|
|
微塑料老化特征及吸附特性研究进展
|
Abstract:
微塑料作为环境污染物的重要载体，对于重金属的迁移、转化和毒理的影响是不可忽视的，微塑料在环境中会受到老化作用，导致其物理结构或化学特性进一步改变，既而影响其在环境中的吸附行为，本文系统地介绍了微塑料在自然环境中的老化行为，并在此基础上总结了老化后微塑料对各类污染物的吸附特性变化，进一步探究微塑料老化后的研究方向，以便后期能更为全面地评估微塑料在环境中的风险，为学者们提供科学指导。
As important carriers of environmental pollutants, microplastics play a significant role in the migration, transformation, and toxicological effects of heavy metals. Microplastics undergo aging processes in the environment, leading to changes in their physical structures and chemical properties, which in turn affect their adsorption behavior. This paper systematically reviews the aging behavior of microplastics in natural environments, summarizes the changes in the adsorption characteristics of various pollutants by aged microplastics, and further explores future research directions. The aim is to provide a more comprehensive assessment of the environmental risks posed by microplastics and to offer scientific guidance for researchers.
| [1] | Rochman, C.M., Hoh, E., Kurobe, T. and Teh, S.J. (2013) Ingested Plastic Transfers Hazardous Chemicals to Fish and Induces Hepatic Stress. Scientific Reports, 3, Article No. 3263. https://doi.org/10.1038/srep03263 |
| [2] | Andrady, A.L. (2017) The Plastic in Microplastics: A Review. Marine Pollution Bulletin, 119, 12-22. https://doi.org/10.1016/j.marpolbul.2017.01.082 |
| [3] | Zhao, L., Rong, L., Xu, J., Lian, J., Wang, L. and Sun, H. (2020) Sorption of Five Organic Compounds by Polar and Nonpolar Microplastics. Chemosphere, 257, Article 127206. https://doi.org/10.1016/j.chemosphere.2020.127206 |
| [4] | Mao, R., Lang, M., Yu, X., Wu, R., Yang, X. and Guo, X. (2020) Aging Mechanism of Microplastics with UV Irradiation and Its Effects on the Adsorption of Heavy Metals. Journal of Hazardous Materials, 393, Article 122515. https://doi.org/10.1016/j.jhazmat.2020.122515 |
| [5] | Guo, C., Wang, L., Lang, D., Qian, Q., Wang, W., Wu, R., et al. (2023) UV and Chemical Aging Alter the Adsorption Behavior of Microplastics for Tetracycline. Environmental Pollution, 318, Article 120859. https://doi.org/10.1016/j.envpol.2022.120859 |
| [6] | Yang, J., Cang, L., Sun, Q., Dong, G., Ataul-Karim, S.T. and Zhou, D. (2019) Effects of Soil Environmental Factors and UV Aging on Cu2+ Adsorption on Microplastics. Environmental Science and Pollution Research, 26, 23027-23036. https://doi.org/10.1007/s11356-019-05643-8 |
| [7] | Yang, Z., Li, Y. and Zhang, G. (2024) Degradation of Microplastic in Water by Advanced Oxidation Processes. Chemosphere, 357, Article 141939. https://doi.org/10.1016/j.chemosphere.2024.141939 |
| [8] | Thakur, B., Singh, J., Singh, J., Angmo, D. and Vig, A.P. (2023) Biodegradation of Different Types of Microplastics: Molecular Mechanism and Degradation Efficiency. Science of the Total Environment, 877, Article 162912. https://doi.org/10.1016/j.scitotenv.2023.162912 |
| [9] | 杜钰赞, 孙姣霞, 付江, 等. 聚酰胺微塑料对磺酸类全氟烷基化合物在水-土界面吸附的影响研究[J]. 中国环境科学: 1-13. https://doi.org/10.19674/j.cnki.issn1000-6923.20241104.001, 2025-01-08. |
| [10] | Liu, G., Zhu, Z., Yang, Y., Sun, Y., Yu, F. and Ma, J. (2019) Sorption Behavior and Mechanism of Hydrophilic Organic Chemicals to Virgin and Aged Microplastics in Freshwater and Seawater. Environmental Pollution, 246, 26-33. https://doi.org/10.1016/j.envpol.2018.11.100 |
| [11] | 陈浩然, 李昊, 林雨男, 等. 生物老化微塑料对重金属铜的吸附特性研究[J]. 海洋环境科学, 2024, 43(6): 963-972. |
| [12] | 李凯贺, 门聪, 程世昆, 等. 土壤中微塑料与抗生素吸附、迁移及复合毒性研究进展[J]. 环境科学: 1-19. https://doi.org/10.13227/j.hjkx.202405030, 2025-01-08. |
| [13] | 曹艳晓, 陈诺, 徐鑫宇, 等. 生物炭修复塑料-镉复合污染土壤潜力与机制研究[J]. 中国环境科学: 1-15. https://doi.org/10.19674/j.cnki.issn1000-6923.20241122.001, 2025-01-08. |
| [14] | Guo, M., Noori, R. and Abolfathi, S. (2024) Microplastics in Freshwater Systems: Dynamic Behaviour and Transport Processes. Resources, Conservation and Recycling, 205, Article 107578. https://doi.org/10.1016/j.resconrec.2024.107578 |
| [15] | Liu, L., Xu, M., Ye, Y. and Zhang, B. (2022) On the Degradation of (Micro) Plastics: Degradation Methods, Influencing Factors, Environmental Impacts. Science of the Total Environment, 806, Article 151312. https://doi.org/10.1016/j.scitotenv.2021.151312 |
| [16] | 寇诗棋, 关卓, 鲁旭阳, 等. 土壤中微塑料迁移及其对有机污染物的影响研究进展[J]. 土壤, 2024, 56(3): 457-470. |
| [17] | Zhang, K., Hamidian, A.H., Tubić, A., Zhang, Y., Fang, J.K.H., Wu, C., et al. (2021) Understanding Plastic Degradation and Microplastic Formation in the Environment: A Review. Environmental Pollution, 274, Article 116554. https://doi.org/10.1016/j.envpol.2021.116554 |
| [18] | 王娜, 张士璀. 水产动物中的微塑料及其对人健康的潜在危险性[J]. 海洋科学, 2023, 47(6): 124-129. |
| [19] | 张哿, 邹亚丹, 徐擎擎, 等. 微塑料与水中污染物的联合作用研究进展[J]. 海洋湖沼通报, 2019(2): 59-69. |
| [20] | 胡洪营, 夏军, 陈卓, 等. 新污染物的水环境伦理问题及对策[J/OL]. 环境工程: 1-12. https://link.cnki.net/urlid/11.2097.X.20241206.1348.002, 2025-01-08. |
