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环境化学  2015 

大气中全氟与多氟有机化合物研究进展

Keywords: 全氟与多氟有机化合物,大气,采样技术,分析方法,气-颗粒两相分配

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Abstract:

全氟与多氟有机化合物(PFCs)作为表面活性剂被广泛应用于工业生产及生活家居领域,部分PFCs已被列为斯德哥尔摩公约受控持久性有机污染物(POPs).PFCs具有一些特殊的理化性质(如高表面活性、憎水憎油性等),使其采样、分析、环境迁移转化过程等都不同于"传统"POPs(如PCBs、PAHs等).相对于其它环境介质(水、沉积物和生物等)研究,大气中PFCs的研究相对较少.本文针对大气中PFCs的研究现状进行综述,内容涵盖了大气PFCs的样品采集、前处理、仪器分析、含量水平和迁移转化过程,其中重点概述了大气中PFCs的气-颗粒两相分配、长距离迁移、干湿沉降和大气降解,并提出了今后的重点研究方向建议.

References

[1]  Conder J M, Hoke R A, Wolf W D, et al. Are PFCAs bioaccumulative? A critical review and comparison with regulatory criteria and persistent lipophilic compounds[J].Environmental Science & Technology, 2008, 42(4):995-1003
[2]  Lau C, Anitole K, Hodes C, et al. Perfluoroalkyl acids: A review of monitoring and toxicological findings[J].Toxicological Sciences, 2007, 99(2):366-394
[3]  Martin J W, Muir D C G, Moody C A, et al. Collection of airborne fluorinated organics and analysis by gas chromatography/chemical ionization mass spectrometry[J]. Analytical Chemistry, 2002, 74(3):584-590
[4]  Stock N L, Ellis D A, Deleebeeck L, et al. Vapor pressures of the fluorinated telomer alcohols limitations of estimation methods[J].Environmental Science & Technology, 2004, 38(6):1693-1699
[5]  Kaiser M A, Larsen B S, Kao C P C, et al. Vapor pressures of perfluorooctanoic, -nonanoic, -decanoic,-undecanoic, and -dodecanoic acids[J].Journal of Chemical and Engineering Data, 2005, 50(6):1841-1843
[6]  胡灿, 王珍珍, 徐文斌, 等. 一些全氟(及多氟)有机化合物蒸汽压的QSPR研究[J].化学研究与应用, 2013, 25(1):43-46
[7]  Arp H P H, Goss K U. Irreversible sorption of trace concentrations of perfluorocarboxylic acids to fiber filters used for air sampling[J].Atmospheric Environment, 2008, 42(28):6869-6872
[8]  Arp H P H, Goss K U. Gas/particle partitioning behavior of perfluorocarboxylic acids with terrestrial aerosols[J].Environmental Science & Technology, 2009, 43(22):8542-8547
[9]  Ahrens L, Shoeib M, Harner T, et al. Comparison of annular diffusion denuder and high volume air samplers for measuring per-and polyfluoroalkyl substances in the atmosphere[J].Analytical Chemistry, 2011, 83(24):9622-9628
[10]  刘向, 张干, 李军, 等. 利用PUF大气被动采样技术监测中国城市大气中的多环芳烃[J].环境科学, 2007, 28(1):26-31
[11]  王俊, 张干, 李向东, 等. 珠江三角洲地区大气中有机氯农药的被动采样观测[J].环境化学, 2007, 26 (3):395-398
[12]  Li X, Li Y, Zhang Q, et al. Evaluation of atmospheric sources of PCDD/Fs, PCBs and PBDEs around a steel industrial complex in northeast China using passive air samplers[J].Chemosphere, 2011, 84(7):957-963
[13]  Gao L, Zhang Q, Liu L, et al. Spatial and seasonal distributions of polychlorinated dibenzo-p-dioxins and dibenzofurans and polychlorinated biphenyls around a municipal solid waste incinerator, determined using polyurethane foam passive air samplers[J].Chemosphere, 2014, 114:317-326
[14]  Li J, Del Vento S, Schuster J, et al. Perfluorinated compounds in the Asian atmosphere[J]. Environmental Science & Technology, 2011, 45(17):7241-7248
[15]  Ahrens L, Harner T, Shoeib M, et al. Characterization of two passive air samplers for per-and polyfluoroalkyl substances[J].Environmental Science & Technology, 2013, 47(24):14024-14033
