OALib Journal期刊
ISSN: 2333-9721
费用:99美元
|
|
|
300mw燃煤电站砷、汞排放特征研究
, PP. 839-844
Keywords: 砷,汞,排放,烟气,飞灰
Abstract:
?对某300mw燃煤电站煤、底灰和静电除尘器(esp)飞灰进行采样并测定了其中的砷、汞含量,同时应用ontariohydromethod(ohm)标准方法和设备对esp前后烟气中的砷、汞分布进行了直接采样和测试.对砷的检测结果表明,esp飞灰中砷含量约6.68×10-6,是原煤中砷含量的2.5倍左右,而底灰中砷含量仅为1.70×10-6,esp前烟气中砷含量约153.27μg/m3,esp后砷含量急剧降低为41.13μg/m3;对汞的检测结果表明,原煤中汞含量约2.5×10-7,飞灰、底灰中的汞含量分别约1.9×10-7、1.5×10-7;esp前后烟气中总汞含量分别为5.49、5.21μg/m3.砷在飞灰中明显富集,而汞在飞灰和底渣中均不具有富集效果.esp单元具有明显的协同脱砷效果,平均脱除率约在71%左右,而对汞的协同脱除效果不明显.
References
[1] | 张军营,任德贻,许德伟,赵峰华.煤中汞及其对环境的影响[j].环境科学进展,1999,7(3):100-104.(zhangjun-ying,rende-yi,xude-wei,zhaofeng-hua.mercuryincoalanditseffectonenvironment[j].advancesinenvironmentalscience,1999,7(3):100-104.)
|
[2] | ngjc,wangjp,shraima.aglobalhealthproblemcausedbyarsenicfromnaturalsources[j].chemosphere,2003,52(9):1353-1359.
|
[3] | 蒋靖坤,郝吉明,吴烨,streetsdg,段雷,田贺忠.中国燃煤汞排放清单的初步建立[j].环境科学,2005,26(2):34-39.(jiangjing-kun,haoji-ming,wuye,streetsdg,duanlei,tianhe-zhong.developmentofmercuryemissioninventoryfromcoalcombustioninchina[j].environmentalscience,2005,26(2):34-39.)
|
[4] | 郭欣,郑楚光,陈丹.300mw煤粉锅炉砷排放特征的实验研究[j].环境科学,2006,27(4):631-634.(guoxin,zhengchu-guang,chendan.characterizationofarsenicemissionsfromacoal-firedpowerplant[j].environmentalscience,2006,27(4):631-634.)
|
[5] | 胡长兴,周劲松,何胜,骆仲泱,岑可法.我国典型电站燃煤锅炉汞排放量估算[j].热力发电,2010,39(3):1-4.(huchang-xing,zhoujin-song,hesheng,luozhong-yang,cenke-fa.estimationofmercuryemissionfromcoal-firedboilersintypicalpowerplantsofchina[j].thermalpowergeneration,2010,39(3):1-4.)
|
[6] | 陈萍,旷红伟,唐修义.煤中砷的分布和赋存规律研究[j].煤炭学报,2002,27(3):259-263.(chenping,kuanghong-wei,tangxiu-yi.researchonthedistributionandoccurrenceofarsenicincoal[j].journalofchinacoalsociety,2002,27(3):259-263.)
|
[7] | 郑刘根,刘桂建,chouchen-lin,高连芬,彭子成.中国煤中砷的含量分布、赋存状态、富集及环境意义[j],地球学报,2006,27(4):355-366.(zhengliu-gen,liugui-jian,chouchen-lin,gaolian-fen,pengzi-cheng.arsenicinchinesecoals:itsabundance,distribution,modesofoccurrence,enrichmentprocesses,andenvironmentalsignificance[j].actageoscienticasinica,2006,27(4):355-366.)
|
[8] | zielinskira,fosteral,meekergp.modeofoccurrenceofarsenicinfeedcoalanditsderivativeflyash,blackwarriorbasin,alabama[j].fuel,2007,86:560-572.
|
[9] | hugginsfe,seniorcl,chup.seleniumandarsenicspeciationinflyashfromfull-scalecoal-burningutilityplants[j].environscitechnol,2007,41(9):3284-3289.
|
[10] | 郭瑞霞,杨建丽,刘东艳,刘振宇.热处理条件对大同煤中微量有害元素变迁规律的影响[j].化工学报,2003,54(11):1603-1607.(guorui-xia,yangjian-li,liudong-yan,liuzhen-yu.influenceofthermaltreatmentconditionsontransformationoftraceelementsindatongcoal[j].journalofchemicalindustryandengineering(china),2003,54(11):1603-1607.)
|
[11] | 张凯华,孙喆,曹晏,潘伟平,张锴.能源高效清洁利用及新能源技术,2012动力工程青年学术论坛论文集.杭州:浙江大学出版社,2012:77-82.(zhangkai-hua,sunzhe,caoyan,panwei-ping,zhangkai.cleanandefficientutilizationofenergyandnewenergytechnology,2012youthacademicforumforpowerengineering.hangzhou:zhejianguniversitypress,2012:77-82.)
|
[12] | astmd6784-02,standardtestmethodforelemental,oxidized,particle-boundandtotalmercuryinfluegasgeneratedfromcoal-firedstationarysources(ontariohydromethod)[s].2008.
|
[13] | tanapoms,jamesch.arsenicandmercurypartitioninginflyashatakentuckypowerplant[j].energyfuels,2003,17:1028-1033.
