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OALib Journal期刊
ISSN: 2333-9721
费用：99美元
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光敏化铱配合物三线态材料
DOI: 10.7536/PC141038, PP. 492-502
Keywords: 铱配合物,三线态,光吸收特性,太阳能电池,能量上转化,光裂解水制氢
Abstract:
铱配合物由于高的激发单线态到三线态的量子转化效率和可调节的三线态寿命,近年来在三线态光敏化应用领域备受瞩目.科学家们就调控铱配合物发光波长和发光量子效率已建立起有效的分子设计策略和原则,但对如何调控铱配合物的可见光吸光响应,三线态量子产率和寿命等光敏化应用要求的重要光物理参数的相关探索并不多,相应的分子设计策略和原则远未建立.本文介绍了铱配合物与光敏化过程相关的光物理特征,改进铱配合物可见光吸收性能、调控三线态量子产率和寿命的分子设计策略,综述了铱配合物近年来应用于染料敏化太阳能电池、三线态-三线态湮灭能量上转化和光裂解水制氢的研究进展,梳理了铱配合物分子结构与光敏化性能之间的部分关联关系.
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