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OALib Journal期刊
ISSN: 2333-9721
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基于脲基氢键组装的功能超分子凝胶
DOI: 10.7536/PC130525, PP. 125-139
Keywords: 超分子凝胶,功能凝胶,刺激响应性,脲基凝胶因子,氢键,自组装
Abstract:
有机小分子化合物在分子间氢键、π-π堆积、亲疏水作用、范德华力等非共价键弱相互作用力驱动下，自组装形成三维网络结构的物理凝胶称为超分子凝胶。含有脲基的凝胶因子由于其强氢键缔合能力以及与阴离子、金属离子、卤素化合物等作用的可调变多样性，成为组装超分子凝胶中特别有效的氢键组装单元。本文分别从单脲基、双脲基和多脲基的凝胶因子分类综述了基于脲基氢键组装的功能超分子凝胶的研究工作，特别是近几年来的重要进展。对一些成功例子，从分子设计及成胶操作条件控制等方面的精细调谐如何解决聚集-溶解这对主要矛盾，从而实现溶胶-凝胶的转化及其可能的应用前景进行了评述。本文展望了该领域的发展方向与趋势，指出超分子凝胶研究经过多年的快速发展，深化对其蕴含机制以及动力学过程的认识与调控以实现具有多种刺激响应、多重信号输出的多组分复合功能凝胶体系的加工制备是发展趋势与必然要求，展现出广泛的应用前景也极富挑战性。
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