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Hyperfine interaction of Vk centres in Cs2NaYCl6 crystals
J. Barreto,J.L. Boldú,H. del Castillo,E. Mu?oz
Revista mexicana de física , 2012,
Abstract: Presentamos los resultados obtenidos por medio de la espectroscopia de resonancia paramagnetica electronica (EPR) del estudio de la interaccion hiperfina de centros Vk en los cristales de hexacloruro de cesio, sodio, itrio (Cs2NaYCl6). Estos centros de defecto electonico se crean por irradiacion a temperatura de nitrogeno liquido en los cristales de Cs2NaYCl6. Nuestros resultados son: g =2.008, g? =2.023, A =91.21(gauss) and A? =3.10 (gauss) y estos resultados se comparan con los obtenidos por Th. Pawlik y J.M. Spaeth [24] para el mismo sistema y los de D. Shoemaker [23] para cloruro de sodio.
Quantum beat spectroscopy: stimulated emission probe of hyperfine quantum beats in the atomic Cs 8p $^{2}P_{3/2}$ level  [PDF]
S. B. Bayram,P. Arndt,O. I. Popov,C. Guney,W. P. Boyle,M. D. Havey,J. McFarland
Physics , 2014, DOI: 10.1103/PhysRevA.90.062510
Abstract: Measurements of hyperfine polarization quantum beats are used determine the magnetic dipole (A) and electric quadrupole (B) coupling constants in the excited atomic Cs 8p level. The experimental approach is a novel combination of pulsed optical pumping and time-delayed stimulated emission probing of the excited level. From the measured evolution of the atomic linear polarization degree as a function of probe delay time, we determine the hyperfine coupling constants A = 7.42(6) MHz and B = 0.14(29) MHz.
Off-diagonal hyperfine interaction between the 6p1/2 and 6p3/2 levels in 133Cs  [PDF]
W. R. Johnson,H. C. Ho,Carol E. Tanner,Andrei Derevianko
Physics , 2004, DOI: 10.1103/PhysRevA.70.014501
Abstract: The off-diagonal hyperfine interaction between the 6p1/2 and 6p3/2 states in 133Cs is evaluated in third-order MBPT giving 37.3 Hz and 48.3 Hz, respectively, for second-order energies of the 6p3/2 F=3 and F=4 levels. This result is a factor of 10 smaller than one obtained from an uncorrelated first-order Dirac-Hartree-Fock calculation and used in the analysis of a recent high-precision (< 2 kHz) measurement of the 6p3/2 hyperfine structure [Gerginov et al. Phys. Rev. Lett. 91, 72301 (2003)]. The factor of 10 difference has negligible effect on the conclusions of the recent experiment but will become important for experiments carried out at a precision of better than 1 kHz.
Level-crossing spectroscopy of the 7, 9, and 10D_5/2 states of 133Cs and validation of relativistic many-body calculations of the polarizabilities and hyperfine constants  [PDF]
M. Auzinsh,K. Blushs,R. Ferber,F. Gahbauer,A. Jarmola,M. S. Safronova,U. I. Safronova,M. Tamanis
Physics , 2006, DOI: 10.1103/PhysRevA.75.022502
Abstract: We present an experimental and theoretical investigation of the polarizabilities and hyperfine constants of D_J states in 133Cs for J=3/2 and J=5/2. New experimental values for the hyperfine constant A are obtained from level-crossing signals of the (7,9,10)D_5/2 states of 133Cs and precise calculations of the tensor polarizabilities alpha_2. The results of relativistic many-body calculations for scalar and tensor polarizabilities of the (5-10)D_3/2 and (5-10)D_5/2 states are presented and compared with measured values from the literature. Calculated values of the hyperfine constants A for these states are also presented and checked for consistency with experimental values.
Characterization of Cs vapor cell coated with octadecyltrichlorosilane using coherent population trapping spectroscopy  [PDF]
Moustafa Abdel Hafiz,Vincent Maurice,Ravinder Chutani,Nicolas Passilly,Christophe Gorecki,Stéphane Guérandel,Emeric de Clercq,Rodolphe Boudot
Physics , 2015,
Abstract: We report the realization and characterization using coherent population trapping (CPT) spectroscopy of an octadecyltrichlorosilane (OTS)-coated centimeter-scale Cs vapor cell. The dual-structure of the resonance lineshape, with presence of a narrow structure line at the top of a Doppler-broadened structure, is clearly observed. The linewidth of the narrow resonance is compared to the linewidth of an evacuated Cs cell and of a buffer gas Cs cell of similar size. The Cs-OTS adsorption energy is measured to be (0.42 $\pm$ 0.03) eV, leading to a clock frequency shift rate of $2.7\times10^{-9}/$K in fractional unit. A hyperfine population lifetime, $T_1$, and a microwave coherence lifetime, $T_2$, of 1.6 and 0.5 ms are reported, corresponding to about 37 and 12 useful bounces, respectively. Atomic-motion induced Ramsey narrowing of dark resonances is observed in Cs-OTS cells by reducing the optical beam diameter. Ramsey CPT fringes are detected using a pulsed CPT interrogation scheme. Potential applications of the Cs-OTS cell to the development of a vapor cell atomic clock are discussed.
