全部 标题 作者
关键词 摘要

OALib Journal期刊
ISSN: 2333-9721
费用:99美元

查看量下载量

相关文章

更多...

“Color-Tripole Ice” as a Conceptual Generalization of “Spin Ice”

DOI: 10.1155/2013/836168

Full-Text   Cite this paper   Add to My Lib

Abstract:

“Spin Ice” is an exotic type of frustrated magnet realized in “pyrochlore” materials Ho2Ti2O7, Dy2Ti2O7, Ho2Sn2O7, and so forth, in which magnetic atoms (spins) reside on a sublattice made of the vertices of corner-sharing tetrahedra. Each spin is Ising-like with respect to a local axis which connects the centers of two tetrahedra sharing the vertex occupied by the spin. The macroscopically degenerate ground states of these magnets obey the “two-in two-out” “ice rule” within each tetrahedron. Magnetic monopoles and antimonopoles emerge as elementary excitations, “fractionalizing” the constituent magnetic dipoles. This system is also a novel type of statistical mechanical system. Here we introduce a conceptual generalization of “spin ice” to what we shall call “color-tripole ice,” in which three types of “color charges” can emerge as elementary excitations, which are Abelian approximations of the color charges introduced in high energy physics. Two two-dimensional (2D) models are introduced first, where the color charges are found to be 1D and constrained 2D, respectively. Generalizations of these two models to 3D are then briefly discussed. In the second one the color charges are likely 3D. Pauling-type estimates of the “residual (or zero-point) entropy” are also made for these models. 1. Introduction Frustration and fractionalization are two fundamental concepts in modern condensed matter physics. Frustration simply means the existence of competing interactions that cannot be minimized simultaneously. It could result from more than one kind of interactions present in the system, but when the interactions are all of one kind, frustration can still arise from the geometric arrangement of the constituent entities of the system (i.e., atoms, spins, etc.); it is then referred to as “geometric frustration” [1–3]. Spin systems have offered paradigmatic examples of these concepts: [4] spin glass is a simple example of a richly frustrated system, where ferromagnetic and antiferromagnetic bonds are randomly distributed in a spin system, leading to disordered, macroscopically degenerate ground states, and a finite residual or zero-point entropy. Antiferromagnetic Ising model on a two-dimensional triangular lattice is a simple example of geometric frustration, with also disordered, macroscopically degenerate ground states and finite residual entropy, even though there is only one kind of (antiferromagnetic) interaction in the system, acting between all nearest-neighbor pairs of “Ising spins,” which just mean quantized magnetic dipoles in strong uniaxial local

