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中国物理 B 2004
The dissociative ionization and Coulomb explosion of ethane by a femtosecond laser field
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Abstract:
Femtosecond laser-induced dissociation and Coulomb explosion of polyatomic molecule C_2H_6 were systematically investigated using a time-of-flight mass spectrometer and a chirped pulse amplifier laser. With the laser intensity varying from 2.4×10^{15}W/cm^{2} to 1.2×10^{16}W/cm^2, strong molecular ions C_2H_n^+ (n=0-6) and atomic ions C^{m+} (m=1-3) signals were observed. The double-peak structure of atomic ions indicated the occurrence of Coulomb explosion. Compared with the nearly isotropic distribution of C^{+}, highly charged ions C^{m+} (m=2-3) exhibited a sharply anisotropic angular distribution, which was attributed to the geometric alignment.