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含铝催化剂对丙酮的催化氧化研究进展
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Abstract:
丙酮等含氧挥发性有机污染物越来越受到人们的重视，不同类型的催化剂通过催化氧化过程可以有效去除丙酮。其中，含铝催化剂对丙酮具有优异的催化氧化活性。综述了共沉淀法、盐模板法、凝胶–水热反应法等合成方法在含铝催化剂制备中的应用。总结了金属负载比例和类型、煅烧温度、载体类型等对催化活性的影响，并简要说明了含铝催化剂去除丙酮的催化活性和机理。从制备方法改进、催化氧化机理深入研究、Al的作用等方面对含铝催化剂的研究进行了展望。
The oxygenated volatile organic pollutants (e.g. acetone) have been paid more attention. Different types of catalysts can effectively remove acetone through catalytic oxidation process. Among them, the aluminum-containing catalysts exhibited excellent catalytic activity in acetone oxidation. The preparation methods of aluminum-containing catalysts, for example co-precipitation method, salt-template synthesis technique, gel-hydrothermal reaction method, were reviewed. The effects of metal loading ratio and type, calcination temperature and support type on catalytic activity were summarized, and the catalytic activity and mechanism of the aluminum-containing catalysts for acetone removal were briefly described. The promising research trends of the aluminum-containing catalysts have been prospected from three aspects: improvement of synthesis method, further study on catalytic oxidation mechanism and the role of Al.
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