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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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含CO2/离子液体系统相行为及其在反应与分离中的应用进展
, PP. 441-449
Keywords: 超临界CO2,离子液体,相行为,反应分离,过程耦合
Abstract:
目前已知的绿色溶剂主要包括超临界流体（Supercriticalfluids，SCFs）、离子液体（Ionicliquids，ILs）、二氧化碳膨胀液体（CO2expandedliquids,CXLs）、水以及上述溶剂的混合物等。其中，由超临界CO2（SupercriticalCO2，SCCO2）与ILs混合而构成的新兴溶剂，因为化学热力学方面的特性，成为近年来研究的热点，未来很有发展前景。本文回顾了目前为止在该领域所开展的工作，总结了影响SCCO2与IL相行为的主要因素。包括温度、压力、ILs的含水量、ILs的阴离子、ILs的阳离子、ILs的摩尔体积以及助溶剂等。同时分析了ILs/SCCO2与溶质形成的多元混合物相行为的成因。介绍了ILs/CO2在萃取、反萃取、膜分离、反胶束、萃取与反应耦合等分离方面的应用。由于传统的单元操作很难满足无污染和对过程集成的要求，因而含有ILs/SCCO2的分离反应耦合过程将是未来是实现清洁生产的发展方向。
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