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热力发电  2015 

生物质焦和煤焦等温co2气化动力学研究

, PP. 102-107

Keywords: 生物质焦,煤焦,气化,动力学,气固反应模型,活化能

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Abstract:

利用失重热天平研究生物质焦和煤焦在900~1050℃下的等温co2气化反应性,以体积模型及收缩核模型2种代表性的气固反应模型,分析了生物质焦和煤焦气化过程的动力学参数。结果表明:随着气化温度升高,生物质焦和煤焦的气化反应时间均缩短,且生物质焦的气化性能优于煤焦;生物质焦颗粒近似平板片状结构,采用收缩核模型(scm)形状因子m=0可以表征其气化过程,且其等温co2气化活化能为101.86kj/mol;煤焦颗粒结构收缩核模型m=1/2及m=2/3均能够表征煤焦气化过程,且其等温co2气化煤焦活化能分别为159.80、168.88kj/mol。

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