|
OALib Journal期刊
ISSN: 2333-9721
费用：99美元
|
|
|
|
CeO2/Ni/Mo/SBA-15甲烷二氧化碳重整催化剂的表征和催化性能
DOI: 10.1016/S1872-2067(11)60347-1, PP. 637-644
Keywords: 二氧化碳重整,甲烷,镍,钼,介孔分子筛SBA-15,铈修饰
Abstract:
？考察了CeO2修饰及未修饰的Ni/Mo/SBA-15催化剂在CH4-CO2重整上的催化性能并采用N2吸脱附、CO2程序升温脱附、H2程序升温还原、傅里叶红外光谱、X射线衍射、扫描电子显微镜和X射线光电子能谱对催化剂进行了表征.结果表明,在常压,800oC条件下,经过100h在线评价后,Ni/Mo/SBA-15和CeO2/Ni/Mo/SBA-15催化剂仍具有高的反应活性和规整的六方介孔结构,其中CeO2修饰的CeO2/Ni/Mo/SBA-15催化剂表面没有积炭形成,表明CeO2的加入促进了Ni物种在SBA-15介孔分子筛表面的分散,从而阻止了Ce/Ni/Mo/SBA-15催化剂上Ni的烧结和积炭.
| [1] | Yan B H, Wang Q, Jin Y, Cheng Y. Plasma Chem Plasma Process, 2010, 30: 257
|
| [2] | Frontera P, Aloise A, Macario A, Antonucci P L, Crea F, Giordano G, Nagy J B. Top Catal, 2010, 53: 265
|
| [3] | Kohn M P, Castaldi M J, Farrauto R J. Appl Catal B, 2010, 94: 125
|
| [4] | Pompeo F, Nichio N N, Souza M M V M, Cesar D V, Ferretti O A, Schmal M. Appl Catal A, 2007, 316: 175
|
| [5] | Fan M S, Abdullah A Z, Bhatia S. ChemCatChem, 2009, 1:192
|
| [6] | Kusakabe K, Sotowa K I, Eda T, Iwamoto Y. Fuel Process Technol, 2004, 86: 319
|
| [7] | Ishihara A, Qian E W, Finahari I N, Sutrisna I P, Kabe T. Fuel, 2005, 84: 1462
|
| [8] | Yang M, Papp H. Catal Today, 2006, 115: 199
|
| [9] | Basile F, Fornasari G, Gazzano M, Kiennemann A, Vaccari A J. J Catal, 2003, 217: 245
|
| [10] | Mehr J Y, Jozani K J, Pour A N, Zamani Y J. React Kinet Catal Lett, 2002, 75: 267
|
| [11] | Chen K, Xie S, Iglesia E, Bell A T. J Catal, 2000, 189: 421
|
| [12] | Lim S, Ciuparu D, Chen Y, Pfefferle L, Haller G L. J Phys Chem B, 2004, 108: 20095
|
| [13] | Craciun R, Daniell W, Knozinger H. Appl Catal A, 2002, 230: 153
|
| [14] | Wang Y, Chin Y H, Rozmiarek R T, Johnson B R, Gao Y, Watson J, Tonkovich A Y L, Vander Wie D P. Catal Today, 2004, 98: 575
|
| [15] | Jeong J H, Lee J W, Seo D J, Seo Y, Yoon W L, Lee D K, Kim D H. Appl Catal A, 2006, 302:151
|
| [16] | Yang Z B, Zhang Y Y, Wang X G, Zhang Y W, Lu X G, Ding W Z. Energy Fuels, 2010, 24: 785
|
| [17] | Enger B C, Lodeng R, Holmen A. Catal Lett, 2010, 134: 13
|
| [18] | 柴晓燕, 尚书勇, 刘改焕, 陶旭梅, 李祥, 白玫瑰, 戴晓雁, 印永祥. 催化学报 (Chai X Y, Shang Sh Y, Liu G H, Tao X M, Li X, Bai M G, Dai X Y, Yin Y X. Chin J Catal), 2010, 31: 353
|
| [19] | Nandini A, Pant K K, Dhingra S C. Appl Catal A, 2005, 290: 166
|
| [20] | Pechimuthu N A, Pant K K, Dhingra S C. Ind Eng Chem Res, 2007, 46: 1731
|
| [21] | Wang W, Stagg-Williams S M, Noronha F B, Mattos L V, Passos F B. Catal Today, 2004, 98: 553
|
| [22] | Roh H S, Potdar H S, Jun K W. Catal Today, 2004, 95: 39
|
| [23] | Shah P, Ramaswamy A V, Lazar K, Ramaswamy V. Appl Catal A, 2004, 273: 239
|
| [24] | Timofeeva M N, Jhung S H, Hwang Y K, Kim D K, Panchenko V N, Melgunov M S, Chesalov Y A, Chang J S. Appl Catal, 2007, 317: 1
|
| [25] | Park Y, Kang T, Lee J, Kim P, Kim H, Yi J. Catal Today, 2004, 97: 195
|
| [26] | Huang J, Ma R, Huang T, Zhang A, Huang W. J Nat Gas Chem, 2011, 20: 465
|
| [27] | Aneggi E, Boaro M, de Leitenburg C, Dolcetti G, Trovarelli A J. J Alloys Compd, 2006, 408: 1096
|
| [28] | Damyanova S, Pawelec B, Arishtirova K, Martinez Huerta M V, Flerro J L G. Appl Catal B, 2009, 89: 149
|
| [29] | Ruiz J A C, Passos F B, Bueno J M C, Souza-Aguiar E F, Mattos L V, Noronha F B. Appl Catal A, 2008, 334: 259
|
| [30] | Hou Z Y, Yokota O, Tanaka T, Yashima T. Catal Lett, 2003, 89: 121
|
| [31] | Montoya J A, Romero-Pascual E, Gimon C, Del Angel P, Monzon A. Catal Today, 2000, 63: 71
|
| [32] | Roh H-S, Jun K-W, Dong W-S, Chang J-S, Park S-E, Joe Y-I. J Mol Catal A, 2002, 181: 137
|
| [33] | Osaki T, Tanaka T, Horiuchi T, Sugiyama T, Suzuki K, Mori T. Appl Organomet Chem, 2000, 14: 789 3.0.CO;2-S target="_blank">
|
| [34] | Tomishige K, Chen Y G, Fujimoto K. J Catal, 1999, 181: 91
|
| [35] | Xu G, Shi K, Gao Y, Xu H, Wei Y. J Mol Catal A, 1999, 147: 47
|
| [36] | Chen J X, Wang R J, Zhang J Y, He F, Han S. J Mol Catal A, 2005, 235: 302
|
| [37] | Ji L, Li H, Zhao F, Chen J, Zhou H. Diamond Relat Mater, 2008, 17: 1949
|
| [38] | Solymosi F, Cserenyi J, Szoke A, Bansagi T, Oszko A. J Catal, 1997, 165: 150
|
| [39] | Zhao D, Feng J, Huo Q, Stucky G D. Science, 1998, 279: 548
|
Full-Text
|
|
Contact Us
service@oalib.com QQ:3279437679 
WhatsApp +8615387084133
|
|
