The vertical structure of aerosol optical and physical properties was measured by Lidar in Eastern Kyrgyzstan, Central Asia, from June 2008 to May 2009. Lidar measurements were supplemented with surface-based measurements of PM2.5 and PM10 mass and chemical composition in both size fractions. Dust transported into the region is common, being detected 33% of the time. The maximum frequency occurred in the spring of 2009. Dust transported to Central Asia comes from regional sources, for example, Taklimakan desert and Aral Sea basin, and from long-range transport, for example, deserts of Arabia, Northeast Africa, Iran, and Pakistan. Regional sources are characterized by pollution transport with maximum values of coarse particles within the planetary boundary layer, aerosol optical thickness, extinction coefficient, integral coefficient of aerosol backscatter, and minimum values of the ?ngstr?m exponent. Pollution associated with air masses transported over long distances has different characteristics during autumn, winter, and spring. During winter, dust emissions were low resulting in high values of the ?ngstr?m exponent (about 0.51) and the fine particle mass fraction (64%). Dust storms were more frequent during spring with an increase in coarse dust particles in comparison to winter. The aerosol vertical profiles can be used to lower uncertainty in estimating radiative forcing. 1. Introduction The solution to many practical problems in the field of environmental and human health protection is connected with the need for improved information about atmospheric aerosols, in particular, levels of pollution and the physicochemical properties of particles. This type of information is especially important for the Central Asian continent due to the large regions with high levels of particulate matter (PM) emissions and a lack of ambient measurement data [1]. In spite of the increasing capabilities to monitor aerosol transport from satellites, there are very limited data for surface-based vertical measurements of aerosol optical properties to validate satellite results and to provide higher spatial resolution than what can be obtained by satellites. Radiative effects of the atmospheric aerosol are mainly connected to their chemical properties [2]. Due to the lack of extensive data on aerosol vertical profiles, there are large uncertainties in forecasting atmospheric radiative forcing due to differences in the vertical profiles of the atmospheric aerosol as applied in models. The ability to retrieve information on the spatial structure of aerosols by ground-based
References
[1]
J. P. Miller-Schulze, M. M. Shafer, J. J. Schauer et al., “Characteristics of fine particle carbonaceous aerosol at two remote sites in Central Asia,” Atmospheric Environment, vol. 45, no. 38, pp. 6955–6964, 2011.
[2]
P. Forster, V. Ramaswamy, P. Artaxo et al., “Changes in atmospheric constituents and in radiative forcing,” in Climate Change 2007: the Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, New York, NY, USA, 2007.
[3]
J. Huang, Q. Fu, J. Su et al., “Taklimakan dust aerosol radiative heating derived from CALIPSO observations using the Fu-Liou radiation model with CERES constraints,” Atmospheric Chemistry and Physics, vol. 9, no. 12, pp. 4011–4021, 2009.
[4]
A. Papayannis, R. E. Mamouri, V. Amiridis et al., “Systematic lidar observations of Saharan dust layers over Athens, Greece in the frame of EARLINET project (2004–2006),” Annales Geophysicae, vol. 27, no. 9, pp. 3611–3620, 2009.
[5]
C. Xie, T. Nishizawa, N. Sugimoto, I. Matsui, and Z. Wang, “Characteristics of aerosol optical properties in pollution and Asian dust episodes over Beijing, China,” Applied Optics, vol. 47, no. 27, pp. 4945–4951, 2008.
[6]
D. Müller, A. Ansmann, V. Freudenthaler et al., “Mineral dust observed with AERONET Sun photometer, Raman lidar, and in situ instruments during SAMUM 2006: shape-dependent particle properties,” Journal of Geophysical Research D, vol. 115, no. 11, Article ID D11207, 2010.
[7]
M. Tesche, A. Ansmann, D. Müller et al., “Vertical profiling of Saharan dust with Raman lidars and airborne HSRL in southern Morocco during SAMUM,” Tellus, Series B, vol. 61, no. 1, pp. 144–164, 2009.
[8]
A. Ansmann, M. Riebesell, U. Wandinger et al., “Combined raman elastic-backscatter LIDAR for vertical profiling of moisture, aerosol extinction, backscatter, and LIDAR ratio,” Applied Physics B Photophysics and Laser Chemistry, vol. 55, no. 1, pp. 18–28, 1992.
[9]
S. A. Imashev, P. V. Kozlov, L. G. Sverdlik, and B. B. Chen, “Methods of Lidar elastic backscatter signal processing,” Journal Vestnik Kyrgyz-Russian Slavic University, vol. 11, no. 7, pp. 157–164, 2011.
