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OALib Journal期刊
ISSN: 2333-9721
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钼、钨系过氧化物在Sharpless烯烃环氧化反应中的应用*
, PP. 1886-1895
Keywords: 钼过氧化物,钨过氧化物,催化环氧化,Sharpless机理
Abstract:
钼、钨系过氧化物是非常重要的Sharpless烯烃环氧化催化剂，有着非常广泛的工业发展前景。本文综述了钼、钨系过氧化物的种类，结构，合成方法及催化活性，分析了各种钼、钨系过氧化物的特点以及在催化环氧化领域的发展现状。同时，本文还讨论了钼、钨系过氧化物催化烯烃环氧化反应的机理。评述了在催化环氧化领域中两种主要理论——Mimoun机理与Sharpless机理的争论焦点及发展现状，以及计算化学对两种理论中间过渡态的研究进展，并且重点分析了Sharpless机理的过渡态结构。此外，本文还综述了影响钼、钨系过氧化物催化剂反应活性的各种因素以及质子所产生的副反应。最后，本文对应用于催化环氧化领域的钼、钨系过氧化物未来的研究方向提出了建议。
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