OALib Journal期刊
ISSN: 2333-9721
费用:99美元
|
|
|
studyoniron-manganesecatalystsforfischer-tropschsynthesis
, PP. 550-557
Keywords: iron-manganesecatalyst,catalyticperformance,operationalconditions,fischer-tropschsynthesis
Abstract:
?iron-manganesecatalystswerepreparedbyco-precipitationmethod.characterizationofcatalystswascarriedoutbyusingx-raydiffraction(xrd),scanningelectronmicroscopy(sem),temperatureprogramreduction(tpr),n2adsorption-desorptionmeasurements.theresultsfromcatalyticperformancetestsinfischer-tropschsynthesisshowedthattheiron-manganesecatalystsaresupersensitivetocatalystcompositionandmaterialssource.itwasfoundthatc2~4lightolefinsincreasedwhilech4andco2decreasedbyusingiron-manganesecatalystpreparedfromiron(ⅱ)sulfate(acatalyst).theactivityandselectivityofacatalystwasstudiedindifferentoperationalconditions.theresultsshowedthatthebestoperationalconditionsforc2~4lightolefinsproductionwereh2/co=1/1(ghsv=2400h-1)at260℃under0.3mpatotalpressure.
References
[1] | madonrj,taylorwf.effectofsulfuronthefischer-tropschsynthesisalkali-promotedprecipitatedcobalt-basedcatalyst[m].advchemser,1979,178:93-111.
|
[2] | griboval-constanta,khodakovay,becharar,zholobenkovl.supportmesoporosity:atoolforbettercontrolofcatalyticbehaviorofcobaltsupportedfischer-tropschcatalysts[m].studsurfscicatal,2002,144:609-616.
|
[3] | claeysm,vansteene.fischer-tropschtechnology[m].studsurfscicatal,2004,152:601-680.
|
[4] | sarkara,sethd,dozierak,neatheryjk,hamdehhh,davisbh.fischer-tropschsynthesis:morphology,phasetransformationandparticlesizegrowthofnano-scaleparticles[j].catallett,2007,117(1/2):1-17.
|
[5] | pouran,taghipoors,shekarrizm,shahrismk,zamaniy.fischer-tropschsynthesiswithfe/cu/la/sio2catalyst[j].jnanoscinanotechnol,2009,9(7):4425-4429.
|
[6] | herranzt,rojass,perez-alonsofj,ojedam,terrerosp,fierrojlg.hydrogenationofcarbonoxidesoverpromotedfe-mncatalystspreparedbythemicroemulsionmethodology[j].applcatala,2006,311:66-75.
|
[7] | pouran,housaindokhtmr,tayyarist,zarkeshj.effectofnano-particlesizeonproductdistributionandkineticparametersoffe/cu/lacatalystinfischer-tropschsynthesis[j].jnatgaschem,2010,19(2):107-116.
|
[8] | erikssons,nylenu,rojass,boutonnetm.preparationofcatalystsfrommicroemulsionsandtheirapplicationsinheterogeneouscatalysis[j].applcatala,2004,265(2):207-219.
|
[9] | schwugerm-j,stickdornk,schomaeckerr.microemulsionsintechnicalprocesse[j].chemrev,1995,95(4):849-864.
|
[10] | liuc,zoub,rondinoneaj,zhangzj.reversemicellesynthesisandcharacterizationofsuperparamagneticmnfe2o4spinelferritenanocrystallites[j].jphyschemb,2000,104(6):1141-1145.
|
[11] | feyzim,mirzaeiaa.performanceandcharacterizationofiron-nickelcatalystsforlightolefinproduction[j].jnatgaschem,2010,19(4):422-430.
|
[12] | feyzim,mirzaeiaa,bozorgzadehhr.effectsofpreparationandoperationconditionsonprecipitatedironnickelcatalystsforfischer-tropschsynthesis[j].jnatgaschem,2010,19(3):341-353.
|
[13] | vandenbergfr,crajemwj,vanderkraanam,geusjw.reductionbehaviouroffe/zro2andfe/k/zro2fischer-tropschcatalysts[j].applcatala,2003,242(2):403-416.
|
[14] | andersonjr.catalysisscienceandtechnology.vol.1[m].springer,newyork:springer-verlagpress,1981.
|
[15] | kingdl,cusumanoja,gartenrl.atechnologicalperspectiveforcatalyticprocessesbasedonsynthesisgas[j].catalrev,1981,23(1/2):233-263.
