%0 Journal Article %T Influence of microscopic parameters of chiral molecules with two couple-oscillators model on sum-frequency generation
耦合双振子模型手性分子的微观参量对和频过程的影响 %A Zheng Yang-Dong %A Li Jun-Qing %A Li Chun-Fei %A
郑仰东 %A 李俊庆 %A 李淳飞 %J 物理学报 %D 2002 %I %X In this paper, using the classical theoretical method, we derived the hyperpolarizabilities of chiral molecules applied to the two-coupled-oscillator model and gave the expressions of hyperpolarizabilities with microscopic parameters. We discussed the influence of microscopic parameters on the efficiency of sum-frequency generation through the relationship of hyperpolarizabilities and susceptibilities. The theoretical results obtained from the model are consistent with the known experimental facts. %K chiral molecular medium %K sum-frequency generation %K hyperpolarizability %K second-order susceptibility
手性分子介质 %K 和频产生 %K 超极化率 %K 二阶极化率 %U http://www.alljournals.cn/get_abstract_url.aspx?pcid=6E709DC38FA1D09A4B578DD0906875B5B44D4D294832BB8E&cid=47EA7CFDDEBB28E0&jid=29DF2CB55EF687E7EFA80DFD4B978260&aid=CE6E4F6D1A80AF99&yid=C3ACC247184A22C1&vid=987EDA49D8A7A635&iid=B31275AF3241DB2D&sid=0B2455B0C3E7C267&eid=9A3A88A3A0B8496C&journal_id=1000-3290&journal_name=物理学报&referenced_num=0&reference_num=15