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Consequences of Disorder on the Stability of Amorphous Solids  [PDF]
Vladimir Dailidonis,Valery Ilyin,Pankaj Mishra,Itamar Procaccia
Physics , 2015, DOI: 10.1103/PhysRevB.92.094105
Abstract: Highly acurate numerical simulations are employed to highlight the subtle but important differences in the mechanical stability of perfect crystalline solids versus amorphous solids. We stress the difference between strain values at which the shear modulus vanishes and strain values at which a plastic instability insues. The temperature dependence of the yield strain is computed for the two types of solids, showing different scaling laws: $\gamma_{_{Y}}\simeq \gamma_{_{Y}}^{0}-C_1 T^{1/3}$ for crystals versus $\gamma_{_{Y}}\simeq \gamma_{_{Y}}^{0}- C_2 T^{2/3}$ for amorphous solids.
On the Rigidity of Amorphous Solids  [PDF]
Matthieu Wyart
Physics , 2005, DOI: 10.1051/anphys:2006003
Abstract: We poorly understand the properties of amorphous systems at small length scales, where a continuous elastic description breaks down. This is apparent when one considers their vibrational and transport properties, or the way forces propagate in these solids. Little is known about the microscopic cause of their rigidity. Recently it has been observed numerically that an assembly of elastic particles has a critical behavior near the jamming threshold where the pressure vanishes. At the transition such a system does not behave as a continuous medium at any length scales. When this system is compressed, scaling is observed for the elastic moduli, the coordination number, but also for the density of vibrational modes. In the present work we derive theoretically these results, and show that they apply to various systems such as granular matter and silica, but also to colloidal glasses. In particular we show that: (i) these systems present a large excess of vibrational modes at low frequency in comparison with normal solids, called the "boson peak" in the glass literature. The corresponding modes are very different from plane waves, and their frequency is related to the system coordination; (ii) rigidity is a non-local property of the packing geometry, characterized by a length scale which can be large. For elastic particles this length diverges near the jamming transition; (iii) for repulsive systems the shear modulus can be much smaller than the bulk modulus. We compute the corresponding scaling laws near the jamming threshold. Finally, we discuss the applications of these results to the glass transition, the transport, and the geometry of the random close packing.
The Plastic Response of Magnetoelastic Amorphous Solids  [PDF]
H. G. E. Hentschel,Valery Ilyin,Itamar Procaccia
Physics , 2012, DOI: 10.1209/0295-5075/99/26003
Abstract: We address the cross effects between mechanical strains and magnetic fields on the plastic response of magnetoelastic amorphous solids. It is well known that plasticity in non-magnetic amorphous solids under external strain $\gamma$ is dominated by the co-dimension 1 saddle-node bifurcation in which an eigenvalue of the Hessian matrix vanishes at $\gamma_P$ like $\sqrt{\gamma_P-\gamma}$. This square-root singularity determines much of the statistical physics of elasto-plasticity, and in particular that of the stress-strain curves under athermal-quasistatic conditions. In this Letter we discuss the much richer physics that can be expected in magnetic amorphous solids. Firstly, magnetic amorphous solids exhibit co-dimension 2 plastic instabilities, when an external strain and an external magnetic field are applied simultaneously. Secondly, the phase diagrams promise a rich array of new effects that have been barely studied; this opens up a novel and extremely rich research program for magnetoplastic materials.
ON THE FORMATION OF AMORPHOUS SOLIDS

Zheng Zhaobo Dept,of Physics,University of Science,Technology of China,

金属学报 , 1979,
Abstract: A general survey on theories of glass or amorphous solid formation, includingthe nature of glass transformation, the theory of free volume and that of entropy,the capability on the retention of the amorphous state as well as methods for de-termining the necessary critical cooling rates etc., has been carried out. The re-sults of kinetic treatment of amorphous solid formation shown by D. Turnbulland D. R. Uhlman and their co-workers have received particular attention.
Hidden structure in amorphous solids  [PDF]
F. Inam,James P. Lewis,D. A. Drabold
Physics , 2009, DOI: 10.1002/pssa.200982877
Abstract: Recent theoretical studies of amorphous silicon [Y. Pan et al. Phys. Rev. Lett. 100 206403 (2008)] have revealed subtle but significant structural correlations in network topology: the tendency for short (long) bonds to be spatially correlated with other short (long) bonds). These structures were linked to the electronic band tails in the optical gap. In this paper, we further examine these issues for amorphous silicon, and demonstrate that analogous correlations exist in amorphous SiO2, and in the organic molecule, b-carotene. We conclude with a discussion of the origin of the effects and its possible generality.