References

[1]  R. Moessner and A. P. Ramirez, “Geometrical frustration,” Physics Today, vol. 59, no. 2, pp. 24–29, 2006.
[2]  R. Moessner, “Magnets with strong geometric frustration,” Canadian Journal of Physics, vol. 79, no. 11-12, pp. 1283–1294, 2001.
[3]  J. E. Greedan, “Geometrically frustrated magnetic materials,” Journal of Materials Chemistry, vol. 11, no. 1, pp. 37–53, 2001.
[4]  H. T. Diep, Ed., Frustrated Spin Systems, World Scientific Publishing, Singapore, 2004.
[5]  W. P. Su, J. R. Schrieffer, and A. J. Heeger, “Soliton excitations in polyacetylene,” Physical Review B, vol. 22, no. 4, pp. 2099–2111, 1980.
[6]  R. B. Laughlin, “Anomalous quantum Hall effect: an incompressible quantum fluid with fractionally charged excitations,” Physical Review Letters, vol. 50, no. 18, pp. 1395–1398, 1983.
[7]  S. T. Bramwell and M. J. P. Gingras, “Spin Ice state in frustrated magnetic pyrochlore materials,” Science, vol. 294, no. 5546, pp. 1495–1501, 2001.
[8]  J. Snyder, J. S. Slusky, R. J. Cava, and P. Schiffer, “How “Spin Ice” freezes,” Nature, vol. 413, no. 6851, pp. 48–51, 2001.
[9]  S. T. Bramwell, M. J. Harris, B. C. Den Hertog et al., “Spin correlations in Ho2Ti2O7: a dipolar Spin Ice system,” Physical Review Letters, vol. 87, no. 4, Article ID 047205, 2001.
[10]  B. C. den Hertog and M. J. P. Gingras, “Dipolar interactions and origin of Spin Ice in ising pyrochlore magnets,” Physical Review Letters, vol. 84, no. 15, pp. 3430–3433, 2000.
[11]  R. Siddharthan, B. S. Shastry, A. P. Ramirez, A. Hayashi, R. J. Cava, and S. Rosenkranz, “Ising pyrochlore magnets: low-temperature properties, “ice rules,” and beyond,” Physical Review Letters, vol. 83, no. 9, pp. 1854–1857, 1999.
[12]  L. Pauling, The Nature of the Chemical Bond, Cornell University Press, Ithaca, NY, USA, 1945.
[13]  A. P. Ramirez, A. Hayashi, R. J. Cava, R. Siddharthan, and B. S. Shastry, “Zero-point entropy in ‘Spin Ice’,” Nature, vol. 399, no. 6734, pp. 333–335, 1999.
[14]  C. Castelnovo, R. Moessner, and S. L. Sondhi, “Magnetic monopoles in Spin Ice,” Nature, vol. 451, no. 7174, pp. 42–45, 2008.
[15]  M. J. Harris, S. T. Bramwell, P. C. W. Holdsworth, and J. D. M. Champion, “Liquid-gas critical behavior in a frustrated pyrochlore ferromagnet,” Physical Review Letters, vol. 81, no. 20, pp. 4496–4499, 1998.
[16]  J. S. Gardner, M. J. P. Gingras, and J. E. Greedan, “Magnetic pyrochlore oxides,” Reviews of Modern Physics, vol. 82, no. 1, pp. 53–107, 2010.
[17]  C. L. Henley, “The “Coulomb Phase” in frustrated systems,” Annual Review of Condensed Matter Physics, vol. 1, pp. 179–210, 2010.
[18]  C. Castelnovo, R. Moessner, and S. L. Sondhi, “Spin Ice, fractionalization, and topological order,” Annual Review of Condensed Matter Physics, vol. 3, pp. 35–55, 2012.
[19]  L. Balents, “Spin liquids in frustrated magnets,” Nature, vol. 464, no. 7286, pp. 199–208, 2010.
[20]  W. R. Branford, “Emergent magnetic monopoles in frustrated magnetic systems,” Philosophical Transactions of the Royal Society A, vol. 370, no. 1981, pp. 5702–5704, 2012.
[21]  A. P. Ramirez, C. L. Broholmb, R. J Cavac, and G. R. Kowacha, “Geometrical frustration, Spin Ice and negative thermal expansion—the physics of underconstraint,” Physica B, vol. 280, no. 1–4, pp. 290–295, 2000.
[22]  R. F. Wang, C. Nisoli, R. S. Freitas et al., “Artificial “Spin Ice” in a geometrically frustrated lattice of nanoscale ferromagnetic islands,” Nature, vol. 439, no. 303, p. 306, 2006.
[23]  S. Ladak, D. E. Read, G. K. Perkins, L. F. Cohen, and W. R. Branford, “Direct observation of magnetic monopole defects in an artificial spin-ice system,” Nature Physics, vol. 6, no. 5, pp. 359–363, 2010.
[24]  G. M?ller and R. Moessner, “Artificial square ice and related dipolar nanoarrays,” Physical Review Letters, vol. 96, no. 23, Article ID 237202, 2006.
[25]  G. M?ller and R. Moessner, “Magnetic multipole analysis of kagome and artificial spin-ice dipolar arrays,” Physical Review B, vol. 80, no. 14, Article ID 140409, 2009.
