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化学进展  2010 

氧化锰基催化剂低温NH3选择性还原NOx反应及其机理*

, PP. 1882-1900

Keywords: 氮氧化物,氨气选择性催化还原,氧化锰,反应机理,抗湿性能

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Abstract:

近年来,氧化锰基催化剂由于在低温氨选择性催化还原(NH3-SCR)NOx反应中表现出优良的催化活性得到了广泛的关注。本文综述了氧化锰基催化剂低温NH3-SCR反应的研究进展,分别分析了氧化锰的氧化态、晶体结构和表面结构以及掺杂离子和载体类型等因素对其催化性能的影响高的氧化态的锰和高比表面积的催化剂有利于低温NH3-SCR反应;金属离子如铈、铬、铁、铜和锡等的掺杂可以提高NOx的转化率和/或N2选择性;具有独特性能的载体如TiO2或硅铝分子筛等可以进一步提高氧化锰基催化剂的抗湿和抗硫性能等。本文同时分别对活化NH3、NO或同时活化NO和NH3的低温NH3-SCR反应机理进行了详细总结,根据不同的反应条件,在氧化锰基催化剂上很多低温NH3-SCR反应,Eley-Rideal、Langmuir-Hinshelwood以及Mars-vanKrevelen机理可能是同时存在的。本文最后论证和指出了氧化锰基催化剂低温NH3-SCR反应研究的主要发展方向。

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