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催化学报  2011 

吡咯亚胺配体与过渡金属的反应性及其催化烯烃聚合

DOI: 10.3724/SP.J.1088.2011.10423, PP. 1439-1445

Keywords: 吡咯亚胺配体,过渡金属配合物,烯烃聚合,电子效应

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Abstract:

？在经典的Brookhart吡啶双亚胺后过渡金属烯烃聚合催化剂基础上,用吡咯五元环代替吡啶六元环骨架可得到具有不同电子效应的新型吡咯亚胺配体.通过吡咯环特殊的电子效应和位阻效应可设计出种类繁多的有别于吡啶亚胺配体的配合物.综述了吡咯亚胺配体与前过渡金属(Ti,Zr等)、后过渡金属(Fe,Co,Ni,Pd等)、稀土金属(Y,Ir,Lu,Nd等)以及其它金属(Cu,U,Cr等)的配位方式、配合物的结构类型、反应性及其催化烯烃聚合反应性能.

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