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OALib Journal期刊
ISSN: 2333-9721
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类石墨相C3N4复合光催化剂
DOI: 10.7536/PC140823, PP. 38-46
Keywords: 光催化,g-C3N4,半导体,复合物
Abstract:
利用半导体光催化技术将太阳能转化为化学能或直接降解和矿化有机污染物,是解决能源短缺和环境污染等问题的有效途径。聚合物类石墨相氮化碳(g-C3N4)具有类似石墨烯的结构,由于其优异的化学稳定性和独特的电子能带结构,可作为太阳能转化、环境污染物降解的催化剂而得到了广泛关注。g-C3N4制备原料便宜易得、制备方法简单,可作为廉价、稳定、不含金属的可见光光催化剂应用于光催化降解污染物、水分解制氢制氧及有机合成领域。然而光生电荷易复合,使得g-C3N4的催化活性还不能满足大规模应用的需求。本文针对g-C3N4光催化活性的提高,综述了国内外在g-C3N4复合改性方面的重要研究进展,如金属/非金属掺杂、半导体复合、表面金属沉积等,并讨论了复合物的催化机理。
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