Do Athermal Amorphous Solids Exist?  [PDF]
H. G. E. Hentschel,Smarajit Karmakar,Edan Lerner,Itamar Procaccia
Physics , 2010, DOI: 10.1103/PhysRevE.83.061101
Abstract: We study the elastic theory of amorphous solids made of particles with finite range interactions in the thermodynamic limit. For the elastic theory to exist one requires all the elastic coefficients, linear and nonlinear, to attain a finite thermodynamic limit. We show that for such systems the existence of non-affine mechanical responses results in anomalous fluctuations of all the nonlinear coefficients of the elastic theory. While the shear modulus exists, the first nonlinear coefficient B_2 has anomalous fluctuations and the second nonlinear coefficient B_3 and all the higher order coefficients (which are non-zero by symmetry) diverge in the thermodynamic limit. These results put a question mark on the existence of elasticity (or solidity) of amorphous solids at finite strains, even at zero temperature. We discuss the physical meaning of these results and propose that in these systems elasticity can never be decoupled from plasticity: the nonlinear response must be very substantially plastic.
Leggett's bound for amorphous solids  [PDF]
Giulio Biroli,Bryan Clark,Laura Foini,Francesco Zamponi
Physics , 2010, DOI: 10.1103/PhysRevB.83.094530
Abstract: We investigate the constraints on the superfluid fraction of an amorphous solid following from an upper bound derived by Leggett. In order to accomplish this, we use as input density profiles generated for amorphous solids in a variety of different manners including by investigating Gaussian fluctuations around classical results. These rough estimates suggest that, at least at the level of the upper bound, there is not much difference in terms of superfluidity between a glass and a crystal characterized by the same Lindemann ratio. Moreover, we perform Path Integral Monte Carlo simulations of distinguishable Helium 4 rapidly quenched from the liquid phase to very lower temperature, at the density of the freezing transition. We find that the system crystallizes very quickly, without any sign of intermediate glassiness. Overall our results suggest that the experimental observations of large superfluid fractions in Helium 4 after a rapid quench correspond to samples evolving far from equilibrium, instead of being in a stable glass phase. Other scenarios and comparisons to other results on the super-glass phase are also discussed.
Breakdown of continuum elasticity in amorphous solids  [PDF]
Edan Lerner,Eric DeGiuli,Gustavo Düring,Matthieu Wyart
Physics , 2013,
Abstract: We show numerically that the response of simple amorphous solids (elastic networks and particle packings) to a local force dipole is characterized by a lengthscale $\ell_c$ that diverges as unjamming is approached as $\ell_c \sim (z - 2d)^{-1/2}$, where $z \ge 2d$ is the mean coordination, and $d$ is the spatial dimension, at odds with previous numerical claims. We also show how the magnitude of the lengthscale $\ell_c$ is amplified by the presence of internal stresses in the disordered solid. Our data suggests a divergence of $\ell_c\sim (p_c-p)^{-1/4}$ with proximity to a critical internal stress $p_c$ at which soft elastic modes become unstable.
Criticality in the approach to failure in amorphous solids  [PDF]
Jie Lin,Thomas Gueudré,Alberto Rosso,Matthieu Wyart
Physics , 2015,
Abstract: Failure of amorphous solids is fundamental to various phenomena, including landslides and earthquakes. Recent experiments indicate that highly plastic regions form elongated structures that are especially apparent near the maximal shear stress $\Sigma_{\max}$ where failure occurs. This observation suggested that $\Sigma_{\max}$ acts as a critical point where the length scale of those structures diverges, possibly causing macroscopic transient shear bands. Here we argue instead that the entire solid phase ($\Sigma<\Sigma_{\max}$) is critical, that plasticity always involves system-spanning events, and that their magnitude diverges at $\Sigma_{\max}$ independently of the presence of shear bands. We relate the statistics and fractal properties of these rearrangements to an exponent $\theta$ that captures the stability of the material, which is observed to vary continuously with stress, and we confirm our predictions in elastoplastic models.
Microalloying and the mechanical properties of amorphous solids  [PDF]
H. George E. Hentschel,Michael Moshe,Itamar Procaccia,Konrad Samwer,Eran Sharon
Physics , 2015,
Abstract: The mechanical properties of amorphous solids like metallic glasses can be dramatically changed by adding small concentrations (as low as 0.1\%) of foreign elements. The glass-forming-ability, the ductility, the yield stress and the elastic moduli can all be greatly effected. This paper presents theoretical considerations with the aim of explaining the magnitude of these changes in light of the small concentrations involved. The theory is built around the experimental evidence that the microalloying elements organize around them a neighborhood that differs from both the crystalline and the glassy phases of the material in the absence of the additional elements. These regions act as {\em isotropic} defects that in unstressed systems dress the shear moduli. When strained, these defects interact with the incipient plastic responses which are quadrupolar in nature. It will be shown that this interaction interferes with the creation of system-spanning shear bands and increases the yield strain. We offer experimentally testable estimates of the lengths of nano-shear bands in the presence of the additional elements.
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