[26]  C. Nisoli, R. Wang, J. Li et al., “Ground state lost but degeneracy found: the effective thermodynamics of artificial Spin Ice,” Physical Review Letters, vol. 98, no. 21, Article ID 217203, 2007.
[27]  J. P. Morgan, A. Stein, S. Langridge, and C. H. Marrows, “Thermal ground-state ordering and elementary excitations in artificial magnetic square ice,” Nature Physics, vol. 7, no. 1, pp. 75–79, 2011.
[28]  Z. Budrikis, P. Politi, R. L. Stamps, et al., “Vertex dynamics in finite two-dimensional square Spin Ices,” Physical Review Letters, vol. 105, no. 1, Article ID 017201, 4 pages, 2010.
[29]  C. Nisoli, J. Li, X. Ke, D. Garand, P. Schiffer, and V. H. Crespi, “Effective temperature in an interacting vertex system: theory and experiment on artificial Spin Ice,” Physical Review Letters, vol. 105, no. 4, Article ID 047205, 2010.
[30]  J. Li, X. Ke, S. Zhang et al., “Comparing artificial frustrated magnets by tuning the symmetry of nanoscale permalloy arrays,” Physical Review B, vol. 81, no. 9, Article ID 092406, 2010.
[31]  P. Mellado, O. Petrova, Y. Shen, and O. Tchernyshyov, “Dynamics of magnetic charges in artificial Spin Ice,” Physical Review Letters, vol. 105, no. 18, Article ID 187206, 4 pages, 2010.
[32]  L. A. Mól, R. L. Silva, R.C. Silva, A. R. Pereira, W. A. Moura-Melo, and B. V. Costa, “Magnetic monopole and string excitations in two-dimensional Spin Ice,” Journal of Applied Physics, vol. 106, no. 6, Article ID 063913, 5 pages, 2009.
[33]  A. Schumann, B. Sothmann, P. Szary, and H. Zabel, “Charge ordering of magnetic dipoles in artificial honeycomb patterns,” Applied Physics Letters, vol. 97, no. 2, Article ID 022509, 2010.
[34]  Y. Qi, T. Brintlinger, and J. Cumings, “Direct observation of the ice rule in an artificial kagome Spin Ice,” Physical Review B, vol. 77, no. 9, Article ID 094418, 2008.
[35]  E. Mengotti, L. J. Heyderman, A. F. Rodríguez, F. Nolting, R. V. Hügli, and H. B. Braun, “Real-space observation of emergent magnetic monopoles and associated Dirac strings in artificial kagome Spin Ice,” Nature Physics, vol. 7, no. 1, pp. 68–74, 2011.
[36]  E. Mengotti, L. J. Heyderman, A. Fraile Rodríguez et al., “Building blocks of an artificial kagome Spin Ice: photoemission electron microscopy of arrays of ferromagnetic islands,” Physical Review B, vol. 78, no. 14, Article ID 144402, 2008.
[37]  N. Rougemaille, F. Montaigne, B. Canals et al., “Artificial kagome arrays of nanomagnets: a frozen dipolar Spin Ice,” Physical Review Letters, vol. 106, no. 5, Article ID 057209, 2011.
[38]  S. A. Daunheimer, O. Petrova, O. Tchernyshyov, and J. Cumings, “Reducing disorder in artificial kagome Ice,” Physical Review Letters, vol. 107, no. 16, Article ID 167201, 4 pages, 2011.
[39]  G.-W. Chern, P. Mellado, and O. Tchernyshyov, “Two-stage ordering of spins in dipolar Spin Ice on the kagome lattice,” Physical Review Letters, vol. 106, no. 20, Article ID 207202, 2011.
[40]  K. Matsuhira, Z. Hiroi, T. Tayama, S. Takagi, and T. Sakakibara, “A new macroscopically degenerate ground state in the Spin Ice compound Dy2Ti2O7 under a magnetic field,” Journal of Physics Condensed Matter, vol. 14, no. 29, pp. L559–L565, 2002.
[41]  T. Sakakibara, T. Tayama, Z. Hiroi, K. Matsuhira, and S. Takagi, “Observation of a liquid-gas-type transition in the pyrochlore Spin Ice compound Dy2Ti2O7 in a magnetic field,” Physical Review Letters, vol. 90, no. 20, Article ID 207205, 2003.
[42]  H. Kadowaki, N. Doi, Y. Aoki, et al., “Observation of magnetic monopoles in Spin Ice,” Journal of the Physical Society of Japan, vol. 78, Article ID 103706, 4 pages, 2009.
[43]  A. S. Wills, R. Ballou, and C. Lacroix, “Model of localized highly frustrated ferromagnetism: the kagomé Spin Ice,” Physical Review B, vol. 66, no. 14, Article ID 144407, 2002.
[44]  E. Mengotti, L. J. Heyderman, A. F. Rodríguez, F. Nolting, R. V. Hügli, and H. B. Braun, “Real-space observation of emergent magnetic monopoles and associated Dirac strings in artificial kagome Spin Ice,” Nature Physics, vol. 7, no. 1, pp. 68–74, 2011.
