%0 Journal Article %T Three-Photon Absorption and Upconversion Fluorescence Properties of Series 1,3,4-Oxadiazole Derivatives %A HUANG Wei %A LU Chang-Gui %A QIAN Ying %A LIU Chang %A WANG Zhu-Yuan %A CUI Yi-Ping %A
黄维 %A 吕昌贵 %A 钱鹰 %A 刘畅 %A 王著元 %A 崔一平 %J 中国物理快报 %D 2008 %I %X A newly synthesized 1,3,4-oxadiazole derivatives have been studied using a femtosecond Ti:sapphire laser system. The series molecules present strong three-photon absorption and frequency upeonversion fluorescence at wavelengths from 1205 nm to 1575 nm. Furthermore, there is no proportional relationship between three-photon absorption cross sections and the chemical structure transformation from monomer, dimer to trimer. Effective charge-transfer distance by π-conjugation bonds may be the contributing factor. In the experimental design, the far-field intensity distribution of femtosecond laser beam has been taken into account. We give the optimized analytical solution of nonlinear transmission in a three-photon absorption (3PA ) process when the incident beam has a Gaussian transverse spatial profile. %K 42 %K 65 %K Ky %K 33 %K 50 %K Dq %K 42 %K 70 %K Jk
上变频 %K 光子吸收 %K 荧光分析 %K 物理学 %U http://www.alljournals.cn/get_abstract_url.aspx?pcid=6E709DC38FA1D09A4B578DD0906875B5B44D4D294832BB8E&cid=47EA7CFDDEBB28E0&jid=E27DA92E19FE279A273627875A70D74D&aid=A818CCC351B4A15FFD0B7A80DBB20B53&yid=67289AFF6305E306&vid=C5154311167311FE&iid=38B194292C032A66&sid=3A9B6DFDAB34D091&eid=1BE4748776BF02C4&journal_id=0256-307X&journal_name=中国物理快报&referenced_num=0&reference_num=16