[16]  Ahrens L, Shoeib M, Del Vento S, et al. Polyfluoroalkyl compounds in the Canadian Arctic atmosphere[J].Environmental Chemistry, 2011, 8(4):399-406
[17]  Cai M, Xie Z, Moller A, et al. Polyfluorinated compounds in the atmosphere along a cruise pathway from the Japan Sea to the Arctic Ocean[J].Chemosphere, 2012, 87(9):989-997
[18]  Shoeib M, Harner T, Vlahos P. Perfluorinated chemicals in the Arctic atmosphere[J]. Environmental Science & Technology, 2006, 40(20):7577-7583
[19]  Barber J L, Berger U, Chaemfa C, et al. Analysis of per-and polyfluorinated alkyl substances in air samples from Northwest Europe[J].Journal of Environmental Monitoring, 2007, 9(6):530-541
[20]  Dreyer A, Temme C, Sturm R, et al. Optimized method avoiding solvent-induced response enhancement in the analysis of volatile and semi-volatile polyfluorinated alkylated compounds using gas chromatography-mass spectrometry[J].Journal of Chromatography A, 2008, 1178(1-2):199-205
[21]  Jahnke A, Ahrens L, Ebinghaus R, et al. An improved method for the analysis of volatile polyfluorinated alkyl substances in environmental air samples[J].Analytical and Bioanalytical Chemistry, 2007, 387(3):965-975
[22]  Jahnke A, Berger U, Ebinghaus R, et al. Latitudinal gradient of airborne polyfluorinated alkyl substances in the marine atmosphere between Germany and South Africa (53° N—33° S)[J].Environmental Science & Technology, 2007, 41(9):3055-3061
[23]  Jahnke A, Huber S, Temme C, et al. Development and application of a simplified sampling method for volatile polyfluorinated alkyl substances in indoor and environmental air[J]. Journal of Chromatography A, 2007, 1164(1-2):1-9
[24]  Shoeib M, Vlahos P, Harner T, et al. Survey of polyfluorinated chemicals (PFCs) in the atmosphere over the northeast Atlantic Ocean[J].Atmospheric Environment, 2010, 44(24):2887-2893
[25]  Dreyer A, Ebinghaus R. Polyfluorinated compounds in ambient air from ship-and land-based measurements in northern Germany[J].Atmospheric Environment, 2009, 43(8):1527-1535
[26]  杨运云, 邓洁薇, 罗辉泰, 等. 加速溶剂萃取-高效液相色谱-串联质谱法测定空气中的全氟化合物[J].分析化学, 2010, 38(11):1583-1587
[27]  Boulanger B, Peck A M, Schnoor J L, et al. Mass budget of perfluorooctane surfactants in Lake Ontario[J].Environmental Science & Technology, 2005, 39(1):74-79
[28]  Piekarz A M, Primbs T, Field J A, et al. Semivolatile fluorinated organic compounds in Asian and western U.S. air masses[J]. Environmental Science & Technology, 2007, 41(24):8248-8255
[29]  Beser M I, Pardo O, Beltran J, et al. Determination of per-and polyfluorinated substances in airborne particulate matter by microwave-assisted extraction and liquid chromatography-tandem mass spectrometry[J]. Journal of Chromatography A, 2011, 1218(30):4847-4855
[30]  Shoeib M, Harner T, Ikonomou M, et al. Indoor and outdoor air concentrations and phase partitioning of perfluoroalkyl sulfonamides and polybrominated diphenyl ethers[J].Environmental Science & Technology, 2004, 38(5):1313-1320
[31]  吕刚. 药品包装材料中全氟辛烷磺酸类物质检测与安全评价技术[D].天津: 天津大学博士学位论文,2009
[32]  王利兵, 吕刚, 刘绍, 等. 气相色谱-质谱法测定包装材料中全氟辛酸及其盐类[J].分析试验室, 2007, 26(2):94-96
[33]  郝双利. 全氟羧酸的富集,衍生化及GC-MS分析[D].西安:陕西师范大学硕士学位论文,2013
