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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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LocationandorientationoftheN,N-diisopropylethylaminetemplatemoleculeintheAlPO4-18frameworkbyX-raysynchrotrondiffractionandmolecularmodelling
DOI: 10.1016/S1872-2067(14)60306-5, PP. 874-879
Keywords: Microporousmaterial,Smallpore,AlPO-18,Structure,Molecularmodeling,X-raydiffraction,Templatelocation
Abstract:
？PhasepureAlPO4withtheAlPO4-18(AEI)structurewassynthesisedusingN,N-diisopropylethylamineasatemplate.UsingacombinationofX-raypowderdiffractionandcomputationalmethods,thelocationandorientationoftheN,N-diisopropylethylaminemoleculesinsidethecagesoftheAEIstructureweredetermined.Thermogravimetricanalysisconfirmedthatthenumberoftemplatemoleculesperunitcellwasconsistentwiththediffractionstudy.WeunequivocallyshowthatonlyonetemplatemoleculeispresentineachcageofthecrystallineAEImaterial.Ourworkdemonstratesthatacombinedapproachenablesaccuratestructureresolutionofsuchcomplexmaterials.
| [1] | Li J Y, Yu J H, Xu R R. Chin J Inorg Chem (李激扬, 于吉红, 徐如人. 无机化学学报), 2004, 20: 1
|
| [2] | Simmen A, McCusker L B, Baerlocher C, Meier W M. Zeolites, 1991, 11: 654
|
| [3] | Thomas J M, Raja R, Sankar G, Bell R G. Nature, 1999, 398: 227
|
| [4] | Thomas J M, Raja R, Sankar G, Bell R G. Acc Chem Res, 2001, 34: 191
|
| [5] | Yu J H, Xu R R. Chem Soc Rev, 2006, 35: 593
|
| [6] | Barrett P A, Sankar G, Stephenson R, Catlow C R A, Thomas J M, Jones R H, Teat S J. Solid State Sci, 2006, 8: 337
|
| [7] | Martinez-Franco R, Moliner M, Yun Y F, Sun J L, Wan W, Zou X D, Corma A. Proc Natl Acad Sci U S A, 2013, 110: 3749
|
| [8] | Stocker M. Microporous Mesoporous Mater, 1999, 29: 3
|
| [9] | Ma L, Cheng Y S, Cavataio G, McCabe R W, Fu L X, Li J H. Chem Eng J, 2013, 225: 323
|
| [10] | Mathisen K, Stockenhuber M, Nicholson D G. Phys Chem Chem Phys, 2009, 11: 5476
|
| [11] | Lewis D W, Catlow C R A, Thomas J M. Chem Mater, 1996, 8: 1112
|
| [12] | Muncaster G, Davies A T, Sankar G, Catlow C R A, Thomas J M, Colston S L, Barnes P, Walton R I, O'Hare D. Phys Chem Chem Phys, 2000, 2: 3523
|
| [13] | Rey F, Sankar G, Thomas J M, Barrett P A, Lewis D W, Catlow C R A, Clark S M, Greaves G N. Chem Mater, 1995, 7: 1435
|
| [14] | Sanchez-Sanchez M, Sankar G, Simperler A, Bell R G, Catlow C R A, Thomas J M. Catal Lett, 2003, 88: 163
|
| [15] | Sankar G, Wyles J K, Catlow C R A. Top Catal, 2003, 24: 173
|
| [16] | Marchese L, Frache A, Gianotti E, Martra G, Causa M, Coluccia S. Microporous Mesoporous Mater, 1999, 30: 145
|
| [17] | Briend M, Vomscheid R, Peltre M J, Man P P, Barthomeuf D. J Phys Chem, 1995, 99: 8270
|
| [18] | Chen J S, Thomas J M, Sankar G. J Chem Soc, Faraday Trans, 1994, 90: 3455
|
| [19] | McCusker L B, Baerlocher C. Stud Surf Sci Catal, 2007, 168: 13
|
| [20] | McCusker L B, Von Dreele R B, Cox D E, Louer D, Scardi P. J Appl Crystallogr, 1999, 32: 36
|
| [21] | Freeman C M, Catlow C R A, Thomas J M, Brode S. Chem Phys Lett, 1991, 186: 137
|
| [22] | Discover 3.1. Biosym Technologies Inc, San Diego, USA, 1996
|
| [23] | Maple J R, Dinur U, Hagler A T. Proc Natl Acad Sci U S A, 1988, 85: 5350
|
| [24] | Martis M, Smith A J, Tang C, Parker J E, Hyde T I, Watson M J, Baucherel X, Kohara S, Wakihara T, Sankar G. Phys Chem Chem Phys, 2013, 15: 11766
|
| [25] | Lewis D W, Freeman C M, Catlow C R A. J Phys Chem, 1995, 99: 11194
|
| [26] | Flanigen E M, Lok B M, Patton R L, Wilson S T. Pure Appl Chem, 1986, 58: 1351
|
| [27] | Wilson S T, Lok B M, Messina C A, Cannan T R, Flanigen E M. J Am Chem Soc, 1982, 104: 1146
|
| [28] | Wilson S T, Lok B M, Messina C A, Cannan T R, Flanigen E M. ACS Symp Ser, 1983, 218: 79
|
| [29] | Cheetham A K, Ferey G, Loiseau T. Angew Chem Int Ed, 1999, 38: 3268
|
| [30] | Cheetham A K, Rao C N R. MRS Bull, 2005, 30: 93
|
| [31] | Hartmann M, Elangovan S P. Adv Nanoporous Mater, 2009, 1: 237
|
| [32] | Li J Y, Yu J H, Xu R R. Proc Royal Soc A, 2012, 468: 1955
|
| [33] | Chen J S, Thomas J M. J Chem Soc, Chem Commun, 1994: 603
|
| [34] | Zenonos C, Sankar G, Cora F, Lewis D W, Pankhurst Q A, Catlow C R A, Thomas J M. Phys Chem Chem Phys, 2002, 4: 5421
|
| [35] | Sankar G, Wyles J K, Jones R H, Thomas J M, Catlow C R A, Lewis D W, Clegg W, Coles S J, Teat S J. Chem Commun, 1998: 117
|
| [36] | Burton A, Darton R J, Davis M E, Hwang S J, Morris R E, Ogino I, Zones S I. J Phys Chem B, 2006, 110: 5273
|
| [37] | Catlow C R A, Ackermann L, Bell R G, Gay D H, Holt S, Lewis D W, Nygren M A, Sastre G, Sayle D C, Sinclair P E. J Mol Catal A, 1997, 115: 431
|
| [38] | Larson A C, Dreele R B V. GSAS Generalised Crystal Structure Analysis System. Los Alamos National Laboratory, Los Alamos, New Mexico, USA, 1997
|
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