全部 标题 作者
关键词 摘要

OALib Journal期刊
ISSN: 2333-9721
费用:99美元

查看量下载量

相关文章

更多...
地球学报  2010 

柴达木盆地察尔汗湖区古湖相沉积物中含氮类分子化石的检出

DOI: 10.3975/cagsb.2010.02.04

Keywords: 含氮类分子化石,古湖相沉积物,脂肪酸酰胺,脂肪腈,青藏高原

Full-Text   Cite this paper   Add to My Lib

Abstract:

利用气相色谱质谱联用仪(GC-MS)对青藏高原柴达木盆地察尔汗湖区贝壳堤剖面古湖相沉积物样品进行了系统地分析,检测出系列脂肪酸酰胺与脂肪腈类含氮类脂物分子化石。并对其在古湖相沉积物中的分布特征作了详细描述。对它们综合研究认为,早期成岩作用使来源于各种生物体的脂肪酸酰胺类分子化石部分地转化为脂肪腈类化合物。此外,不饱和脂肪酸酰胺与饱和脂肪酸酰胺的含量比值在剖面上并没有呈现明显下降的趋势,说明在降解过程中各种生物、物理及化学作用对它们不存在明显的选择性,指示有机质在沉积过程中可能处于一个偏氧化的环境。本文首次报道这两类物质,为更好地理解含氮类脂物分子化石在湖泊沉积物中的转化过程提供了一定的理论依据。

