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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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OnthephotoactivityofS-dopednanoporouscarbons：Importanceofsurfacechemistryandporosity
DOI: 10.1016/S1872-2067(14)60100-5, PP. 807-814
Keywords: Nanoporouscarbons,Photoactivity,Oxidation,Surfacechemistry,Oxygenreductionreaction(ORR),Capacitivebehavior
Abstract:
？ThisminireviewsummarizesourrecentfindingsonthephotoactivityofS-dopednanoporouscarbons.Thematerialswereeithersynthesizedfromthesulfur-containingpolymersorobtainedbyheattreatmentofcommercialcarbonwithhydrogensulfide.Theirsurfacewasextensivelycharacterizedfromthepointsofviewofitssurfacechemistry,porosity,morphology,andelectronicproperties.Thecarbonsshowedenhancedactivitytowardsoxidationofarsineandremovalofdibenzothiophenesfrommodeldieselfuel.ThelatterwereoxidizedtovariousoxygencontainingintermediatesandthecleavageofC-CbondsinaromaticringwasdetectedwhencarbonwithadsorbedspecieswasexposedtoUVorvisiblelight.Irradiationresultedingenerationofphotocurrentinabroadrangeofwavelength.Thepresenceofsulfurledtothereductionofoxygenandcontributedtoanincreasedcapacitiveperformance.Welinktheseeffectstothepresenceofreducedsulfurinthesmallporeswhichenhancesthedispersiveinteractionsviainducingapositivechargetocarbonatoms,tosulfurinoxygenatedformswhichcontributetoFaradaicreactionsandincreasethepolarinteractions,andtothehydrophobicityofasurfaceinsmallporeswhereoxygencanbereducedbyexcitedelectronsfromchromophoric-likesulfurcontaininggroups.
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