[10]
V. A. Korshunov, “Retrieval of integral parameters of tropospheric aerosol from two-wavelength lidar sounding,” Izvestiya—Atmospheric and Ocean Physics, vol. 43, no. 5, pp. 618–633, 2007.
[11]
B. B. Chen, L. G. Sverdlik, and P. V. Kozlov, Optics and Microphysics of Atmospheric Aerosol, Bishkek, Kyrgyzstan, 2004.
[12]
C. Ichoku, R. Levy, Y. J. Kaufman et al., “Analysis of the performance characteristics of the five-channel Microtops II Sun photometer for measuring aerosol optical thickness and precipitable water vapor,” Journal of Geophysical Research D, vol. 107, no. D13, pp. 1–17, 2002.
[13]
R. R. Draxler and G. D. Rolph, “HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model,” 2003, http://www.arl.noaa.gov/ready.
[14]
V. P. Kurbatkin, E. S. Skiba, and V. F. Ushintseva, “Characteristic of Kyrgyzstan synoptic processes,” Central Asia Institute of Hydrometeorology Research, vol. 75, no. 156, pp. 61–73, 1980.
[15]
M. Lugauer, U. Baltensperger, M. Furger et al., “Aerosol transport to the high Alpine sites Jungfraujoch (3454?m asl) and Colle Gnifetti (4452?m asl),” Tellus, Series B, vol. 50, no. 1, pp. 76–92, 1998.
[16]
M. Schüepp and H. Schirmer, “Climates of Central Europe,” in Climates of Central and Southern Europe, vol. 6, pp. 3–73, World Survey of Climatology, 1977.
[17]
B. B. Chen and L. G. Sverdlik, Optical Characteristics of the Central Tien-Shan Aerosols on the Laser Sensing Data, Bishkek, Kyrgyzstan, 2006.
[18]
A. Papayannis, H. Q. Zhang, V. Amiridis et al., “Extraordinary dust event over Beijing, China, during April 2006: lidar, Sun photometric, satellite observations and model validation,” Geophysical Research Letters, vol. 34, no. 7, Article ID L07806, 2007.
[19]
O. Dubovik, B. Holben, T. F. Eck et al., “Variability of absorption and optical properties of key aerosol types observed in worldwide locations,” Journal of the Atmospheric Sciences, vol. 59, no. 3, pp. 590–608, 2002.
[20]
A. Lampert, C. Ritter, A. Hoffmann et al., “Lidar characterization of the Arctic atmosphere during ASTAR 2007: four cases studies of boundary layer, mixed-phase and multi-layer clouds,” Atmospheric Chemistry and Physics, vol. 10, no. 6, pp. 2847–2866, 2010.
[21]
A. Ansmann, I. Mattis, D. Müller et al., “Ice formation in Saharan dust over central Europe observed with temperature/humidity/aerosol Raman lidar,” Journal of Geophysical Research D, vol. 110, no. 18, article 27, Article ID D18S12, 2005.
[22]
T. Sakai, T. Nagai, T. Kobayashi, A. Yamazaki, A. Uchiyama, and Y. Mano, “Multiwavelength and polarization lidar measurements of Asian dust layers over Tsukuba, Japan: a case study,” Atmospheric Chemistry and Physics Discussions, vol. 7, no. 4, pp. 10179–10203, 2007.
[23]
I. Uno, K. Eguchi, K. Yumimoto et al., “Asian dust transported one full circuit around the globe,” Nature Geoscience, vol. 2, no. 8, pp. 557–560, 2009.
[24]
E. Giannakaki, D. S. Balis, V. Amiridis, and S. Kazadzis, “Optical and geometrical characteristics of cirrus clouds over a Southern European lidar station,” Atmospheric Chemistry and Physics, vol. 7, no. 21, pp. 5519–5530, 2007.
[25]
G. Pappalardo, A. Amodeo, S. Amoruso, L. Mona, M. Pandolfi, and V. Cuomo, “One year of tropospheric lidar measurements of aerosol extinction and backscatter,” Annali di Geofisica, vol. 46, no. 2, pp. 401–414, 2003.
[26]
T. F. Eck, B. N. Holben, O. Dubovik et al., “Columnar aerosol optical properties at AERONET sites in central eastern Asia and aerosol transport to the tropical mid-Pacific,” Journal of Geophysical Research D, vol. 110, no. D6, article 27, 2005.
[27]
W.-N. Chen, F.-J. Tsai, C. C.-K. Chou, S.-Y. Chang, Y.-W. Chen, and J.-P. Chen, “Optical properties of Asian dusts in the free atmosphere measured by Raman lidar at Taipei, Taiwan,” Atmospheric Environment, vol. 41, no. 36, pp. 7698–7714, 2007.