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珠江三角洲对流层气溶胶时空变化特征分析

DOI: 10.6038/cjg20130605, PP. 1835-1842

Keywords: 对流层气溶胶,时空变化,气溶胶模型,珠三角地区

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Abstract:

利用AERONET资料对珠三角地区气溶胶物理性质特征进行分析,建立珠三角地区的气溶胶模型,在此基础上,根据RT3辐射传输模型构建矢量查找表,采用多角度偏振方法从PARASOLL1B数据反演得到细模态气溶胶光学厚度(AOD),最后采用2007—2009年MODIS总的AOD产品和本文的细模态AOD三年的反演结果分析了珠三角地区气溶胶的时间变化和空间分布特征,为深入研究珠三角地区污染物的局地排放和输送提供了条件.结果表明:(1)珠三角地区对流层气溶胶呈双峰型对数正态分布,其中细粒子平均半径主要集中在0.05~0.1,标准方差以0.5、0.6为主,粗粒子平均半径以0.9、1.0为主,标准方差为0.6、0.7,复折射指数实部以1.4、1.5居多,虚部以0、0.01为主,细粒子所占比例大于70%,珠三角气溶胶呈现出粗颗粒物和细颗粒物并存的特征;(2)PARASOL业务算法中的气溶胶模型在珠三角地区有较大的局限性,引入当地气溶胶模型使细模态AOD的反演精度较卫星产品有了很大提高,细模态AOD主要反映了珠三角地区二次污染的强度;(3)珠三角地区总AOD值春季较大,秋夏季次之,冬季较小,并呈现逐年较小的趋势;(4)珠三角地区细模态AOD也在逐年降低,2009年细模态AOD年均值比2007年低了0.02,在空间分布上,高值地区主要集中在广州、佛山、中山等城市.

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