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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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基于TiO2的绿色多相催化剂催化CO2与环氧化合物偶联反应
DOI: 10.1016/S1872-2067(14)60110-8, PP. 1669-1675
Keywords: 二氧化碳,环氧化合物,环碳酸酯,多相催化剂,掺杂纳米二氧化钛
Abstract:
？金属离子掺杂纳米TiO2（M-TiO2，M=Zn2+，Cu2+，CO2+，Mn2+，Ni2+）在CO2与环氧化合物的偶联反应中表现出较高的催化活性.反应以四正丁基碘化铵（TBAI）为共催化剂，在无溶剂条件下进行.考察了反应温度、反应时间和CO2压力在Zn-TiO2/TBAI体系中对反应性能的影响.作为无毒的多相催化剂，Zn-TiO2可循环使用5次，其催化活性没有明显降低.
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