[34]  Berger U, Langlois I, Oehme M, et al. Comparison of three types of mass spectrometers for HPLC/MS analysis of perfluoroalkylated substances and fluorotelomer alcohols[J].European Journal of Mass Spectrometry, 2004, 10(5):579-588
[35]  Taniyasu S, Kannan K, So M K, et al. Analysis of fluorotelomer alcohols, fluorotelomer acids, and short-and long-chain perfluorinated acids in water and biota[J].Journal of Chromatography A, 2005, 1093(1):89-97
[36]  Sun C, Sun H, Lai Y, et al. Liquid Chromatography/mass spectrometry method for determination of perfluorooctane sulfonyl fluoride upon derivatization with benzylamine[J].Analytical Chemistry, 2011, 83(15):5822-5826
[37]  Stock N L, Lau F K, Ellis D A, et al. Polyfluorinated telomer alcohols and sulfonamides in the North American troposphere[J].Environmental Science & Technology, 2004, 38(4):991-996
[38]  Dreyer A, Weinberg I, Temme C, et al. Polyfluorinated compounds in the atmosphere of the Atlantic and Southern Oceans: Evidence for a global distribution[J].Environmental Science & Technology, 2009, 43(17):6507-6514
[39]  Dreyer A, Matthias V, Temme C, et al. Annual time series of air concentrations of polyfluorinated compounds[J].Environmental Science & Technology, 2009, 43(11):4029-4036
[40]  Jahnke A, Ahrens L, Ebinghaus R, et al. Urban versus remote air concentrations of fluorotelomer alcohols and other polyfluorinated alkyl substances in Germany[J]. Environmental Science & Technology, 2007, 41(3):745-752
[41]  Jang M, Kamens R M. A Thermodynamic approach for modeling partitioning of semivolatile organic compounds on atmospheric particulate matter: Humidity effects[J].Environmental Science & Technology, 1998, 32(9):1237-1243
[42]  Chandramouli B, Jang M, Kamens R M. Gas-particle partitioning of semivolatile organic compounds (SOCs) on mixtures of aerosols in a smog chamber[J].Environmental Science & Technology, 2003, 37(18):4113-4121
[43]  Hung H, Thomas G O, Jones K C, et al. Grass-air exchange of polychlorinated biphenyls[J].Environmental Science & Technology, 2001, 35(20):4066-4073
[44]  Yang R, Zhang S, Li A, et al. Altitudinal and spatial signature of persistent organic pollutants in soil, lichen, conifer needles, and bark of the Southeast Tibetan Plateau: Implications for sources and environmental cycling[J].Environmental Science & Technology, 2013, 47(22):12736-12743
[45]  Brown T N, Wania F. Screening chemicals for the potential to be persistent organic pollutants: A case study of Arctic contaminants[J].Environmental Science & Technology, 2008, 42(14):5202-5209
[46]  Li Y F, Jia H L. Prediction of gas/particle partition quotients of polybrominated diphenyl ethers (PBDEs) in north temperate zone air: An empirical approach[J].Ecotoxicology and Environmental Safety, 2014, 108:65-71
[47]  Goss K-U, Bronner G, Harner T, et al. The partition behavior of fluorotelomer alcohols and olefins[J].Environmental Science & Technology, 2006, 40(11):3572-3577
[48]  Arp H P H, Goss K U. Response to commenton "Irreversible sorption of trace concentrations of perfluorocarboxylic acids to fiber filters used for air sampling" by Arp and Goss (Atmospheric Environment,42,6869-6872,2008)[J]. Atmospheric Environment, 2009, 43(22-23):3654-3655
