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Physics  2013 

High-order harmonic generation from field-distorted orbitals

DOI: 10.1103/PhysRevA.87.043424

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Abstract:

We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results allow us to suggest that field-distortion is the reason why the two-center interference minimum has never been observed experimentally in N2. We propose experimental parameters which should allow an observation of the two-center interference minimum.

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