References

[1]  谢树成;梁斌;顾延生;杨欢.脂肪酮分子在第四纪古土壤中的分布及其古气候意义[J].古生物学报,2008(03)
[2]  张成君;陈发虎;尚华明;曹洁.中国西北干旱区湖泊沉积物中有机质碳同位索组成的环境意义-以民勤盆地三角城古湖泊为例[J].第四纪研究,2004(01)
[3]  谢树成;梁斌;郭建秋;易轶 EVERSHED R P MADDY D CHAMBERS F M.生物标志化合物与相关的全球变化[J].第四纪研究,2003(05)
[4]  ZHANG Hong-liang;LI Shi-jie;FENG Qing-lai;ZHANG Shi-tao,Quaternary International.Environmental change and human activities during the 20th century reconstructed from the sediment of Xingyun Lake,Yunnan Province,China,2010(01).
[5]  ZHANG Cheng-jun;CHEN Fa-hu;SHANG Hua-ming;CAO Jie.The palenenvironmentai significance of organic carbon isotope in lacustrine sediments in the arid China:an experimental from Sanjiaocheng palaeolake in Minqin[J].Quaternary Sciences,2004(01)
[6]  XIE Shu-cheng;LIANG Bing;GUO Jian-qiu;YI Yi EVERSHED R P MADDY D CHAMBERS F M.Biomarkers and the related global change[J].Quaternary Sciences,2003(05)
[7]  REGTOP R A;CRISP P T;ELLIS J,Chemical characterization of shale oil from Rundle,Queensland,Fuel,1982(02).
[8]  B.S.Radovic ;M.Careri ;A.Mangia ;M.Musci ;M.Gerboles ;E.Anklam,Contribution of dynamic headspace GC-MS analysis of aroma compounds to authenticity testing of honey,Food Chemistry?,2001, 72(4).
[9]  吴艳宏;L(U)CKE A;W(U)NNEMANN B 李世杰 王苏民.青藏高原中部全新世气候变化的湖泊沉积地球化学记录[J].中国科学D辑,2007(09)
[10]  DUAN Yi.Pentaeyclic triterpenoid ketones in peat from Gannan Marsh[J].Chinese Science Bulletin,2001(17)
[11]  DEMBITSKY V M;SHKROB I;ROZENTSVET O A Fatty acid amides from freshwater green alga Rhizoclonium hieroglyphicum [J] 2000(08) doi:10.1016/S0031-9422(00)00183-7
[12]  FUENTE D L;SANZ M L;MARTiEZ-CASTRO I;SANZ J RUIZ-MATUTE A I Volatile and carbohydrate composition of rare unifloral honeys from Spain [J] 2007(01) doi:10.1016/j.foodchem.2007.03.039
[13]  ZHU Da-gang;ZHAO Xi-tuo,Nam Tso lacustrine sediments and the ancient big lake in northern Tibet Plateau,Acta Geoscientica Sinica,2001(02).
[14]  ZHENG Mien-ping;LIU Xi-fang;YUAN He-ran;ZHANG Cheng-jun WANG Hai-lei.Some Characteristics of stratigraphic sequences and lacustrine sediments of main quaternary lakes on the Qinghai-Tibet Plateau[J].Acta Geoscientica Sinica,2008(03)
[15]  ZHAO Xi-tao;WU Zhong-hai;HU Dao-gong;YAN Fu-hua MA Zhi-bang MAI Xue-shnn YAN Xi-Li.The discovery of late Pleistocene highstand lacustrine sediments of the Co Ngoin Lake and adjacent areas,Tibet[J].Acta Geoscientica Sinica,2005(04)
[16]  张虎才;常凤琴;李斌;雷国良 陈玥 张文翔 牛洁 樊红芳 杨明生.柴达木察尔汗湖贝壳堤剖面长链支链烷烃及其古环境意义[J].科学通报,2007(06)
[17]  陈江;万力;梁四海;金晓媚 陈立.青藏高原生态环境变化趋势的初步探索[J].地球学报,2007(06)
[18]  常凤琴;张虎才;陈玥;杨明生 牛洁 樊红芳 雷国良 张文翔 类延斌 杨伦庆.柴达木盆地察尔汗古湖贝壳堤剖面沉积地球化学与环境变化[J].地球科学-中国地质大学学报,2008(02)
[19]  谢树成;赖旭龙;黄咸雨;马相如 杨淑娟.分子地层学的原理、方法及应用实例[J].地层学杂志,2007(03)
[20]  ZHANG Z H;ZHAO M X;YANG X D;WANG S M JIANG X Z FRANK O GEOFFREY E A hydrocarbon biomarker record for the last 40 kyr of plant input to Lake Heqing,southwestern China [J] 2004(05)
[21]  ZHANG Hu-cai;WANG Qiang;PENG Jin-lan;CHEN Guang-jie.Ostracod assemblages and their paleoenvironmental significance from shell bar section of paleolake Qarhan,Qaidam basin[J].Quaternary Sciences,2008(01)
[22]  ZHANG Hu-cai;LEI Guo-liang;CHANG Feng-qin;FAN Hong-fang,YANG Ming-sheng.ZHANG Wen-xiang.Age Determination of shell bar section in salt lake Qarhan,Qaidam Basin[J].Quaternary Sciences,2007(04)
[23]  ZHANG Hu-cai;CHANG Feng-qin;LI Bing;LEI Guo-liang CHEN Yue ZHANG Wen-xiang NIU Jie FAN Hong-fang YANG Ming-sheng.Branched aliphatic alkanes of the Late Pleistocene paleolake deposits from the Qaidam Basin,NE Tibetan Plateau[J].Chinese Science Bulletin,2007(09)doi:10.1007/s11434-007-0167-3
[24]  ZHANG Hu-Cai;LEI Guo-Lieng;CHANG Feng-Qin;PU Yang FAN Hong-Fang LEI Yan-Bin YANG Ming-Sheng ZHANG Wen-Xiang YANG Lun-Qing,Chronology of the shell bar section and a discussion on the ages of the Late Pleistocene lacustrine deposits in the paleolake Qarhan,Qaidam basin,Frontiers of Earth Science in China,2008(02).
[25]  ZHANG Hu-Cai;FAN Hong-Fang;CHANG Feng-Qin;ZHANG Wen-Xieng LEI Guo-Linag YANG Ming-Sheng LEI Yan-Bin YANG Lun-Qing,AMS dating on the Shell Bar section from Qaidam Basin,NE Tibetan Plateau,China,Radiocarbon,2008(02).
[26]  XIE Shn-cheng;LIANG Bing;GU Yan-sheng;YANG Huan.Distributions of n-alkan-2-ones in quaternary palensols indicative of paleoclimate changes[J].Acta Palaeontologica Sinica,2008(03)
[27]  XIE Shu-cheng;LAI Xu-long;HUANG Xian-yu;MA Xiang-ru YANG Shu-juan.Principles,methodology and application of molecular stratigraph[J].Journal of Stratigraphy,2007(03)
