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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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Ru/ZSM-5催化葡萄糖选择性加氢制备山梨醇
DOI: 10.1016/S1872-2067(14)60077-2, PP. 733-740
Keywords: 加氢,葡萄糖,山梨醇,钌,ZSM-5
Abstract:
？采用无有机模板剂一步法制备了Ru/ZSM-5催化剂，利用X射线衍射、N2吸附-脱附、NH3-程序升温脱附和CO2-程序升温脱附、扫描电镜和透射电镜等方法对催化剂进行了表征.考察了反应温度、钌负载量和催化剂重复利用等因素对Ru/ZSM-5上葡萄糖加氢反应性能的影响，并与浸渍法制备的Ru/ZSM-5催化剂进行了对比.结果表明，与传统浸渍法相比，一步法制备的Ru/ZSM-5催化剂钌粒子具有更高的分散性和稳定性.在120℃和4MPa的温和反应条件下，葡萄糖接近完全转化，山梨醇选择性高达99.2%，催化剂可重复利用5次，仍保持较高活性.
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