|
[14] | 王起超,沈文国,麻壮伟.中国燃煤汞排放量估算[j].中国环境科学,1999,19(4):318-321.(wangqi-chao,shenwen-guo,mazhuang-wei.theestimationofmercuryemissionfromcoalcombustioninchina[j].chinaenvironmentalscience,1999,19(4):318-321.)
|
[15] | tianhz,wangy,xuezg,quyp,chaifh,haojm.atmosphericemissionsestimationofhg,as,andsefromcoal-firedpowerplantsinchina,2007[j].scitotalenviron,2011,409:3078-3081.
|
[16] | 田贺忠,曲益萍.2005年中国燃煤大气砷排放清单[j].环境科学,2009,30(4):956-962.(tianhe-zhong,quyi-ping.inventoriesofatmosphericarsenicemissionsfromcoalcombustioninchina,2005[j].environmentalscience,2009,30(4):956-962.)
|
[17] | 王明仕,郑宝山,finkelmanrb,胡军,吴代赦,李社红.煤中砷赋存状态与其脱洗率的关系[j].燃料化学学报,2005,33(2):253-256.(wangming-shi,zhengbao-shan,finkelmanrb,hujun,wudai-she,lishe-hong.relationshipbetweenoccurrencemodeofarsenicincoalanditswashingrate[j].journaloffuelchemistryandtechnology,2005,33(2):253-256.)
|
[18] | 李扬,张军营,赵永椿,吴幼青,高晋生,郑楚光.热解条件对煤中微量元素挥发性影响的实验研究[j].工程热物理学报,2007,28(2):189-192.(liyang,zhangjun-ying,zhaoyong-chun,wuyou-qing,gaojin-sheng,zhengchu-guang.influenceofpyrolysisconditionsonvolatilityoftraceelementsincoals[j].journalofeengineeringthermophysics,2007,28(2):189-192.)
|
[19] | 王运军,段钰峰,杨立国,孟素丽,黄治军,吴成军,王乾.湿法烟气脱硫装置和静电除尘器联合脱除烟气中汞的试验研究[j].中国电机工程学报,2008,28(29):64-69.(wangyun-jun,duanyu-feng,yangli-guo,mengsu-li,huangzhi-jun,wucheng-jun,wangqian.experimentalstudyonmercuryremovalbycombinedwetfluegasdesulphurizationwithelectrostaticprecipitator[j].proceedingsofthecsee,2008,28(29):64-69.)
|
[20] | thompsond,argentbb.predictionofthedistributionoftraceelementsbetweentheproductstreamsoftheprenflogasifierandcomparisonwithreporteddata[j].fuel,2002,81(5):555-570.
|
[21] | argentbb.thermodynamicequilibriumstudyoftraceelementmobilizationunderairblowngasificationconditions[j].fuel,2002,81(1):75-89.
|
[22] | clarkel,slossl.traceelements-emissionsfromcoalcombustionandgasification[m].london:ieacoalresearch,1992.
|
[23] | lopez-antonma,diaz-somoanom,spearsda.arsenicandseleniumcapturebyflyashesatlowtemperature[j].environscitechnol,2006,40(12):3947-3951.
|
[24] | constancels,helblejj.emissionsofmercury,traceelements,andfineparticlesfromstationarycombustionsource[j].fuelprocesstechnol,2000,65-66:263-288.
|
[25] | zollerwh,gladneyes,ducera.atmosphericconcentrationsandsourcesoftracemetalsatthesouthpole[j].science,1974,183(4121):198-200.
|
[26] | 雒昆利,张新民,陈昌和,陆毅伦.我国燃煤电厂砷的大气排放量初步估算[j].科学通报,2004,49(19):2014-2019.(luokun-li,zhangxin-min,chenchang-he,luyi-lun.estimationofarsenicemissionfromcoal-firedpowerplantsofchina[j].chinesesciencebulletin,2004,49(19):2014-2019.)
|
[27] | tangq,liugj,yanzc,sunry.distributionandfateofenvironmentallysensitiveelements(arsenic,mercury,stibiumandselenium)incoal-firedpowerplantsathuainan,anhui,china[j].fuel,2012,95:334-339.
|
[28] | 王运军,段钰锋,杨立国,江贻满,吴成军,王乾,杨详花.燃煤电站布袋除尘器和静电除尘器脱汞性能比较[j].燃料化学学报,2008,36(1):23-29.(wangyun-jun,duanyu-feng,yangli-guo,jiangyi-man,wucheng-jun,wangqian,yangxiang-hua.comparisonofmercuryremovalcharacteristicbetweenfabricfilterandelectrostaticprecipitatorsofcoal-firedpowerplants[j].journaloffuelchemistryandtechnology,2008,36(1):23-29.)
|
[29] | 钟丽萍,曹晏,李文英,潘伟平,谢克昌.燃煤电厂污染控制单元对汞释放的控制作用[j].燃料化学学报,2010,38(6):641-646.(zhongli-ping,caoyan,liwen-ying,panwei-ping,xieke-chang.effectoftheexistingairpollutantcontroldevicesonmercuryemissionincoal-firedpowerplants[j].journaloffuelchemistryandtechnology,2010,38(6):641-646.)
|
Full-Text
|
|
Contact Us
service@oalib.com QQ:3279437679 
WhatsApp +8615387084133
|
|