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化学进展  2011 

核壳结构:燃料电池中实现低铂电催化剂的最佳途径

, PP. 852-859

Keywords: 低温燃料电池,电催化剂,核壳结构

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Abstract:

电催化剂是决定低温燃料电池性能、寿命和成本的关键材料之一,核壳结构电催化剂由于其在降低铂载量、提高催化剂活性方面表现出的良好性质,已成为燃料电池领域的研究热点。本文综述了低温燃料电池核壳结构电催化剂的最新研究进展。首先,在概述核壳结构电催化剂总体特征的基础上,详细介绍了核壳结构电催化剂的制备方法,主要包括胶体法、热分解法、置换法、电化学法等,其中胶体法是目前应用最为广泛的一种方法,具有合成过程简单易控等优点;置换法和电化学法则是在最近几年得到了迅速的发展,并有望用于核壳结构电催化剂的批量化生产。然后,分别从二元及其他多元催化剂组成方面阐述了核壳型电催化剂体系的研究进展,核壳结构电催化剂不仅可有效提高贵金属铂的质量比活性,同时,其他金属元素与铂之间存在的相互作用可对电催化剂的活性及稳定性产生十分重要的调变作用。最后,我们对低温燃料电池核壳结构电催化剂的发展趋势作了展望。

References

[1]  衣宝廉(Yi B L). 燃料电池--高效、环境友好的发电方式(Fuel Cells--Efficient and Environmentally friendly Way to Power generation). 北京:化学工业出版社(Beijing: Chemical Industry Press), 2000. 5-9
[2]  Borup R, Meyers J, Pivovar B, Kim Y S, Mukundan R, Garland N, Myers D, Wilson M, Garzon F, Wood D, Zelenay P, More K, Stroh K, Zawodzinski T, Boncella J, McGrath J E, Inaba M, Miyatake K, Hori M, Ota K, Ogumi Z, Miyata S, Nishikata A, Siroma Z, Uchimoto Y, Yasuda K, Kimijima K I, Iwashita N. Chem. Rev., 2007, 107: 3904-3951
[3]  Santiago E I, Varanda L C, Villullas H M. J. Phys. Chem. C, 2007, 111: 3146-3151
[4]  Stamenkovic V, Schmidt T J, Ross P N, Markovic N M. J. Phys. Chem. B, 2002, 106: 11970-11979
[5]  Alayoglu S, Eichhorn B. J. Am. Chem. Soc., 2008, 130: 17479-17486
[6]  Cao L Y, Tong L M, Diao P, Zhu T, Liu Z F. Chem. Mater., 2004, 16: 3239-3245
[7]  Sobal N S, Ebels U, Mohwald H, Giersig M. J. Phys. Chem. B, 2003, 107: 7351-7354
[8]  Lee M H, Do J S. J. Power Sources, 2009, 188: 353-358
[9]  Zeng J H, Yang J, Lee J Y, Zhou W J. J. Phys. Chem. B, 2006, 110: 24606-24611
[10]  Yang J H, Zhou W J, Cheng C H, Lee J Y, Liu Z L. ACS Applied Materials Int., 2010, 2: 119-126
[11]  Yang J H, Lu L H, Wang H S, Zhang H J. Scripta Mater., 2006, 54: 159-162
[12]  Schimizu K, Cheng I F, Wai C M. Electrochem. Commun., 2009, 11: 691-694
[13]  Zhou W P, Sasaki K, Su D, Zhu Y M, Wang J X, Adzic R R. J. Phys. Chem. C, 2010, 114: 8950-8957
[14]  Zhou W P, Yang X F, Vukmirovic M B, Koel B E, Jiao J, Peng G W, Mavrikakis M, Adzic R R. J. Am. Chem. Soc., 2009, 131: 12755-12762
[15]  Jin Y D, Shen Y, Dong S J. J. Phys. Chem. B, 2004, 108: 8142-8147
[16]  Jiang L H, Hsu A, Chu D, Chen R R. Electrochim. Acta, 2010, 55: 4506-4511
[17]  Harpeness R, Gedanken A. Langmuir, 2004, 20: 3431-3434
[18]  Mani P, Srivastava R, Strasser P. J. Phys. Chem. C, 2008, 112: 2770-2778
[19]  Wang H, Xu C W, Cheng F L, Zhang M, Wang S Y, Jiang S P. Electrochem. Commun., 2008, 10: 1575-1578
[20]  Ah C S, Kim S J, Jang D J. J. Phys. Chem. B, 2006, 110: 5486-5489
[21]  Lim B, Jiang M J, Camargo P H C, Cho E C, Tao J, Lu X M, Zhu Y M, Xia Y A. Science, 2009, 324: 1302-1305
[22]  Adzic R R. J. Am. Chem. Soc., 2005, 127: 12480-12481
[23]  Kristian N, Wang X. Electrochem. Commun., 2008, 10: 12-15
[24]  Guo S J, Fang Y X, Dong S J, Wang E. J. Phys. Chem. C, 2007, 111: 17104-17109
[25]  Kang J Q, Ma W T, Wu J J, Pan M. Catal. Commun., 2009, 10: 1271-1274
[26]  Liu Z F, Hu J E, Wang Q, Gaskell K, Frenkel A I, Jackson G S, Eichhorn B. J. Am. Chem. Soc., 2009, 131: 6924-6925
