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大气科学  2004 

东亚地区春季二氧化硫的输送与转化过程研究I.模式及其验证

DOI: 10.3878/j.issn.1006-9895.2004.03.01

Keywords: 关键词:硫酸盐气溶胶,三维化学输送模式,长距离输送,气粒转化

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Abstract:

结合新近评估的东亚地区污染源资料,作者利用一个耦合的区域化学输送模式系统以探讨东亚地区春季期间气象过程、气相与液相化学过程、非均相化学过程、气溶胶过程和干湿沉降过程对二氧化硫输送及转化过程的影响,并研究二氧化硫和硫酸盐气溶胶的空间分布及变化特征.模拟的二氧化硫和硫酸盐气溶胶的浓度值与2001年春季飞机和地面获取的观测值进行了比较.比较结果显示,模拟值与观测值具有很好的一致性,模式系统很好地反映了二氧化硫和硫酸盐气溶胶的分布特征和变化规律,再现了许多观测到的重要特征,为进一步分析模拟结果奠定了基础.

References

[1]  Chang, JS., RABrost, ISIsaksen et al., A three-dimensional Eulerian acid deposition model: physical concepts and formulation, JGeophysRes., 1987, 92, 14681~14700.
[2]  秦瑜、纪飞,一个欧拉型污染物沉降的中尺度模式,北京大学学报,1992,28,603~612.
[3]  雷孝恩、杨锦德、袁素珍,一个高分辨对流层物质交换模式,气象学报,1993,51,75~86.
[4]  贾新媛,区域酸沉降模式,大气科学,1993,17,732~740.
[5]  Huang, M., et al., Modeling studies of sulfur deposition and transport in east Asia, Water, Soil and Air Pollution, 1995, 85, 1921~1926.
[6]  王体健、李宗恺、南方,区域酸性沉降的数值研究 I模式,大气科学,1996,20,606~614.
[7]  高会旺、黄美元、徐华英等,欧拉型区域硫沉降模式研究,大气科学,1997,21,615~626.
[8]  Benkovitz, CM., MTSchultz, JPacyna et al., Global gridded inventories of anthropogenic emissions of sulfur and nitrogen, JGeophysRes., 1996, 101, 29239~29253.
[9]  http://hakone.eri.u-tokyo.ac.jp/vrc/erup/miyake.html.26 http://www.joss.ucar.edu/ace-asia/dm/.
[10]  Chuang, CC., JEPenner, KETaylor et al., An assessment of the radiative effects of anthropogenic sulfate, JGeophysRes., 1997, 102, 3761~3778.
[11]  Zhang Renjian, Wang Minxing, and Fu Jianzhong, Preliminary research on the size distribution of aerosols in Beijing, AdvAtmosSci., 2001, 18(2), 225~230.
[12]  Streets, DG., NYTsai, HAkimoto et al., Sulfur dioxide emissions in the period 1985-1997, 2001,AtmosEnviron., 2000, 34, 4413~4424.
[13]  Venkatram, A., PKKaramchandani, and PKMisra, Testing a comprehensive acid deposition model, AtmosEnviron., 1998, 22, 737~747.
[14]  Carmichael, GR., LKPeters, and TKitada, A second-generation model for regional-scale transport/chemistry/deposition, AtmosEnviron., 1986, 20, 173~188.
[15]  王自发、黄美元、何东阳等,关于我国和东亚酸性物质的输送研究 I三维欧拉污染物输送实用模式,大气科学,1997,21,366~378.
[16]  高会旺、黄美元、周玲等,酸性污染物欧拉型输送转化模式的研究,地球科学进展,1997,12,422~427.
[17]  Byun, DW., and JKSChing, ed., Science Algorithms of the EPA Models-3 Community Multi-scale Air Quality (CMAQ) Modeling System, NERL, Research Triangle Park, NC.,1999, 425pp.
[18]  Zhang, Meigen, IUno, SSugata et al., Numerical study of boundary layer ozone transport and photochemical production in east Asia in the wintertime, GeophysResLett., 2002, 10.1029/2001GL014368.
[19]  Zhang, Meigen, IUno, GRCarmichael et al., Large-scale structure of trace gas and aerosol distributions over the western Pacific Ocean during TRACE-P, JGeophysRes., 2003, 108(D21), 8820, doi: 10.1029 /2002JD 002946.
[20]  Carter, WPL., Condensed atmospheric photooxidation mechanisms for isoprene, AtmosEnviron., 1996, 24, 4275-4290.
[21]  Stockwell, WR., PMiddleton, and JSChang, The second generation regional acid deposition model chemical mechanism for regional air quality modeling, JGeophysRes., 1990, 95, 16343~16367.
[22]  Binkowski, FS., and UShankar, The regional particulate matter model: 1Model description and preliminary results, JGeophysRes., 1995, 100, 26191~26209.
[23]  Pielke, RA., WRCotton, RLWalko et al., A comprehensive meteorological modeling system RAMS, MeteorAtmosPhys., 1992, 49, 69~91.
[24]  Streets, DG., TCBond, GRCarmichael, et alA inventory of gaseous and primary aerosol emissions in Asia in the year 2000, JGeophysRes., 2003, 108(D21), 8809, doi: 10.1029/ 2002JD003093.
[25]  Oliver, JGJ., AFBouwman, CWMVan der Maas et al., Description of EDGAR Version 2.0: A set of global emission inventories of greenhouse gases and ozone-depleting substances for all anthropogenic and most natural sources on a per country basis and on 10×10 grid, National Institute of Public Health and the Environment (RIVM) report no771060 002 / TNO-MEP report noR96/119, 1996, 236pp.

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