全部 标题 作者
关键词 摘要

OALib Journal期刊
ISSN: 2333-9721
费用:99美元

查看量下载量

相关文章

更多...
环境化学  2015 

雨水作用下典型土壤中Cd的释放及其赋存的形态变化

Keywords: Cd解吸,形态转化,pH,有机质含量

Full-Text   Cite this paper   Add to My Lib

Abstract:

本文模拟研究了土壤中Cd在雨水作用下的释放过程中,土壤中总Cd的释放动力学及释放过程中赋存形态的转化.结果表明,土壤中总Cd的解吸有快反应和慢反应两个过程,可用多项式、Frendlich及Elovich方程描述,且Elovich方程描述效果最优;土壤中总Cd解吸强度随土壤pH值、有机质含量的下降而增大,其中土壤pH值是主要影响因素;在低有机质、低pH值土壤中,Cd主要以可交换态存在;高有机质、高pH值土壤更有利于碳酸盐结合态、铁锰氧化态、有机结合态存在;可交换态Cd在不同pH土壤中均为最易解吸形态,土壤pH值越高,可交换态越容易向铁锰氧化态、有机结合态转化;土壤有机质越高越不利于可交换态的解吸,但有利于可交换态向其他形态转化.

References

[1]  陈明,冯流,J Yvon.缓变型地球化学灾害:概念、模型及案例研究[J].地球科学,2005,35(Ⅰ):261-266
[2]  王莹,陈玉成,李章平.我国城市土壤重金属的污染格局分析[J]. 环境化学,2012,31(6): 763-770
[3]  Scheidegger A M, Sparks D L. A critical assessment of sorption desortion mechanisms at the soil mineral/water interface [J]. Soil Science,1996,161(12):813-821
[4]  Yu S, He Z L, Huang C Y, et al. Adsorption-desorption behavior of copper at contaminated levels in red soils from China[J]. Journal of Environmental Quality, 2002,31:1130-1134
[5]  Abollino O, Aceto M, Malandrino M, et al. Adsorption of heavy metals on Na-montmorillonite. Effect of pH and organic substances[J]. Water research, 2003, 37(7): 1619-1627
[6]  焦文涛,蒋新,余贵芬,等.土壤有机质对镉在土壤中吸附-解吸行为的影响[J].环境化学,2005,24(5):345-549
[7]  Usero J, Gamerom, Morillo J. Comparative study of three sequential extraction procedures for metals in marine sediments [J]. Environ Int, 1998, 24(4): 487-496
[8]  Margu E, Salvadó V, Queralt I, et al. Comparison of three-stage sequential extraction and toxicity characteristic leaching tests to evaluate metal mobility in mining wastes[J]. Analytica Chimica Acta, 2004, 524(1): 151-159
[9]  Poulton S W, Canfield D E. Development of a sequential extraction procedure for iron: implications for iron partitioning in continentally derived particulates[J]. Chemical Geology, 2005, 214(3): 209-221
[10]  邱敏娴, 胡恭任, 于瑞莲,等.泉州湾洛阳江河口潮滩表层沉积物中重金属赋存形态分析[J]. 环境化学, 2013,32(2): 212-218
[11]  段小艳,赖细巧. 增施鸡粪对水稻产量与土壤肥力的影响[J].北京农业,2011,24:36-37
[12]  史贵涛,陈振楼,李海雯,等.城市土壤重金属污染研究现状与趋势[J]. 环境监测管理与技术,2006,18(6):9-12
[13]  Mireles A, Solis C, Andrade E, et al. Heavy metal accumulation in plants and soil irrigated with waste water from mexico city[J].Nuclear Instruments and Methods in Physics Research B:Beam Interactions with Materials and Atoms,2004, 219-220(6): 187-190
[14]  刘春阳,张宇峰,腾洁.土壤中重金属污染的研究进展[J].污染防治技术,2006,19(4): 42-46
[15]  余贵芬,蒋新,吴泓涛,等.镉铅在粘土上的吸附及受腐植酸的影响[J].环境科学,2002,23(5):109-112
[16]  徐龙君,袁智.外源镉污染及水溶性有机质对土壤中Cd形态的影响研究[J].土壤通报,2009,4(6):1442-1445
[17]  Tessier A, Campbell P G C, Bisson M. Sequential extraction procedure for the specification of particulate trace metals [J]. Anal Chem, 1979, (51): 844-850
[18]  冯素萍,刘慎坦,杜伟,等.利用BCR改进法和Tessier修正法提取不同类型土壤中Cu、Zn、Fe、Mn的对比研究[J].分析测试学报,2009,3(28):297-300
[19]  全国土壤普查办公室.中国土壤[M].中国农业出版社, 1998:875-876

Full-Text

Contact Us

service@oalib.com

QQ:3279437679

WhatsApp +8615387084133