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环境化学  2015 

SO42-/TiO2表面的酸性对其光催化性能的影响

Keywords: SO42-/TiO2,光催化还原,Cr(Ⅵ)

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Abstract:

采用Na2CO3溶液将SO42-/TiO2表面的SO42-洗脱下来,用热重(TG)、NH3程序升温脱附(NH3-TPD)和吡啶吸附的红外光谱等手段,分析洗脱前后SO42-/TiO2表面的酸量和酸类型的变化;在相同晶型、结晶度和吸光特性条件下,考察了SO42-/TiO2表面的酸性对Cr(Ⅵ)光催化还原效率的影响.结果表明SO42-/TiO2表面同时存在Lewis酸位和Bronsted酸位,通过Na2CO3溶液降低SO34-/TiO2表面的酸量并去除Bronsted酸位后,其对Cr(Ⅵ)的光催化活性显著降低.

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