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化学进展 2015

基于金属-有机骨架前驱体的先进功能材料

DOI: 10.7536/PC140925, PP. 174-191

张慧,周雅静,宋肖锴

Keywords: 金属-有机骨架,前驱体,多孔碳材料,金属氧化物,复合材料

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Abstract:

由于金属-有机骨架(metal-organicframeworks,MOFs)结构中含有碳源(有机配体)和金属源(金属或金属簇)物质,以MOFs为前驱体合成先进功能材料,如纳米多孔碳材料和金属氧化物纳米材料,是目前MOFs化学以及新功能材料研究领域一个新的热点。本文综述了近年来以MOFs为前驱体制备碳材料(纳米多孔碳材料、碳纳米点、碳纳米管等)、金属氧化物纳米材料(单金属氧化物Fe2O3、ZnO、Co3O4、MgO、In2O3等;多金属氧化物纳米复合材料Gd2O3/Eu2O3、Fe2O3@TiO2等)、金属氧化物/碳纳米复合材料(Fe3O4/C、ZnO/C等)等的合成方法,以及这些先进功能材料在超级电容器(supercapacitor)、氧还原反应(ORR)催化剂、氢气吸附、CO2捕获、光催化制氢催化剂等研究领域的应用,并对其今后的发展进行了展望。

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