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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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Sorbitolhydrogenolysistoglycolsbysupportedrutheniumcatalysts
DOI: 10.1016/S1872-2067(14)60086-3, PP. 614-621
Keywords: Sorbitol,Glycols,Hydrogenolysis,Ruthenium,Oxidesupports
Abstract:
？SupportedRucatalystswerepreparedbywetimpregnationtoevaluatetheroleofdifferentoxidesupports(Al2O3,SiO2,TiO2,ZrO2)insorbitolhydrogenolysistoglycols.X-raydiffraction,transmissionelectronmicroscopy,hydrogenchemisorption,X-rayphotoelectronspectroscopy,andNH3temperature-programmeddesorptionwereusedtocharacterizethecatalysts,whichwereactiveinthehydrogenolysisofsorbitol.ThesupportaffectedboththephysicochemicalpropertiesandcatalyticbehaviorofthesupportedRuparticles.ThecharacterizationresultsrevealedthattheRu/Al2O3catalysthasahighsurfaceacidity,partiallyoxidizedRuspeciesonthesurface,andahighersurfaceRu/Alatomicratio,whichgaveitthehighestselectivityandyieldtoglycols.
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