Femtosecond frequency comb measurement of absolute frequencies and hyperfine coupling constants in cesium vapor  [PDF]
Jason E. Stalnaker,Vela Mbele,Vladislav Gerginov,Tara M. Fortier,Scott A. Diddams,Leo Hollberg,Carol E. Tanner
Physics , 2010, DOI: 10.1103/PhysRevA.81.043840
Abstract: We report measurements of absolute transition frequencies and hyperfine coupling constants for the 8S_{1/2}, 9S_{1/2}, 7D_{3/2}, and 7D_{5/2} states in ^{133}Cs vapor. The stepwise excitation through either the 6P_{1/2} or 6P_{3/2} intermediate state is performed directly with broadband laser light from a stabilized femtosecond laser optical-frequency comb. The laser beam is split, counter-propagated and focused into a room-temperature Cs vapor cell. The repetition rate of the frequency comb is scanned and we detect the fluorescence on the 7P_{1/2,3/2} -> 6S_{1/2} branches of the decay of the excited states. The excitations to the different states are isolated by the introduction of narrow-bandwidth interference filters in the laser beam paths. Using a nonlinear least-squares method we find measurements of transition frequencies and hyperfine coupling constants that are in agreement with other recent measurements for the 8S state and provide improvement by two orders of magnitude over previously published results for the 9S and 7D states.
Measurement of the Kerr nonlinear refractive index of Cs vapor  [PDF]
Michelle O. Araújo,Hugo L. D. de S. Cavalcante,Marcos Oriá,Martine Chevrollier,Thierry Passerat de Silans,Romeu Castro,Danieverton Moretti
Physics , 2014, DOI: 10.1103/PhysRevA.88.063818
Abstract: Atomic vapors are systems well suited for nonlinear optics studies but very few direct measurements of their nonlinear refractive index have been reported. Here we use the z-scan technique to measure the Kerr coefficient, $n_2$, for a Cs vapor. Our results are analyzed through a four-level model, and we show that coherence between excited levels as well as cross-population effects contribute to the Kerr-nonlinearity.
An optical isolator using an atomic vapor in the hyperfine Paschen-Back regime  [PDF]
L. Weller,K. S. Kleinbach,M. A. Zentile,S. Knappe,I. G. Hughes,C. S. Adams
Physics , 2012, DOI: 10.1364/OL.37.003405
Abstract: A light, compact optical isolator using an atomic vapor in the hyperfine Paschen-Back regime is presented. Absolute transmission spectra for experiment and theory through an isotopically pure 87Rb vapor cell show excellent agreement for fields of 0.6 T. We show \pi/4 rotation for a linearly polarized beam in the vicinity of the D2 line and achieve an isolation of 30 dB with a transmission > 95 %.
Doubly magic trapping for Cs atom hyperfine clock transitions  [PDF]
A. W. Carr,M. Saffman
Physics , 2014,
Abstract: We analyze doubly magic trapping of Cs hyperfine transitions including previously neglected contributions from the ground state hyperpolarizability and the interaction of the laser light and a static magnetic field. Extensive numerical searches do not reveal any doubly magic trapping conditions for any pair of hyperfine states. However, including the hyperpolarizability reveals light intensity insensitive traps for a wide range of wavelengths at specific intensities. We then investigate the possibility of using bichromatic trapping light fields. Deploying a bichromatic scheme, we demonstrate doubly magic red and blue detuned traps for pairs of states separated by one or two single photon transitions.
Sub-Doppler spectroscopy of Rb atoms in a sub-micron vapor cell in the presence of a magnetic field  [PDF]
David Sarkisyan,Aram Papoyan,Tigran Varzhapetyan,Janis Alnis,Kaspars Blush,Marcis Auzinsh
Physics , 2003, DOI: 10.1088/1464-4258/6/3/023
Abstract: We report the first use of an extremely thin vapor cell (thickness ~ 400 nm) to study the magnetic-field dependence of laser-induced-fluorescence excitation spectra of alkali atoms. This thin cell allows for sub-Doppler resolution without the complexity of atomic beam or laser cooling techniques. This technique is used to study the laser-induced-fluorescence excitation spectra of Rb in a 50 G magnetic field. At this field strength the electronic angular momentum J and nuclear angular momentum I are only partially decoupled. As a result of the mixing of wavefunctions of different hyperfine states, we observe a nonlinear Zeeman effect for each sublevel, a substantial modification of the transition probabilities between different magnetic sublevels, and the appearance of transitions that are strictly forbidden in the absence of the magnetic field. For the case of right- and left- handed circularly polarized laser excitation, the fluorescence spectra differs qualitatively. Well pronounced magnetic field induced circular dichroism is observed. These observations are explained with a standard approach that describes the partial decoupling of I and J states.
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