全部 标题 作者
关键词 摘要

OALib Journal期刊
ISSN: 2333-9721
费用:99美元

查看量下载量

相关文章

更多...

南京市溧水区夏季大气细颗粒物来源解析
Source Analysis of Atmospheric Fine Particulate Matter in Lishui District, Nanjing in Summer

DOI: 10.12677/AEP.2020.105081, PP. 653-662

Keywords: 细颗粒物,在线监测,化学成分,源解析
Fine Particulate Matter
, Online Monitoring, Chemical Composition, Source Analysis

Full-Text   Cite this paper   Add to My Lib

Abstract:

利用在线气溶胶质谱仪(SPAMS)于2019年7月16日至2019年8月31日对南京市溧水区环境空气细颗粒物开展高时间分辨化学成分监测。结果显示,在监测时段内,监测点空气质量细颗粒物(PM2.5)污染较2018年同期变差,PM2.5均值浓度为21.0 μg?m?3。通过对细颗粒物成分分类,最终确定了八类颗粒物。根据对细颗粒物排放源分类分析,PM2.5主要来源于机动车尾气源(34.9%)、扬尘源(20.0%)、工业工艺源(10.1%)。此外,考虑到气象因素,在静稳天气条件下区域内更易发生细颗粒物浓度升高。结合不同风向判断,不同时段PM2.5数量浓度的升高会分别受到机动车尾气源、工业工艺源、扬尘源、燃煤源、生物质燃烧源等不同类型源的排放累积影响,说明溧水区颗粒物来源综合性较强。
Online aerosol mass spectrometer (SPAMS) was used to monitor the chemical composition of fine particles in ambient air in Lishui district in Nanjing with a high time resolution, from July 16th to August 31st, 2019. The results showed that during the monitoring period, fine particulate matter (PM2.5) pollution at the monitoring points became worse than the same period in 2018, with the mean concentration of PM2.5 being 21.0 μg?m?3. Through the classification of fine particulate com-position, eight kinds of particulate matter were finally determined. According to the classification analysis of fine particulate matter emission sources, PM2.5 mainly comes from automobile exhaust source (34.9%), dust source (20.0%) and industrial process source (10.1%). In addition, consid-ering the meteorological factors, higher concentration of fine particulate matter were more likely to happen in the static stable weather conditions. Combined with different wind direction, the increase of PM2.5 concentration in different time periods will be affected by the emission accumulation of different types of sources, such as automobile exhaust source, industrial process source, dust source, coal burning source and biomass combustion source, indicating that the sources of particulate matter in Lishhui district were relatively comprehensive.

References

[1]  穰敏. 我国大气污染防治工作的思考[J]. 应用能源技术, 2018(5): 5-7.
[2]  雷宇, 宁淼. 对“十三五”时期挥发性有机物污染防治路径的系统思考[J]. 环境保护, 2017, 45(13): 14-17.
[3]  黄子龙, 曾立民, 董华斌, 等. 利用SPAMS研究华北乡村站点(曲周) 夏季大气单颗粒物老化与混合状态[J]. 环境科学, 2016, 37(4): 1188-1198.
[4]  王苏蓉, 喻义勇, 王勤耕, 等. 基于PMF模式的南京市大气细颗粒物源解析[J]. 中国环境科学, 2015, 35(12): 3535-3542.
[5]  郑玫, 张延君, 闫才青, 等. 中国PM2.5来源解析方法综述[J]. 北京大学学报(自然科学版), 2014, 50(6): 1141-1154.
[6]  Zhang, G., Bi, X., Li, L., et al. (2013) Mixing State of Individual Submicron Carbon-Containing Particles during Spring and Fall Seasons in Urban Guangzhou, China: A Case Study. Atmospheric Chemistry and Physics, 13, 4723- 4735.
https://doi.org/10.5194/acp-13-4723-2013
[7]  赵辉, 郑有飞, 吴晓云, 等. 江苏省大气复合污染特征与相关气象驱动[J]. 中国环境科学, 2018, 38(8): 2830-2839.
[8]  贾梦唯, 赵天良, 张祥志, 等. 南京主要大气污染物季节变化及相关气象分析[J]. 中国环境科学, 2016, 36(9): 2567-2577.
[9]  沈毅, 王体健, 韩永, 等. 南京近郊主要大气污染物的观测分析研究[J]. 南京大学学报(自然科学), 2009, 45(6): 746-756.
[10]  吴万宁, 查勇, 王强, 等. 南京地区冬夏季大气重污染个例对比分析[J]. 中国环境科学, 2014, 34(3): 581-587.
[11]  龚宇麟, 银燕, 陈魁, 等. 南京北郊秋季气溶胶理化特征及潜在源区分布[J]. 中国环境科学, 2017, 37(11): 4032-4043.
[12]  秦鑫, 张泽锋, 李艳伟, 等. 南京北郊春季含Pb气溶胶粒子来源分析[J]. 环境科学学报, 2015, 35(3): 641-646.
[13]  张俊, 吉祝美, 咸月, 等. 大气细颗粒物实时在线源解析技术解析盐城市大气细颗粒物来源[J]. 污染防治技术, 2015, 28(2): 18-22.
[14]  李梅, 李磊, 黄正旭, 等. 运用单颗粒气溶胶质谱技术初步研究广州大气矿尘污染[J]. 环境科学研究, 2011, 24(6): 632-636.
[15]  Jia, M.W., Zhao, T.L., Cheng, X.H., et al. (2017) Inverse Relations of PM2.5 and O3 in Air Compound Pollution between Cold and Hot Seasons over an Urban Area of East China. Atmosphere, 8, 59.
https://doi.org/10.3390/atmos8030059
[16]  Wang, H.L., Zhu, B., Shen, L.J., Xu, H.H., An, J.L., Xue, G.Q. and Cao, J.F. (2015) Water-Soluble Ions in Atmospheric Aerosols Measured in Five Sites in the Yangtze River Delta, China: Size-Fractionated, Seasonal Variations And Sources. Atmospheric Environment, 123, 370-379.
https://doi.org/10.1016/j.atmosenv.2015.05.070
[17]  Ming, L., Jin, L., Li, J., Fu, P.Q., Yang, W.Y., Liu, D., Zhang, G., Wang, Z.F. and Li, X.D. (2017) PM2.5 in the Yangtze River Delta, China: Chemical Compositions, Seasonal Variations, and Regional Pollution Events. Environment Pollution, 223, 200-212.
https://doi.org/10.1016/j.envpol.2017.01.013
[18]  周静博, 任毅斌, 洪纲, 等. 利用SPAMS研究石家庄市冬季连续灰霾天气的污染特征及成因[J]. 环境科学, 2015, 36(11): 3972-3980.
[19]  蔡靖, 郑玫, 闫才青, 等. 单颗粒气溶胶飞行时间质谱仪在细颗粒物研究中的应用和进展[J]. 分析化学. 2015, 43(5): 765-774.
[20]  付怀于, 闰才青, 郑玫, 等. 在线单颗粒气溶胶质谱SPAMS对细颗粒物中主要组分提取方法的研究[J]. 环境科学, 2014, 36(11): 4070-4077.

Full-Text

Contact Us

service@oalib.com

QQ:3279437679

WhatsApp +8615387084133