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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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Selectiveoxidationofsulfursandoxidationdesulfurizationofmodeloilby12-tungstophosphoricacidoncobalt-ferritenanoparticlesasmagneticallyrecoverablecatalyst
DOI: 10.1016/S1872-2067(15)60862-2, PP. 1342-1349
Keywords: Phosphotungsticacid,Cobalt,Ferrite,Oxidativedesulfurization,Dibenzothiophene,Magneticcatalyst
Abstract:
？Silica-coatedCoFe2O4nanoparticleswerepreparedandusedasasupportfortheimmobilizationof12-tungstophosphoricacid,toproduceanewmagneticallyseparablecatalyst.ThiscatalystwascharacterizedusingX-raydiffraction,wavelength-dispersiveX-rayspectroscopy,Fourier-transforminfraredspectroscopy,scanningelectronmicroscopy,transmissionelectronmicroscopy,laserparticlesizeanalysis,andvibratingsamplemagnetometry.Thecatalystshowedhighactivityintheselectiveoxidationofthioethersandthiophenestothecorrespondingsulfonesundermildconditions.Thecatalyticactivityofthenanocatalystintheoxidativedesulfurizationofmodeloilwasinvestigated.Theeffectofnitrogen-containingcompoundsonsulfurremovalfromthemodeloilwasalsoevaluated.Thecatalystshowedhighactivityintheoxidativedesulfurizationofdiesel.Thecatalystcanbereadilyisolatedfromtheoxidationsystemusinganexternalmagnetandnoobviouslossofactivitywasobservedwhenthecatalystwasreusedinfourconsecutiveruns.
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