EC) Using Iron Electrodes under a Magnetic Field (MF). II. Effect of Connection Mode. World Journal of Applied Chemistry, 3, 56-64.
https://doi.org/10.11648/j.wjac.20180302.13
[37]  Ghernaout, D. and Elboughdiri, N. (2019) Iron Electrocoagulation Process for Disinfecting Water: A Review. Applied Engineering, 3, 154-158.
[38]  Ghernaout, D. and Elboughdiri, N. (2019) Mechanistic Insight into Disinfection Using Ferrate(VI). Open Access Library Journal, 6, e5946.
https://doi.org/10.4236/oalib.1105946
[39]  Ghernaout, D. and Elboughdiri, N. (2019) Water Disinfection: Ferrate(VI) as the Greenest Chemical: A Review. Applied Engineering, 3, 171-180.
[40]  Ghernaout, D. and Ghernaout, B. (2010) From Chemical Disinfection to Electrodisinfection: The Obligatory Itinerary? Desalination and Water Treatment, 16, 156-175. https://doi.org/10.5004/dwt.2010.1085
[41]  Ghernaout, D. and Ghernaout, B. (2011) On the Controversial Effect of Sodium Sulphate as Supporting Electrolyte on Electrocoagulation Process: A Review. Desalination and Water Treatment, 27, 243-254.
https://doi.org/10.5004/dwt.2011.1983
[42]  Irki, S., Ghernaout, D., Naceur, M.W., Alghamdi, A. and Aichouni, M. (2018) Decolorizing Methyl Orange by Fe-Electrocoagulation Process: A Mechanistic Insight. International Journal of Environmental Chemistry, 2, 18-28.
https://doi.org/10.11648/j.ijec.20180201.14
[43]  Ghernaout, D., Naceur, M.W. and Aouabed, A. (2011) On the Dependence of Chlorine by-Products Generated Species Formation of the Electrode Material and Applied Charge during Electrochemical Water Treatment. Desalination, 270, 9-22.
https://doi.org/10.1016/j.desal.2011.01.010
[44]  Ghernaout, D., Touahmia, M. and Aichouni, M. (2019) Disinfecting Water: Electrocoagulation as an Efficient Process. Applied Engineering, 3, 1-12.
[45]  Ghernaout, D., Alghamdi, A. and Ghernaout, B. (2019) Electrocoagulation Process: A Mechanistic Review at the Dawn of Its Modeling. Journal of Environmental Science and Allied Research, 2, 51-67.
https://doi.org/10.29199/2637-7063/ESAR-201019
[46]  Ghernaout, D. and Elboughdiri, N. (2019) Electrocoagulation Process Intensification for Disinfecting Water: A Review. Applied Engineering, 3, 140-147.
[47]  Ghernaout, D. (2019) Disinfection via Electrocoagulation Process: Implied Mechanisms and Future Tendencies. EC Microbiology, 15, 79-90.
[48]  Holt, P.K. (2002) Electrocoagulation: Unraveling and Synthesizing the Mechanisms behind a Water Treatment Process. The University of Sydney, Sydney.
[49]  Hakizimana, J.N., Gourich, B., Chafi, M., Stiriba, Y., Vial, C., Drogui, P. and Naja, J. (2017) Electrocoagulation Process in Water Treatment: A Review of Electrocoagulation Modeling Approaches. Desalination, 404, 1-21.
https://doi.org/10.1016/j.desal.2016.10.011
[50]  Kim, T.H., Park, C., Shin, E.B. and Kim, S. (2002) Decolorization of Disperse and Reactive Dyes by Continuous Electrocoagulation Process. Desalination, 150, 165-175. https://doi.org/10.1016/S0011-9164(02)00941-4
[51]  Papadopoulos, K.P., Argyriou, R., Economou, C.N., Charalampous, N., Dailianis, S., Tatoulis, T.I., Tekerlekopoulou, A.G. and Vayenas, D.V. (2019) Treatment of Printing Ink Wastewater Using Electrocoagulation. Journal of Environmental Management, 237, 442-448. https://doi.org/10.1016/j.jenvman.2019.02.080
[52]  Ben Hariz, I., Halleb, A., Adhoum, N. and Monser, L. (2013) Treatment of Petroleum Refinery Sulfidic Spent Caustic Wastes by Electrocoagulation. Separation and Purification Technology, 107, 150-157.
https://doi.org/10.1016/j.seppur.2013.01.051
[53]  Mameri, N., Lounici, H., Belhocine, D., Grib, H., Piron, D.L. and Yahiat, Y. (2001) Defluoridation of Sahara Water by Small Plant Electrocoagulation Using Bipolar Aluminium Electrodes. Separation and Purification Technology, 24, 113-119.
