全部 标题 作者
关键词 摘要

OALib Journal期刊
ISSN: 2333-9721
费用:99美元

查看量下载量

相关文章

更多...

The Influence of Meteorology and Atmospheric Transport Patterns on the Sulfate Levels in Raiwater in Orizaba Valley, Veracruz, Mexico

DOI: 10.4236/jep.2019.106049, PP. 821-837

Keywords: Atmospheric Transport, Rainwater, Sulfate

Full-Text   Cite this paper   Add to My Lib

Abstract:

This work assessed the relationship between synoptic circulation patterns, meteorological conditions and sulfate levels in rainwater in Orizaba Valley, Veracruz, Mexico during 2015. Samples were collected by using an automatic deposition sampler considering three climatic periods: Cold fronts or Nortes, Dry and Rainy seasons. Sulfate in rainwater was determined by turbidimetry (NMX-AA-SCFI-074-1981). A backward trajectory model (HYSPLIT) was used to characterize the potential source regions and transport pathways for air parcels arriving to Orizaba Valley; trajectories extended five days during 2015 were calculated. Mean concentrations of sulfate were 105.33, 37.5, and 52.5 μEq·l-1, for Cold Fronts, Dry and Rainy seasons, respectively. An evident dilution pattern was observed with lower concentration levels when rainfall increased. Mean values for sulfate concentration exceeded the background hemispheric value reported by Galloway et al. (1982) for remote sites (10 μEq·l-1), exceeding almost 10, 3.7 and 5.2 times, during the Nortes, Rainy and Dry seasons, respectively. From the obtained results, it was concluded that the high sulfate levels in the rainwater measured in Orizaba Valley had their origin in different upwind regional sources as a result of long-range transport during Rainy and Nortes seasons.

References

[1]  Hutchinson, T.C. and Havas, M. (2012) Effects of Acid Precipitation on Terrestrial Ecosystems. Springer, Berlin, 654 p.
https://doi.org/10.1007/978-1-4613-3033-2
[2]  Baron, J.S., Rueth, H.M., Wolfe, A.M., Nydick, K.R., Allstott, E.J., Minear, J.T. and Moraska, B. (2000) Ecosystem Responses to Nitrogen Deposition in the Colorado Front Range. Ecosystems, 3, 352-368.
https://doi.org/10.1007/s100210000032
[3]  Benedict, K.B., Day, D., Schwandner, F.M., Kreidenweis, S.M., Schichtel, B., Malm, W.C. and Collett Jr., J.L. (2013) Observations of Atmospheric Reactive Nitrogen Species in Rocky Mountain National Park and across Northern Colorado. Atmospheric Environment, 64, 66-76.
https://doi.org/10.1016/j.atmosenv.2012.08.066
[4]  Marquardt, W., Buggemann, E., Auel, R., Herrmann, H. and Moller, D. (2001) Trends of Pollution in Rain over East Germany Caused by Changing Emissions. Tellus B. Chemical and Physical Meteorology, 53, 529-541.
https://doi.org/10.1034/j.1600-0889.2001.530502.x
[5]  Shen, Z., Wong, Z., Zhang, R., Ho, K., Cao, J. and Zhang, M. (2011) Chemical Composition of Water-Soluble Ions and Carbonate Estimation in Spring Aerosol at a Semi-Arid Site of Tongyu, China. Aerosol and Air Quality Research, 10, 360-368.
https://doi.org/10.4209/aaqr.2011.02.0010
[6]  Durana, N., Casado, H., Ezcurra, A., Garcia, A. and Lacaux, J.P. (1992) Experimental Study of the Scavenging Process by Means of a Sequential Precipitation Collector, Preliminary Results. Atmospheric Environment, 26, 2437-2443.
https://doi.org/10.1016/0960-1686(92)90373-S
[7]  Cerón, R., Cerón, J., Kahl, J., Lara, R., Rangel, M. and Rustrian, E. (2018) Potential Influence of Emissions and Transport of N and S in the Orizaba Valley, Veracruz, Mexico. Agrociencia, 52, 653-670.
[8]  NMX-AA-074-1981. Análisis de aguas. Determinación del ión sulfato en aguas naturales, residuales y residuales tratadas.
[9]  Galloway, J.N., Thornton, J.D., Norton, S.A., Volchok, H.L. and McLean, R.A.N. (1982) Trace Metals in Atmospheric Deposition: A Review and Assessment. Atmospheric Environment, 16, 1677-1700.
https://doi.org/10.1016/0004-6981(82)90262-1
[10]  Ponette-González, A.G., Weathers, K.C. and Curran, L.M. (2010) Tropical Land-Cover Change Alters Biogeochemical Inputs to Ecosystems in a Mexican Montane Landscape. Ecological Applications, 20, 1820-1837.
https://doi.org/10.1890/09-1125.1
[11]  Parungo, F., Nagamoto, C., Hoyt, S. and Bravo, H.A. (1990) The Investigation of Air Quality and Acid Rain over the Gulf of Mexico. Atmospheric Environment. Part A. General Topics, 24, 109-123.
https://doi.org/10.1016/0960-1686(90)90446-T
[12]  Cerón, B., Escoffie, R.C., et al. (2015) Spatial and Temporal Distribution of through Fall Deposition of Nitrogen and Sulfur in the Mangrove Forests Associated to Terminos Lagoon. In: Nejadkoorki, F., Ed., Current Air Quality Issues, Intech Open Access Publisher, Rijeka, 147-164.
https://doi.org/10.5772/59726
[13]  Sosa, R., Bravo, H., Alarcón, A., Torres, M.C., Jaimes, M., Sánchez, P. and Granados, E. (2018) Acid Rain in a Mexian Site on the Coast of the Gulf of Mexico. Atmosfera, 31, 317-330.
https://doi.org/10.20937/ATM.2018.31.04.01
[14]  Huang, D.Y., Xu, Y.G., Peng, P., Zhang, H.H. and Lan, J.B. (2009) Chemical Composition and Seasonal Variation of Acid Deposition in Guangzhou, South China: Comparison with Precipitation in Other Major Chinese Cities. Environmental Pollution, 157, 35-41.
https://doi.org/10.1016/j.envpol.2008.08.001
[15]  Cerón, R., Padilla, H., Belmont, R., Torres, M.C., García, R. and Báez, A. (2002) Rainwater Chemical Composition at the End of the Mid-Summer Drought in the Caribbean Shore of the Yucatan Peninsula. Atmospheric Environment, 36, 2367-2374.
https://doi.org/10.1016/S1352-2310(02)00169-3
[16]  Zhang, M.Y., Wong, S.J., Wu, F.C., Yuan, X.H. and Zhang, Y. (2007) Chemical Composition of Wet Precipitation and Anthropogenic Influences at a Developing Urban Site in Southeastern China. Atmospheric Research, 84, 311-322.
https://doi.org/10.1016/j.atmosres.2006.09.003
[17]  Draxler, R.R. and Rolph, G.D. (2003) Hysplit (Hybrid Single-Particle Lagrangian Integrated Trajectory) Model.
[18]  Kahl, J.D.W., Bravo-álvarez, H., Sosa-Echeverría, R., Sánchez álvarez, P., Alarcón-Jiménez, A.L. and SotoAyala, R. (2007) Characterization of Atmospheric Transport to the El Tajín Archaeological Zone in Veracruz, México. Atmósfera, 20, 359-371.

Full-Text

Contact Us

service@oalib.com

QQ:3279437679

WhatsApp +8615387084133