[27]  Lee K S, Park I S, Park H Y, Jeon T Y, Sung Y E. Catal. Today, 2009, 146: 20-24
[28]  Wu Y N, Liao S J, Liang Z X, Yang L J, Wang R F. J. Power Sources, 2009, 194: 805-810
[29]  Shao M H, Sasaki K. Marinkovic N S, Zhang L H, Adzic R R. Electrochem. Commun., 2007, 9: 2848-2853
[30]  Ramirez-Caballero G E, Ma Y G, Callejas-Tovar R, Balbuena P B. Phys. Chem. Chem. Phys., 2010, 12: 2209-2218
[31]  Wang R F, Li H, Feng H Q, Wang H, Lei Z Q. J. Power Sources, 2010, 195: 1099-1102
[32]  Zeis R, Mathur A, Fritz G, Lee J, Erlebacher J. J. Power Sources, 2007, 165: 65-72
[33]  Sarapuu A, Kallip S, Kasikov A, Matisen L, Tammeveski K. J. Electroanal. Chem., 2008, 624: 144-150
[34]  Liao S J, Holmes K A, Tsaprailis H, Birss V I. J. Am. Chem. Soc., 2006, 128: 3504-3505
[35]  Ma L, Zhang H M, Liang Y M, Xu D Y, Ye W, Zhang J L, Yi B L. Catal. Commun., 2007, 8: 921-925
[36]  Alex B, Elod L G, Colin W O. J. Power Sources, 2007, 167: 281-287
[37]  Wang Z B, Yin G P, Shao Y Y, Yang B Q, Shi P F, Feng P X. J. Power Sources, 2007, 165: 9-15
[38]  Baglio V, Arico A S, Stassi A, Urso C, Di B A, Castro L A M, Antonucci V. J. Power Sources, 2006, 159: 900-904
[39]  Yang H, Alonso-Vante N, Leger J M, Lamy C. J. Phys. Chem. B, 2004, 108: 1938-1947
[40]  Alayoglu S, Nilekar A U, Mavrikakis M, Eichhorn B. Nature Materials, 2008, 7: 333-338
[41]  Wu Y N, Liao S J, Su Y L, Zeng J H, Dang D. J. Power Sources, 2010, 195: 6459-6462
[42]  Do J S, Chen Y T, Lee M H. J. Power Sources, 2007, 172: 623-632
[43]  Lee M H, Wang P S, Do J S. J. Solid State Electrochem., 2008, 12: 879-884
[44]  Grzegorz W S, Francis P Z. Langmuir, 2007, 23: 10357-10365
[45]  Wei Z D, Feng Y C, Li L, Liao M J, Fu Y, Sun C X, Shao Z G, Shen P K. J. Power Sources, 2008, 180: 84-91
[46]  Vukmirovic M B, Zhang J, Sasaki K, Nilekar A U, Uribe F, Mavrikakis M, Adzic R R. Electrochim. Acta, 2007, 52: 2257-2263
[47]  Wang J X, Inada H, Wu L J, Zhu Y M, Choi Y M, Liu P, Zhou W P, Adzic R R. J. Am. Chem. Soc., 2009, 131: 17298-17302
[48]  Ghosh T, Vukmirovic M B, Disalvo F J, Adzic R R. J. Am. Chem. Soc., 2010, 132: 906-907
[49]  Adzic R R, Zhang J, Sasaki K, Vukmirovic M B, Shao M, Wang J X, Nilekar A U, Mavrikakis M, Valerio J A, Uribe F. Top. Catal., 2007, 46: 249-262
[50]  Sasaki K, Wang J X, Naohara H, Marinkovic N, More K, Inada H, Adzic R R. Electrochim. Acta, 2010, 55: 2645-2652
[51]  Ma Y W, Zhang H M, Zhong H X, Xu T, Jin H, Geng X Y. Catal. Commun., 2010, 11: 434-437
[52]  Fu X Z, Liang Y, Chen S P, Lin J D, Liao D W. Catal. Commun., 2009, 10: 1893-1897
[53]  Zhao H B, Li L, Yang J, Zhang Y M. Electrochem. Commun., 2008, 10: 1527-1529
[54]  Zhang W, Wang R, Wang H, Lei Z. Fuel Cells, 2010, 10: 734-749
[55]  Wang R F, Li H, Ji S, Wang H, Lei Z Q. Electrochim. Acta, 2010, 55: 1519-1522
[56]  Wang W, Wang R F, Ji S, Feng H Q, Wang H, Lei Z Q. J. Power Sources, 2010, 195: 3498-3503
[57]  Gong K P, Chen W F, Sasaki K, Su D, Vukmirovic M B, Zhou W P, Izzo E, Perez-Acosta C, Hirunsit P, Balbuena P B, Adzic R R. J. Electroanal. Chem., 2010, 649: 232-237

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