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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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SizedependenceofphotocatalyticoxidationreactionsofRhnanoparticlesdispersedon(Ga1-xZnx)(N1-xOx)support
DOI: 10.1016/S1872-2067(14)60181-9, PP. 1944-1954
Keywords: Oxynitride,Rhodiumnanoparticle,Watersplitting,Carbonmonoxideoxidation,Hydrogenoxidation
Abstract:
？MixedGa-Znoxynitridesweresynthesizedusingcoprecipitation,wet-precipitation,andsolid-solutionmethods.TheoxynitrideswereusedassupportsforRhnanoparticlecatalystsinphotocatalyticwatersplitting,COoxidation,andH2oxidation.MixedGa-Znoxynitridesproducedbywetprecipitationandnitridationhadgoodvisible-light-absorptionpropertiesandhighsurfaceareas,sotheywereusedtosupportuniformlysizedpoly(vinylpyrrolidone)-stabilizedRhnanoparticles.Thenanoparticlesizerangewas2-9nm.ThesecatalystshadnegligibleactivityinphotocatalyticH2productionbywatersplittingwithmethanolasasacrificialagent.OthermixedGa-Znoxynitrideswerealsoinactive.AreferencesampleprovidedbyDomenalsoshowedverylowactivity.TheinfluenceofparticlesizeonRh-catalyzedoxidationofCOandH2wasinvestigated.ForCOoxidation,theactivitiesofsmallparticleswerehigherforparticleswithhigherRhoxidationdegrees.TheoppositeholdsforH2oxidation.
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