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化学进展 2006

加氢脱氮催化研究的新进展

, PP. 417-428

刘大鹏,李永丹

Keywords: 加氢脱氮,有机氮化物,金属硫化物,金属碳化物,金属氮化物,金属磷化物,活性位本质,C—N断裂,反应网络

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Abstract:

化石燃料的加氢脱氮有利于改善油品质量及其稳定性，同时避免燃烧时NOx的排放。本文介绍了不同化石燃料中有机氮化物的含量及类型，对不同加氢脱氮催化剂及其催化活性位的本质进行了探讨，同时论述了C—N键断裂机理及燃料中主要有机氮化物的HDN反应网络。着重概述了传统金属硫化物催化剂的改性方法，新型的金属碳化物、金属氮化物和金属磷化物催化剂的研究现状。

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