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-  2018 

Self-Templating Synthesis of Cobalt Hexacyanoferrate Hollow Structures with Superior Performance for Na-Ion Hybrid Supercapacitors

DOI: https://doi.org/10.1021/acsami.8b08455

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Abstract:

Prussian blue (PB) and its analogues (PBA), especially with hollow structures, have attracted growing attention from the researchers of energy storage field. Herein, we have developed a facile self-templating method to synthesize hollow-structured cobalt hexacyanoferrate (CoHCF) with controllable morphologies by using water-soluble precursors as templates. The method is versatile and can be extended to synthesize various PB/PBA hollow structures with tunable composition and morphology. Profiting from the unique hollow structure, the CoHCF hollow prisms manifest exceptional electrochemical performance in the Na2SO4 aqueous electrolyte, including a high specific capacitance (284 F g–1 at 1 A g–1), a high rate capability, and an excellent cycling stability (92% retention after 5000 cycles). A hybrid supercapacitor device assembled with the CoHCF hollow prisms and activated carbon shows a high specific density of 47 W h kg–1 at a specific power of 1000 W kg–1 and stable cycling performance

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