%0 Journal Article
%T Influence of microscopic parameters of chiral molecules with two couple-oscillators model on sum-frequency generation
耦合双振子模型手性分子的微观参量对和频过程的影响
%A Zheng Yang-Dong
%A Li Jun-Qing
%A Li Chun-Fei
%A
郑仰东
%A 李俊庆
%A 李淳飞
%J 物理学报
%D 2002
%I
%X In this paper, using the classical theoretical method, we derived the hyperpolarizabilities of chiral molecules applied to the two-coupled-oscillator model and gave the expressions of hyperpolarizabilities with microscopic parameters. We discussed the influence of microscopic parameters on the efficiency of sum-frequency generation through the relationship of hyperpolarizabilities and susceptibilities. The theoretical results obtained from the model are consistent with the known experimental facts.
%K chiral molecular medium
%K sum-frequency generation
%K hyperpolarizability
%K second-order susceptibility
手性分子介质
%K 和频产生
%K 超极化率
%K 二阶极化率
%U http://www.alljournals.cn/get_abstract_url.aspx?pcid=6E709DC38FA1D09A4B578DD0906875B5B44D4D294832BB8E&cid=47EA7CFDDEBB28E0&jid=29DF2CB55EF687E7EFA80DFD4B978260&aid=CE6E4F6D1A80AF99&yid=C3ACC247184A22C1&vid=987EDA49D8A7A635&iid=B31275AF3241DB2D&sid=0B2455B0C3E7C267&eid=9A3A88A3A0B8496C&journal_id=1000-3290&journal_name=物理学报&referenced_num=0&reference_num=15