[45]  R. Moessner and S. L. Sondhi, “Theory of the [111] magnetization plateau in Spin Ice,” Physical Review B, vol. 68, no. 6, Article ID 064411, 12 pages, 2003.
[46]  Z. Hiroi, K. Matsuhira, S. Takagi, T. Tayama, and T. Sakakibara, “Specific heat of kagomé Ice in the pyrochlore oxide Dy2Ti2O7,” Journal of the Physical Society of Japan, vol. 72, no. 2, pp. 411–418, 2003.
[47]  R. Higashinaka, H. Fukazawa, and Y. Maeno, “Anisotropic release of the residual zero-point entropy in the Spin Ice compound Dy22O7: kagome Ice behavior,” Physical Review B, vol. 68, no. 1, Article ID 014415, pp. 144151–144155, 2003.
[48]  T. Fennell, S. T. Bramwell, D. F. McMorrow, P. Manuel, and A. R. Wildes, “Pinch points and Kasteleyn transitions in kagome Ice,” Nature Physics, vol. 3, no. 8, pp. 566–572, 2007.
[49]  M. Udagawa, M. Ogata, and Z. Hiroi, “Exact result of ground-state entropy for ising pyrochlore magnets under a magnetic field along [111] axis,” Journal of the Physical Society of Japan, vol. 71, no. 10, pp. 2365–2368, 2002.
[50]  Y. Tabata, H. Kadowaki, K. Matsuhira et al., “Kagomé Ice state in the dipolar Spin Ice Dy2Ti2O7,” Physical Review Letters, vol. 97, no. 25, Article ID 257205, 2006.
[51]  S. V. Isakov, K. S. Raman, R. Moessner, and S. L. Sondhi, “Magnetization curve of Spin Ice in a [111] magnetic field,” Physical Review B, vol. 70, no. 10, Article ID 104418, 2004.
[52]  H. Aoki, T. Sakakibara, K. Matsuhira, and Z. Hiroi, “Magnetocaloric effect study on the pyrochlore Spin Ice compound Dy2Ti2O7 in a [111] magnetic field,” Journal of the Physical Society of Japan, vol. 73, no. 10, pp. 2851–2856, 2004.
[53]  J. M. Hopkinson and H. Y. Kee, “Geometric frustration inherent to the trillium lattice, a sublattice of the B20 structure,” Physical Review B, vol. 74, no. 22, Article ID 224441, 14 pages, 2006.
[54]  A. Dong, X. Ye, J. Chen, and C. B. Murray, “Two-dimensional binary and ternary nanocrystal superlattices: the case of monolayers and bilayers,” Nano Letters, vol. 11, no. 4, pp. 1804–1809, 2011.
[55]  S. A. Chin, “Classical quark matter in one dimension: abelian approximation,” Physical Review D, vol. 17, no. 2, pp. 565–573, 1978.
[56]  K. Nagasaki and H. Yamakawa, “Dynamics of weakly bending rods: a trumbbell model,” Journal of Chemical Physics B, vol. 83, no. 12, Article ID 6480, 9 pages, 1985.
[57]  T. E. Redpath and J. M. Hopkinson, “Spin ice on the trillium lattice studied by Monte Carlo calculations,” Physical Review B, vol. 82, no. 1, Article ID 014410, 9 pages, 2010.
[58]  S. V. Isakov, J. M. Hopkinson, and H.-Y. Kee, “Fate of partial order on trillium and distorted windmill lattices,” Physical Review B, vol. 78, no. 1, Article ID 014404, 2008.
[59]  N. A. Hill, “Why are there so few magnetic ferroelectrics?” Journal of Physical Chemistry B, vol. 104, no. 29, pp. 6694–6709, 2000.
[60]  K. Ueda, H. Tabata, and T. Kawai, “Coexistence of ferroelectricity and ferromagnetism in BiFeO3-BaTiO3 thin films at room temperature,” Applied Physics Letters, vol. 75, no. 4, pp. 555–557, 1999.
[61]  M.-H. Tsai, Y.-H. Tang, and S. K. Dey, “Co-existence of ferroelectricity and ferromagnetism in 1.4?nm SrBi2Ta2O11 film,” Journal of Physics Condensed Matter, vol. 15, no. 46, pp. 7901–7915, 2003.
[62]  J. H. Lee, L. Fang, E. Vlahos et al., “A strong ferroelectric ferromagnet created by means of spin-lattice coupling,” Nature, vol. 476, article 114, 2011.
[63]  Y. Shimakawa, M. Azuma, and N. Ichikawa, “Multiferroic compounds with double-perovskite structures,” Materials, vol. 4, no. 1, pp. 153–168, 2011.
[64]  W. Fa, C. Luo, and J. Dong, “Coexistence of ferroelectricity and ferromagnetism in tantalum clusters,” Journal of Chemical Physics, vol. 125, no. 11, Article ID 114305, 2006.
[65]  P. B. Allen, A. G. Abanov, and R. Requist, “Quantum electrical dipole in triangular systems: a model for spontaneous polarity in metal clusters,” Physical Review A, vol. 71, no. 4, Article ID 043203, 10 pages, 2005.

Full-Text

Contact Us

service@oalib.com

QQ:3279437679

WhatsApp +8615387084133