|
- 2015
镁钙合金表面贻贝类吸附蛋白膜的NaIO4氧化处理及抗腐蚀性能
|
Abstract:
摘要 利用极化曲线及电化学阻抗谱,并结合扫描电镜、原子力显微镜、电子探针显微镜及红外光谱技术研究氧化处理对镁钙合金表面贻贝类吸附蛋白膜层抗蚀性能的影响. 结果表明,在NaIO4氧化作用下,镁钙合金表面的贻贝吸附蛋白(Mefp-1)膜层由孔状结构转变为网状结构,且趋于均匀致密;未氧化处理的蛋白膜层对镁钙合金的保护作用随时间逐渐增加,而氧化处理的蛋白膜层使镁钙合金的点蚀电位正移,3 d时其腐蚀保护性能达到最佳,浸泡时间延长,膜层的防护性能略有下降
[1] | Kim W C, Kim J G, Lee J Y, et al. Influence of Ca on the corrosion properties of magnesium for biomaterials[J]. Materials Letters, 2008, 62(25): 4146-4148. |
[2] | Waite J H. Adhesion a la moule[J]. Integrative and comparative biology, 2002, 42(6): 1172-1180. |
[3] | Jung J Y, Kwon S J, Han H S, et al. Rapid in vitro corrosion induced by crack-like pathway in biodegradable Mg-10% Ca alloy[J]. Microscopy and Microanalysis, 2013, 19(Suppl 5): 210-214. |
[4] | Guo J B (郭京波), Tao Z Y (陶宗娅), Nuo X G (罗学刚). Analysis of Bamboo Lignin with FTIR and XPS[J]. Acta Chimica Sinica (化学学报), 2005, 63(16): 1536-1540. |
[5] | Zvarec O, Purushotham S, Masic A, et al. Catechol-functionalized chitosan/iron oxide nanoparticle composite inspired by mussel thread coating and squid beak interfacial chemistry[J]. Langmuir, 2013, 29(34): 10899-10906. |
[6] | Guo X W, Chang J W, He S M, et al. Investigation of corrosion behaviors of Mg–6Gd–3Y–0.4 Zr alloy in NaCl aqueous solutions[J]. Electrochimica Acta, 2007, 52(7): 2570-2579. |
[7] | Wan D, Wang J, Lin L, et al. Damping properties of Mg-Ca binary alloys[J]. Physica B: Condensed Matter, 2008, 403(13-16): 2438-2442. |
[8] | Fant C, Hedlund J, H??k F, et al. Investigation of adsorption and cross-linking of a mussel adhesive protein using attenuated total internal reflection Fourier transform infrared spectroscopy (ATR-FTIR)[J]. The Journal of Adhesion, 2010, 86(1): 25-38. |
[9] | Zhang F, Sababi M, Brinck T, et al. In situ investigations of Fe3+ induced complexation of adsorbed Mefp-1 protein film on iron substrate[J]. Journal of colloid and interface science, 2013, 404: 62-71. |
[10] | Poursaee A. Determining the appropriate scan rate to perform cyclic polarization test on the steel bars in concrete[J]. Electrochimica Acta, 2010, 55(3): 1200-1206. |
[11] | Cai C, Zhang Z, Wei Z L, et al. Electrochemical and corrosion behaviors of pure Mg in neutral 1.0% NaCl solution[J]. Transactions of Nonferrous Metals Society of China, 2012, 22(4): 970-976. |
[12] | Keera S, Deyab M. Effect of some organic surfactants on the electrochemical behaviour of carbon steel in formation water[J]. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2005, 266(1): 129-140. |
[13] | Ye C Q, Hu R G, Dong S G, et al. EIS analysis on chloride-induced corrosion behavior of reinforcement steel in simulated carbonated concrete pore solutions[J]. Journal of Electroanalytical Chemistry, 2012, 688: 275-281. |
[14] | Zhang F, Pan J, Claesson P M. Electrochemical and AFM studies of mussel adhesive protein (Mefp-1) as corrosion inhibitor for carbon steel[J]. Electrochimica Acta, 2011, 56(3): 1636-1645. |
[15] | Zhang F, Pan J, Claesson P M, et al. Electrochemical, atomic force microscopy and infrared reflection absorption spectroscopy studies of pre-formed mussel adhesive protein films on carbon steel for corrosion protection[J]. Thin Solid Films, 2012, 520 (24): 7136-7143. |
[16] | Haemers S, Van der Leeden M C, Koper G J, et al. Cross-linking and multilayer adsorption of mussel adhesive proteins[J]. Langmuir, 2002, 18 (12): 4903-4907. |
[17] | Haemers S, Van der Leeden M, Nijman E, et al. The degree of aggregation in solution controls the adsorbed amount of mussel adhesive proteins on a hydrophilic surface[J]. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2001, 190(1): 193-203. |
[18] | Gu X N, Li N, Zhou W R, et al. Corrosion resistance and surface biocompatibility of a microarc oxidation coating on a Mg-Ca alloy[J]. Acta Biomaterialia, 2011, 7(4): 1880-1889. |
[19] | Harrington M J, Masic A, Holten-Andersen N, et al. Iron-clad fibers: A metal-based biological strategy for hard flexible coatings[J]. Science, 2010, 328(5975): 216-220. |
[20] | Wei W, Yu J, Broomell C, et al. Hydrophobic enhancement of Dopa-mediated adhesion in a mussel foot protein[J]. Journal of the American Chemical Society, 2013, 135(1): 377-383. |
[21] | Doraiswamy A, Narayan R, Cristescu R, et al. Laser processing of natural mussel adhesive protein thin films[J]. Materials Science and Engineering: C, 2007, 27(3): 409-413. |
[22] | Nuo M (罗曼), Guan P (关平), Liu W H (刘文汇). The identification of several saturated fatty acids and their salts by means of infrared spectrometry [J]. Spectroscop y and Spectral Analysis(光谱学与光谱分析), 2007, 27(2): 250-253. |
[23] | Liu C L, Wang Y J, Zeng R C, et al., In vitro corrosion degradation behaviour of Mg-Ca alloy in the presence of albumin[J]. Corrosion Science, 2010, 52(10): 3341-3347. |
[24] | Haemers S, van der Leeden M C, Frens G. Coil dimensions of the mussel adhesive protein Mefp-1[J]. Biomaterials, 2005, 26(11): 1231-1236. |
[25] | Haemers S, Koper G J, Frens G. Effect of oxidation rate on cross-linking of mussel adhesive proteins[J]. Biomacromolecules, 2003, 4(3): 632-640. |
[26] | Li Z, Gu X, Lou S, et al. The development of binary Mg-Ca alloys for use as biodegradable materials within bone[J]. Biomaterials, 2008, 29(10): 1329-1344. |
[27] | Hedlund J, Andersson M, Fant C, et al. Change of colloidal and surface properties of Mytilus edulis foot protein 1 in the presence of an oxidation (NaIO4) or a complex-binding (Cu2+) agent[J]. Biomacromolecules, 2009, 10(4): 845-849. |