|
[16] | maitigc,malessar,baernsm.iron/manganeseoxidecatalystsforfischer-tropschsynthesis:partistructuralandtexturalchangesbycalcination,reductionandsynthesis[j].applcatal,1983,5(2):151-170.
|
[17] | malessar,baernsm.iron/manganeseoxidecatalystsforfischer-tropschsynthesis:4activityandselectivity[j].indengchemres,1988,27(2):279-283.
|
[18] | kolbelh,tillmetzkd.processfortheproductionofhydrocarbonsandoxygen-containingcompoundsandcatalyststherefore:us,4177203[p].1979-12-04.
|
[19] | dasck,dasns,choudhurydp,ravichandrang,chakrabartydk.hydrogenationofcarbonmonoxideonunsupportedfe-mn-kcatalystsforthesynthesisofloweralkenes:promotereffectofmanganese[j].applcatala,1994,111(2):119–132.
|
[20] | vanderlaangp,beenackersaacm.kineticsandselectivityofthefischer-tropschsynthesis:aliteraturereview[j].catalrev,1999,41(3/4):255-318.
|
[21] | gonzalez-cortessl,arodulfo-baechlersm,oliverosa,orozcoj,fontalb,moraaj,delgadog.synthesisoflightalkenesonmanganesepromotedironandiron-cobaltfischer-tropschcatalysts[j].reactkinetcatallett,2002,75(1):3-12.
|
[22] | lij,covillenj.effectofborononthesulfurpoisoningofco/tio2fischer-tropschcatalysts[j].applcatala,2001,208(1/2):177-184.
|
[23] | yamadam,koizumin,miyazawaa,furukawat.novelcatalyticpropertiesofrhsulfideforthesynthesisofmethanolfromco+h2inthepresenceofh2s[j].catallett,2002,78(1/4):195-199.
|
[24] | beckj,hilberttt.einaltes'rhodiumsulfidmitüberraschenderstruktur:synthese,kristallstrukturundelektronischeeigenschaftenvonrh3s4[j].chemie,2000,626:72-79.
|
[25] | lit,yangy,zhangc,anx,wanh,taoz,xiangh,liy,yif,xub.effectofmanganeseonaniron-basedfischer-tropschsynthesiscatalystpreparedfromferroussulfate[j].fuel,2007,86(7/8):921-928.
|
[26] | stengerhg,satterfieldcn.effectofliquidcompositionontheslurryfischer-tropschsynthesis:2productselectivity[j].indengchemprocessdesdev,1985,24(2):411-415.
|
[27] | vanderkraanam,ramselaarwltm,debeervhj.mossbauerspectroscopyappliedtoinorganicchemistry,vol.3[m]//longgj,grandjeanf.newyork:plenumpress,1989:376.
|
[28] | feyzim,irandoustm,mirzaeiaa.effectsofpromotersandcalcinationconditionsonthecatalyticperformanceofiron–manganesecatalystsforfischer–tropschsynthesis[j].fuelprocesstechnol,2011,92(5):1136-1143.
|
[29] | barraultj,forquyc,perrichonv.effectsofmanganeseoxideandsulphateonolefinselectivityofironsupportedcatalystsinthefischer-tropschreaction[j].applcatal,1983,5(1):119-125.
|
[30] | kitzelmannd,vielstichw.in-situstudyoftheprimaryreactionsinthehydrogenationofcoonfe-catalystsfischer-tropschsynthesis[j].zphyschem,1978,112(2):215-233.
|
[31] | mirzaeiaa,habibpourr,kashie.preparationandoptimizationofmixedironcobaltoxidecatalystsforconversionofsynthesisgastolightolefins[j].applcatala,2005,296(2):222-231.
|
[32] | hutchingsgj,mirzaeiaa,joynerrw,siddiquimrh,taylorsh.effectofpreparationconditionsonthecatalyticperformanceofcoppermanganeseoxidecatalystsforcooxidation[j].applcatala,1998,166(1):143-152.
|
[33] | whittledm,mirzaeiaa,hargreavesjsj,joynerrw,kielycj,taylorsh,hutchingsgj.co-precipitatedcopperzincoxidecatalystsforambienttemperaturecarbonmonoxideoxidation:effectofprecipitateageingoncatalystactivity[j].physchemchemphys,2002,4(23):5915-5920.
|
[34] | gonzales-cortessl,rodulfo-baechlerma,orozcoj.characterizationoffe-co-mncatalystsaftercarbonmonoxidehydrogenation[j].revmexfis,2003,49s3:204-206.
|
Full-Text
|
|
Contact Us
service@oalib.com QQ:3279437679 
WhatsApp +8615387084133
|
|