[49]  Stock N L, Furdui V I, Muir D C G, et al. Perfluoroalkyl contaminants in the Canadian Arctic: Evidence of atmospheric transport and local contamination[J]. Environmental Science & Technology, 2007, 41(10):3529-3536
[50]  Armitage J M, MacLeod M, Cousins I T. Comparative assessment of the global fate and transport pathways of long-chain perfluorocarboxylic acids (PFCAs) and perfluorocarboxylates (PFCs) emitted from direct sources[J].Environmental Science & Technology, 2009, 43(15):5830-5836
[51]  Wallington T, Hurley M, Xia J, et al. Formation of C7F15COOH (PFOA) and other perfluorocarboxylic acids during the atmospheric oxidation of 8∶2 fluorotelomer alcohol[J].Environmental Science & Technology, 2006, 40(3):924-930
[52]  王杰明, 潘媛媛, 史亚利, 等. 北京城区降雪中全氟化合物的污染水平[J].中国科学:化学, 2011, 41(5):900-906
[53]  Liu W, Jin Y, Quan X, et al. Perfluorosulfonates and perfluorocarboxylates in snow and rain in Dalian, China[J].Environment International, 2009, 35(4):737-742
[54]  Loewen M, Halldorson T, Wang F, et al. Fluorotelomer carboxylic acids and PFOS in rainwater from an urban center in Canada[J].Environmental Science & Technology, 2005, 39(9):2944-2951
[55]  Dreyer A, Matthias V, Weinberg I, et al. Wet deposition of poly-and perfluorinated compounds in Northern Germany[J].Environmental Pollution, 2010, 158(5):1221-1227
[56]  Reth M, Berger U, Broman D, et al. Water-to-air transfer of perfluorinated carboxylates and sulfonates in a sea spray simulator[J].Environmental Chemistry, 2011, 8(4):381-388
[57]  Vierke L, Ahrens L, Shoeib M, et al. Air concentrations and particle-gas partitioning of polyfluoroalkyl compounds at a wastewater treatment plant[J].Environmental Chemistry, 2011, 8(4):363-371
[58]  Ellis D A, Martin J W, De Silva A O, et al. Degradation of fluorotelomer alcohols: A likely atmospheric source of perfluorinated carboxylic acids[J].Environmental Science & Technology, 2004, 38(12):3316-3321
[59]  Martin J W, Ellis D A, Mabury S A, et al. Atmospheric chemistry of perfluoroalkanesulfonamides: Kinetic and product studies of the OH radical and Cl atom initiated oxidation of N-ethyl perfluorobutanesulfonamide[J].Environmental Science & Technology, 2006, 40(3):864-872
[60]  Ellis D A, Martin J W, Mabury S A, et al. Atmospheric lifetime of fluorotelomer alcohols[J].Environmental Science & Technology, 2003, 37(17):3816-3820
[61]  D'eon J C, Hurley M D, Wallington T J, et al. Atmospheric chemistry of N-methyl perfluorobutane sulfonamidoethanol, C4F9SO2N (CH3) CH2CH2OH: Kinetics and mechanism of reaction with OH[J].Environmental Science & Technology, 2006, 40(6):1862-1868
[62]  Prevedouros K, Cousins I T, Buck R C, et al. Sources, fate and transport of perfluorocarboxylates[J]. Environmental Science & Technology, 2006, 40(1):32-44
[63]  Bhhatarai B, Gramatica P. Prediction of aqueous solubility, vapor pressure and critical micelle concentration for aquatic partitioning of perfluorinated chemicals[J]. Environmental Science & Technology, 2011, 45(19):8120-8128
[64]  Arp H P H, Niederer C, Goss K-U. Predicting the partitioning behavior of various highly fluorinated compounds[J].Environmental Science & Technology, 2006, 40(23):7298-7304

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