https://doi.org/10.1016/S1383-5866(00)00218-5
[54]  Mameri, N., Yeddou, A.R., Lounici, H., Belhocine, D., Grib, H. and Bariou, B. (1998) Defluoridation of Septentrional Sahara Water of North Africa by Electrocoagulation Process Using Bipolar Aluminium Electrodes. Water Research, 32, 1604-1612. https://doi.org/10.1016/S0043-1354(97)00357-6
[55]  Zhu, J., Zhao, H. and Ni, J. (2007) Fluoride Distribution in Electrocoagulation Defluoridation Process. Separation and Purification Technology, 56, 184-191.
https://doi.org/10.1016/j.seppur.2007.01.030
[56]  Kobya, M., Demirbas, E. and Ulu, F. (2016) Evaluation of Operating Parameters with Respect to Charge Loading on the Removal Efficiency of Arsenic from Potable Water by Electrocoagulation. Journal of Environmental Chemical Engineering, 4, 1484-1494. https://doi.org/10.1016/j.jece.2016.02.016
[57]  Dubrawski, K.L., Fauvel, M. and Mohseni, M. (2013) Metal Type and Natural Organic Matter Source for Direct Filtration Electrocoagulation of Drinking Water. Journal of Hazardous Materials, 244-245, 135-141.
https://doi.org/10.1016/j.jhazmat.2012.11.027
[58]  Dubrawski, K.L. and Mohseni, M. (2013) In-Situ Identification of Iron Electrocoagulation Speciation and Application for Natural Organic Matter (NOM) Removal. Water Research, 47, 5371-5380. https://doi.org/10.1016/j.watres.2013.06.021
[59]  Vázquez, A., Nava, J.L., Cruz, R., Lázaro, I. and Rodríguez, I. (2014) The Importance of Current Distribution and Cell Hydrodynamic Analysis for the Design of Electrocoagulation Reactors. Journal of Chemical Technology & Biotechnology, 89, 220-229. https://doi.org/10.1002/jctb.4105
[60]  Vázquez, A., Rodríguez, I. and Lázaro, I. (2012) Primary Potential and Current Density Distribution Analysis: A First Approach for Designing Electrocoagulation Reactors. Chemical Engineering Journal, 179, 253-261.
https://doi.org/10.1016/j.cej.2011.10.078
[61]  Martinez-Delgadillo, S., Mollinedo-Ponce, H., Mendoza-Escamilla, V., Gutiérrez-Torres, C., Jiménez-Bernal, J. and Barrera-Diaz, C. (2012) Performance Evaluation of an Electrochemical Reactor Used to Reduce Cr(VI) from Aqueous Media Applying CFD Simulations. Journal of Cleaner Production, 34, 120-124.
https://doi.org/10.1016/j.jclepro.2011.10.036
[62]  Choudhary, A. and Mathur, S. (2017) Performance Evaluation of 3D Rotating Anode in Electro Coagulation Reactor: Part I: Effect of Impeller. The Journal of Water Process Engineering, 19, 322-330. https://doi.org/10.1016/j.jwpe.2017.08.020
[63]  Gilhotra, V., Das, L., Sharma, A., Kang, T.S., Singh, P., Dhuria, R.S. and Bhatti, M.S. (2018) Electrocoagulation Technology for High Strength Arsenic Wastewater: Process Optimization and Mechanistic Study. Journal of Cleaner Production, 198, 693-703. https://doi.org/10.1016/j.jclepro.2018.07.023
[64]  Song, P., Song, Q., Yang, Z., Zeng, G., Xu, X., Li, X. and Xiong, W. (2018) Numerical Simulation and Exploration of Electrocoagulation Process for Arsenic and Antimony Removal: Electric Field, Flow Field, and Mass Transfer Studies. Journal of Environmental Management, 228, 336-345.
https://doi.org/10.1016/j.jenvman.2018.09.001
[65]  Song, P., Yang, Z., Zeng, G., Yang, X., Xu, H., Wang, L., Xu, R., Xiong, W. and Ahmad, K. (2017) Electrocoagulation Treatment of Arsenic in Wastewaters: A Comprehensive Review. Chemical Engineering Journal, 317, 707-725.
https://doi.org/10.1016/j.cej.2017.02.086
[66]  Villalobos-Lara, A.D., Pérez, T., Uribe, A.R., Alfaro-Ayala, J.A., de Jesús Ramírez-Minguela, J. and Minchaca-Mojica, J.I. (2020) CFD Simulation of Biphasic Flow, Mass Transport and Current Distribution in a Continuous Rotating Cylinder Electrode Reactor for Electrocoagulation Process. Journal of Electroanalytical Chemistry, 858, Article ID: 113807.
https://doi.org/10.1016/j.jelechem.2019.113807
[67]  Casta?eda, L.F., Core?o, O., Nava, J.L. and Carre?o, G. (2020) Removal of Fluoride and Hydrated Silica from Underground Water by Electrocoagulation in a Flow Channel Reactor. Chemosphere, 244, Article ID: 125417.
https://doi.org/10.1016/j.chemosphere.2019.125417

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