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OALib Journal期刊
ISSN: 2333-9721
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电-Fenton及类电-Fenton技术处理水中有机污染物
DOI: 10.7536/PC141233, PP. 1123-1132
Keywords: 电-Fenton,类电-Fenton,羟基自由基,硫酸根自由基,有机污染物
Abstract:
传统Fenton技术是一种广泛用于水体里有机污染物降解的高级氧化技术(advancedoxidationtechnologies,AOTs)。它利用Fenton试剂Fe2+与H2O2反应生成具有强氧化性的羟基自由基(·OH),从而降解有机污染物。基于相似的机理,过渡金属离子(Fe2+、Co2+和Ag+等)也可与过硫酸盐反应生成氧化能力较强的硫酸根自由基(SO4·-),而被称之为类Fenton技术。传统Fenton技术存在Fe2+投加量多,产生的铁污泥多等缺点,因此,有学者将Fenton技术与电化学技术结合,使Fe2+在阴极得以持续再生,这就是广为关注的电-Fenton技术。同样地,类Fenton技术也遇到与传统Fenton技术相似的问题。借鉴电-Fenton技术的成功应用,基于硫酸根自由基的类电-Fenton技术应运而生。本文在介绍电-Fenton和类电-Fenton技术原理的基础上,概括了电-Fenton和类电-Fenton技术的主要类型及其改进方法,并就值得深入研究的问题和热点趋势进行了展望。
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