Laser pulse control of ultrafast heterogeneous electron transfer——The multiple vibrational mode three electronic state system
飞秒激光控制的量子分子动力学研究——多维三能级系统

With the combination of the optimal control theory and MCTDH method, optimal controlling of multi-dimensional multi-state molecule such as pyrazine is realized. The quantum dynamics of this molecule under the excitation of optimal pulse is simulated. On the basis of the simulation of two-state multi-dimensional system, we consider the two excited states as target states, and the effect of target state on the quantum dynamics is discussed.