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OALib Journal期刊
ISSN: 2333-9721
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丙烯气相环氧化催化剂及其机理研究
DOI: 10.7536/PC140208, PP. 1307-1316
Keywords: 丙烯,环氧丙烷,反应机理,选择性氧化,金属氧化物
Abstract:
环氧丙烷是一种重要的化工中间体，广泛应用于化工、医药、食品、轻工等行业。环氧丙烷的传统工业生产方法——氯醇法和共氧化法存在着很多缺点，而最新开发的H2O2氧化法则存在催化剂寿命短、H2O2利用率低等问题没有根本解决。本文对环氧丙烷更为有前景的生产方法——以分子氧为氧源的气相选择性氧化丙烯的研究进展进行了总结，着重介绍了丙烯气相环氧化反应中的金、银、铜、铋-钼、钒、熔融盐催化剂以及其他以氧气为氧源的金属催化剂的研究进展，同时对丙烯气相氧化过程中涉及到的金催化剂的Ti活性位机理，铜、银催化剂上的金属环氧化中间物机理，银及其他金属的自由基机理作了相应的介绍。
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