[28]  XIE S C;PANCOST R D;YIN H F;WANG H M EVERSHED R P Two episodes of microbial change coupled with Permo/Triassic faunal mass extinction [J] 2005(24)
[29]  WU Yan-hong;LOCKE ANDREAS;W(U)NNEMANN BERND;LI Shi-Jie WANG Su-min.Holocene climate change in the Central Tibetan Plateau inferred by lacustrine sediment geochemical records[J].Science in China(Earth Sciences),2007(10)
[30]  Wu M. ;Gerwick WH. ;Milligan KE.,THREE NEW MALYNGAMIDES FROM THE MARINE CYANOBACTERIUM LYNGBYA MAJUSCULA,Tetrahedron?,1997, 53(47).
[31]  UCAR S;OZKAN A R,Characterization of products from the pyrolysis of rapeseed oil cake,Bioresource Technology,2008(18).
[32]  TANAKA I;MATSUOKA S;MURATA M;TACHIBANA K,Absolute configuration of a ceramide with a novel branched-chain fatty acid isolated from the epiphytic dinoflagellate,Coolia monotis,Bioscience,Biotechnology,and Biochemistry,2000(09).
[33]  Bernd R. T. Simoneit ;A. I. Rushdi ;M. R. Bin Abas ;B.M. Didyk,Alkyl amides and nitriles as novel tracers for biomass burning,Environmental Science & Technology?,2003, 37(1).
[34]  ROGGE W F;HILDEMANN L M;MARUREK,M A;CASS,G R,Sources of fine organic aerosol.1.Charbroilers and meat cooking operations,Environmental Science and Technology,1991(06).
[35]  段毅.甘南沼泽泥炭中五环三萜酮系列化合物的检出[J].科学通报,2001(11)
[36]  MORRIS R J,The occurrence of wax esters in crustaceans from the North-east Atlantic Ocean,Marine Biology,1972(02).
[37]  MARKETON M;GRONQUIST M;EBERHARD A;GONZALEZ J Characterization of the Sinorhizobium meliloti sinR/sinI locus and the production of novel N-acyl homoserine lactones [J] 2002(20)
[38]  LIU X Q;DONG H L;YANG X D;HERZSCHUH U ZHANG E L STUUT J-B W WANG Y B,Late Holocene forcing of the Asian winter and summer monsoon as evidenced by proxy records from the northern Qinghai-Tibetan Plateau,Earth and Planetary Science Letters,2009(1-4).
[39]  KAWASAKI W;MATSUI K;AKAKABE Y;ITAI N KAJIWARA T Volatiles from Zostera marina [J] 1998(01) doi:10.1016/S0031-9422(97)88555-X
[40]  KAWAMURA K;ISHIWATARI R,Polyunsaturated fatry acids in a lacustrine sediment as a possible indicator of paleoclimate,Geochiimca et Cosmochimica Acta,1981(02).
[41]  KAWAMURA K;ISHIWATARI R;YAMAZAKI M,Identification of polyunsaturated fatty acids in surface lacustrine sediments,Chemical Geology,1980.
[42]  ISHIWATARI R;YAMAMOTO S;SHINOYAMA S Lignin and fatty acid records in Lake Baikal sodiments over the last 130Kyr:A comparison with pollen records [J] 2006(12) doi:10.1016/j.orggeochem.2006.10.005
[43]  EVANS E J;BATTS B D;CANTN W;SMITH J W,The origin of nitriles in shale oil,Organic Geochemistry,1985(05).
[44]  Eglinton, TI ;Eglinton, G,Molecular proxies for paleoclimatology,Earth and Planetary Science Letters?,2008, 275(1/2).
[45]  DUNN R J K;WELSH D T;TEASDALE P R;LEE S Y LEMCKERT C J MEZIANE T,Investigating the distribution and sources of organic matter in surface sediment of Coombabah Lake(Australia)using elemental,isotopic and fatty acid biomarkers,Continental Shelf Research,2008(18).
[46]  Chu, GQ ;Sun, Q ;Li, SQ ;Zheng, MP ;Jia, XX ;Lu, CF ;Liu, JQ ;Liu, TS,Long-chain alkenone distributions and temperature dependence in lacustrine surface sediments from China,Geochimica et Cosmochimica Acta?,2005, 69(21).
[47]  Chen Kezao;Bowler J M,Late Pleistocene evolution of salt lakes in the Qaidam Basin,Qinghai Province,China,Palaeogeography,Palaeoclimatology,Palaeoecology? ,1986, 54.
[48]  CHEN Jiang;WAN Li;LIANG Si-hai;JIN Xiao-mei CHEN Li.A tentative discussion on the trend of ecological environment change in Qinghai-Tibet Plateau[J].Acta Geoscientica Sinica,2007(06)
[49]  CHANG Feng-qin;ZHANG Hu-cai;CHEN Yue;YANG Ming-sheng NIU Jie FAN Hong-fang LEI Guo-liang ZHANG Wen-xiang LEI Yan-bing YANG Lun-qing,Sedimentation Geochemistry and Environmental Changes during the Late Pleistocene of Paleolake Qarhan in the Qaidam Basin,Journal of China University of Geosciences,2008(02).
[50]  BEZUGLOV V;BOBROV M;ARCHAKOV A,Bioactive amides of fatty acids,Biochemistry(Moscow),1998(01).
[51]  朱大岗;赵希涛.纳木错湖相沉积与藏北高原古大湖[J].地球学报,2001(02)
[52]  郑绵平;刘喜方;袁鹤然;张成君 王海雷.青藏高原第四纪重点湖泊地层序列和湖相沉积若干特点[J].地球学报,2008(03)
[53]  赵希涛;吴中海;胡道功;严富华 马志邦 麦学舜 鄢犀利.西藏错鄂及邻区晚更新世高位湖相沉积的发现及其意义[J].地球学报,2005(04)
[54]  张虎才;王强;彭金兰;陈光杰.柴达木察尔汗盐湖贝壳堤剖面介形类组合及其环境意义[J].第四纪研究,2008(01)
[55]  张虎才;雷国良;常凤琴;樊红芳 杨明生 张文翔.柴达木盆地察尔汗贝壳堤剖面年代学研究[J].第四纪研究,2007(04)

Full-Text

Contact Us

service@oalib.com

QQ:3279437679

WhatsApp +8615387084133