OALib Journal期刊
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cs2对完全液相法制备的cu-zn-al催化剂上合成气制dme反应性能的影响
, PP. 447-451
Keywords: 铜锌铝催化剂,完全液相制备法,二甲醚,cs2,硫中毒
Abstract:
?实验以cs2为硫源,考察硫对完全液相法制备cu-zn-al催化剂活性的影响,并用x射线粉末衍射(xrd)、氢气程序升温吸附(h2-tpr)、氨气程序升温脱附(nh3-tpd)等方法对催化剂性能进行了表征。结果表明,对完全液相法制备的cu-zn-al催化剂而言,加入小于4mg/l的cs2对催化剂的活性影响不大;催化剂的活性随着加入硫含量的增加,下降程度增大。
References
[1] | 李德宝,马玉刚,齐会杰,李文怀,孙予罕,钟柄.co加氢合成低碳混合醇催化体系研究新进展[j].化学进展,2004,16(4):584-592.(lide-bao,mayu-gang,qihui-jie,liwen-huai,sunyu-han,zhongbing.progressinsynthesisofmixedalcoholsfromcohydrogenation[j].processinchemistry,2004,16(4):584-592.)
|
[2] | 张建国,宋昭峥,史德文,蒋庆哲,孙贵利.合成气合成低碳混合醇技术的研究[j].现代化工,2007,增刊(2):494-496.(zhangjian-guo,songzhao-zheng,shide-wen,jiangqing-zhe,sungui-li.studyonmixedalcoholsynthesisfromsyngas[j].modernchemicalindustry,2007,suppl(2):s494-s496.)
|
[3] | strohmjj,zhengj,songc.low-temperaturesteamreformingofjetfuelintheabsenceandpresenceofsulfuroverrhandrh-nicatalystsforfuelcells[j].jcatal,2006,238(2):309-320.
|
[4] | lij,covillenj.effectofborononthesulfurpoisoningofco/tio2fischer-tropschcatalysts[j].applcatala,2001,208(1/2):177-184.
|
[5] | liuz-t,zhouj-l,zhangb-j.poisoningofironcatalystbycosinsyngasforfischer-tropschsynthesis[j].jmolcatal,1994,94(2):255-261.
|
[6] | 黄伟,高志华,郝利峰.浆态床用催化剂及制备方法:中国,1613560a.2004-09-18.(huangwei,gaozhi-hua,haoli-feng.slurryphaseforthecatalystpreparationethod:cn,1613560a.2004-09-18.)
|
[7] | zhangl,milletj-mm,ozkanus.deactiuationcharacteristicsoffe-al-cuwater-gasshiftcatalystsinthepresenceofh2s[j].jmolcatala,2009,309(1/2):63-70.
|
[8] | forzattip,liettil.catalystdeactivation[j].cataltoday,1999,52(2/3):165-181.
|
[9] | kimms,rodrigueznm,bakerrtk.theinterplaybetweensulfuradsorptionandcarbondepositiononcobaltcatalysts[j].jcatal,1993,143(2):449-463.
|
[10] | 樊金串,吴慧,黄伟,谢克昌.表面活性剂对完全液相法制cu-zn-al浆状催化剂结构和性能的影响[j].高等学校化学学报,2008,29(5):993-999.(fanjin-chuan,wuhui,huangwei,xieke-chang.effectofsurfactantsonstructureandperformanceofcu-zn-alcatalystpreparedbycompleteliquid-phasetechnology[j].chemicalresearchinchineseuniversities,2008,29(5):993-999.)
|
[11] | 王立楠,储伟,张雄伟.低温液相合成甲醇用新型铜基催化剂研究[j].天然气化工,2005,30(1):27-30.(wangli-nan,chuwei,zhangxiong-wei.investigationonnovelcopper-basedcatalystsforlowtemperaturemethanolsynthesis(ltms)inliquidphase[j].naturalgaschemicalindustry,2005,30(1):27-30.
|
[12] | 化明利,郭宪吉,鲍改玲,谭羚艳.二步共沉淀法制备的铜基甲醇合成催化剂的研究[j].天然气化工,2003,28(6):1-4.(huaming-li,guoxiang-ji,baogai-ling,tanling-yan.studyoncopper-basedcatalystformethanolsynthesispreparedbytwo-stepcoprecipitation[j].naturalgaschemicalindustry,2003,28(6):1-4.)
|
[13] | kimc,somorjaiga.theeffectofrheniumandsulfuronthereactivityandselectivityofptsingle-crystal[j].jcatal,1992,134(1):179-185.
|
[14] | 谭猗生,解红娟,崔海涛,韩怡卓,钟柄.脱水催化剂的改性对浆态床一步法合成二甲醚的影响[j].催化学报,2005,26(3):229-232.(tanyi-sheng,xiehong-juan,cuihai-tao,hanyi-zhuo,zhongbing.effectofmodificationofdehydrationcatalystondimethylethersynthesisfromsyngasinslurryphase[j].chinesejournalofcatalysis,2005,26(3):229-232.)
|
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