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化学进展 2014

卤代有机污染物的光化学降解

DOI: 10.7536/PC131134, PP. 1079-1098

张峰振,吴超飞,胡芸,韦朝海

Keywords: 卤代有机污染物,光催化,直接光解,羟基自由基,水合电子

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Abstract:

包括全氟或部分氟代化合物（PFCs）、氯代有机物（COCs）以及溴代有机物（BOCs）等的卤代有机污染物（halogenatedorganiccontaminants，HOCs）排放到环境中会表现出持久性有机污染物的特征，因此涉及HOCs性质、光吸收与量子效应、材料与界面特性、环境条件等方面优化的光化学清除方法成为一个重要的研究方向。基于此，本文归纳分析了光激发催化剂产生活性物种如hVB+、eCB-、·OH、eaq-等氧化或还原全氟辛酸、多氯联苯、多溴联苯醚的反应机理及直接光解机理，指出HOCs的光化学降解主要是通过其与活性物种之间电子转移或其激发态光致还原脱卤来实现，认为光催化材料和反应过程优化设计是影响光催化降解HOCs的重要因素。基于目前已经取得的研究发现与成果，从界面电子转移、材料能带信息、反应与分离集成化等方面提出本领域未来学术与技术层面值得深入探索的关键问题。

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