|
OALib Journal期刊
ISSN: 2333-9721
费用：99美元
|
|
|
|
预处理方法对Ru/SBA-15催化丙三醇氢解反应性能的影响
DOI: 10.1016/S1872-2067(14)60032-2, PP. 677-683
Keywords: 钌,负载型催化剂,丙三醇,氢解反应,预处理,结构敏感反应
Abstract:
？使用浸渍法结合不同预处理方法制备了一系列的Ru/SBA-15催化剂，并将其应用于丙三醇氢解反应中.使用N2吸附-脱附、X射线衍射、CO化学吸附以及透射电子显微镜等方法对所制备Ru/SBA-15进行了表征.结果表明，催化剂前驱体经过空气焙烧后再经H2还原的Ru/SBA-15催化剂上Ru的分散度较低，而直接使用H2处理较高.同时，随着H2还原温度提高，Ru分散度逐渐降低.保持反应活性接近时，随着Ru分散度的降低，TOF增加.表明Ru/SBA-15催化剂上丙三醇氢解是结构敏感反应.
| [1] | Omata K, Izumi S, Murayama T, Ueda W. Catal Today, 2013, 201: 7
|
| [2] | Kwak B K, Park D S, Yun Y S, Yi J. Catal Commum, 2012, 24: 90
|
| [3] | Niu L, Wei R P, Yang H, Li X, Jing F, Xiao G M. Chin J Catal (牛磊, 魏瑞平, 杨慧, 李想, 姜枫, 肖国民. 催化学报), 2013, 34: 2230
|
| [4] | Huang L, Zhu Y L, Zheng H Y, Ding G Q, Li Y W. Catal Lett, 2009, 131: 312
|
| [5] | Ma L, He D H, Li Z P. Catal Commun, 2008, 9: 2489
|
| [6] | Huang Z W, Cui F, Kang H X, Chen J, Xia C G. Appl Catal A, 2009, 366: 288
|
| [7] | Gsllegos-Suarez E, Perez-Cademas M, Guerrero-Ruiz A, Rodriguez-Ramos I, Arcoya A. Appl Surf Sci, 2013, 287: 108
|
| [8] | Liu H Z, Liang S G, Jiang T, Han B X, Zhou Y X. Clean Soil Air Water, 2012, 40: 318
|
| [9] | Feng J, Fu H Y, Wang J B, Li R X, Chen H, Li X J. Catal Commun, 2008, 9: 1458
|
| [10] | Zhou W, He D H. Chem Commun, 2008, 9: 5839
|
| [11] | Ma L, Li Y M, He D H. Chin J Catal (马兰, 李宇明, 贺德华. 催化学报), 2011, 32: 872
|
| [12] | Ma L, He D H. Chin J Catal (马兰, 贺德华. 催化学报), 2009, 30: 471
|
| [13] | Ni X, Zhang B, Li C, Pang M, Su D, Williams C, Liang C. Catal Commun, 2012, 24: 65
|
| [14] | Kang J C, Zhang S L, Zhang Q H, Wang Y. Angew Chem Int Ed, 2009, 48: 2565
|
| [15] | Bezemer G L, Bitter J H, Kuipers H P C E, Oosterbeek H, Holewijn J E, Xu X D, Kapteijn F, van Dillen A, Jong K P. J Am Chem Soc, 2006, 128: 3956
|
| [16] | Prieto G, Martínez A, Concepción P, Morcno-Tost R. J Catal, 2009, 266: 129
|
| [17] | Li Q Y, Ji S F, Hu J Y, Jiang S. Chin J Catal (李庆远, 季生福, 胡金勇, 蒋赛. 催化学报), 2013, 34: 1462
|
| [18] | Dasari M A, Kiatsimkul P P, Sutterilin W R, Suppes G J. Appl Catal A, 2005, 281: 225
|
| [19] | Gil S, Marchena M, Fernandez C M, Samchez-Silca L, Romero A, Valverde J L. Appl Catal A, 2013, 450: 189
|
| [20] | Takagaki A, Iwatani K, Nishimura S, Ebitani K. Green Chem, 2010, 12: 578
|
| [21] | Corma A, Iborra S, Velty A. Chem Rev, 2007, 107: 2411
|
| [22] | Balaraju M, Rekha V, Sai P, Prasad P S S, Devo B L A P, Prasad R B N, Lingaiah N. Appl Catal A, 2009, 354: 82
|
| [23] | Xia S X, Nie R F, Lu X Y, Wang L N, Chen P, Hou Z Y. J Catal, 2012, 296: 1
|
| [24] | Yin A Y, Guo X Y, Dai W L, Fan K N. Green Chem, 2009, 11: 1514
|
| [25] | Yu W Q, Zhao J, Ma H, Miao H, Song Q, Xu J. Appl Catal A, 2010, 1-2: 73
|
| [26] | Wang J, Shen S H, Li B D, Lin H Q, Yuan Y Z. Chem Lett, 2009, 38: 572
|
| [27] | Van Ryneveld E, Mahomed A S, Heerden P S, Friedrich H B. Catal Lett, 2011, 141: 958
|
| [28] | Guan J, Chen X F, Peng G W, Wang X C, Cao Q, Lan Z G, Mu X D. Chin J Catal (关静, 陈秀芳, 彭功名, 王喜成, 曹泉, 兰峥岗, 牟新东. 催化学报), 2013, 34: 1656
|
| [29] | Liu L J, Zhang Y H, Wang A G, Zhang T. Chin J Catal (刘龙杰, 张艳华, 王爱琴, 张涛. 催化学报), 2012, 33: 1257
|
| [30] | Hamzah N, Nordin N M, Nadzri A H A, Nik Y A, Kassim M B, Yarmo M A. Appl Catal A, 2012, 419-420: 133
|
| [31] | Zhou W, He D H. Green Chem, 2009, 11: 1146
|
| [32] | Zhang C, Zhou W, Liu S X. J Phys Chem B, 2005, 109: 24319
|
| [33] | Ma L, He D H. Top Catal, 2009, 52: 834
|
| [34] | Karim A M, Prasad V, Mpourmpakis G, Lonergan W W, Frenkel A I, Chen J, Vlachos D G. J Am Chem Soc, 2009, 131: 12230
|
| [35] | Lin B Y, Wei K M, Lin J X, Ni J. Catal Commun, 2013, 39: 14
|
| [36] | Balaraju M, Rekha V, Sai P, Devi B L A P, Prasad R B N, Prasad P S S, Lingaiah N. Appl Catal A, 2010, 384: 107
|
| [37] | Carballo J M G, Yang J, Holmen A, Garcia-Rodríguez S, Rojas S, Ojeda M, Fierro J L G. J Catal, 2011, 284: 102
|
Full-Text
|
|
Contact Us
service@oalib.com QQ:3279437679 
WhatsApp +8615387084133
|
|
